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Recently, realizations of Kitaev physics have been sought in the A2IrO3 family of honeycomb iridates, originating from oxygen-mediated exchange through edge-shared octahedra. However, for the j = 1/2 Mott insulator in these materials…

Strongly Correlated Electrons · Physics 2014-03-18 Jeffrey G. Rau , Eric Kin-Ho Lee , Hae-Young Kee

The exactly solvable spin-1/2 Kitaev model on a honeycomb lattice has drawn significant interest, as it offers a pathway to realizing the long-sought after quantum spin liquid. Building upon the Kitaev model, Yao and Lee introduced another…

Strongly Correlated Electrons · Physics 2025-03-12 Derek Churchill , Emily Z. Zhang , Hae-Young Kee

In the class of materials called spin liquids, a magnetically ordered state cannot be attained even at milliKelvin temperatures because of conflicting constraints on each spin (for e.g. from geometric or exchange frustration). The resulting…

The frustrated magnet $\alpha$-RuCl$_3$ constitutes a fascinating quantum material platform that harbors the intriguing Kitaev physics. However, a consensus on its intricate spin interactions and field-induced quantum phases has not been…

Strongly Correlated Electrons · Physics 2021-07-16 Han Li , Hao-Kai Zhang , Jiucai Wang , Han-Qing Wu , Yuan Gao , Dai-Wei Qu , Zheng-Xin Liu , Shou-Shu Gong , Wei Li

YbMgGaO$_{4}$, a structurally perfect two-dimensional triangular lattice with odd number of electrons per unit cell and spin-orbit entangled effective spin-1/2 local moments of Yb$^{3+}$ ions, is likely to experimentally realize the quantum…

Strongly Correlated Electrons · Physics 2015-10-20 Yuesheng Li , Gang Chen , Wei Tong , Li Pi , Juanjuan Liu , Zhaorong Yang , Xiaoqun Wang , Qingming Zhang

We report the synthesis and properties of (H,Li)$_{6}$Ru$_{2}$O$_{6}$, which is shown to be a $J_{\text{eff}}=\frac{1}{2}$ system made out of Ru$^{3+}$ moments in a honeycomb geometry. Bulk magnetization, heat capacity, nuclear magnetic…

Strongly Correlated Electrons · Physics 2025-02-06 Sanjay Bachhar , M. Baenitz , Hubertus Luetkens , John Wilkinson , Sumiran Pujari , A. V. Mahajan

We present numerical evidence for the presence of a finite-temperature ($T$) phase transition separating paramagnet and quantum spin liquid in a three-dimensional variant of the Kitaev model defined on a hyperhoneycomb lattice in the limit…

Strongly Correlated Electrons · Physics 2015-06-17 J. Nasu , T. Kaji , K. Matsuura , M. Udagawa , Y. Motome

Quantum spin liquids (QSLs) represent highly entangled states of matter in which frustration-induced quantum fluctuations suppress any symmetry-breaking phase transition down to absolute zero, giving rise to fractionalized excitations and…

Na$_4$Ir$_3$O$_8$ is a candidate material for a 3-dimensional quantum spin-liquid on the hyperkagome lattice. We present thermodynamic measurements of heat capacity $C$ and thermal conductivity $\kappa$ on high quality polycrystalline…

Strongly Correlated Electrons · Physics 2015-06-18 Yogesh Singh , Y. Tokiwa , J. Dong , P. Gegenwart

Quantum spin liquid is an elusive state that display strong many-body entanglement with potential applications in future quantum computing. This study reports muon spin relaxation ($\mu^+$SR) measurements on a novel high-pressure…

Quantum spin liquids are long-range entangled states of matter with emergent gauge fields and fractionalized excitations. While candidate materials, such as the Kitaev honeycomb ruthenate $\alpha$-RuCl$_3$, show magnetic order at low…

Strongly Correlated Electrons · Physics 2019-07-16 I. Rousochatzakis , S. Kourtis , J. Knolle , R. Moessner , N. B. Perkins

$\rm{Sr_2CuTe_{0.5}W_{0.5}O_6}$ is a square-lattice magnet with super-exchange between S=1/2 $\rm{Cu^{2+}}$ spins mediated by randomly distributed Te and W ions. Here, using sub-K temperature and 20 $\rm{\mu}$eV energy resolution neutron…

Motivated by recent experiments on the quantum-spin-liquid candidate material LiZn2Mo3O8, we study a single-band extended Hubbard model on an anisotropic Kagome lattice with the 1/6 electron filling. Due to the partial filling of the…

Strongly Correlated Electrons · Physics 2014-08-18 Gang Chen , Hae-Young Kee , Yong Baek Kim

After the discovery of the ARECh2 (A=alkali or monovalent ions, RE=rare-earth, Ch= chalcogen) triangular lattice quantum spin liquid (QSL) family, a series of its oxide, sulfide, and selenide counterparts has been consistently reported and…

Strongly Correlated Electrons · Physics 2024-08-20 Weiwei Liu , Zheng Zhang , Dayu Yan , Jianshu Li , Zhitao Zhang , Jianting Ji , Feng Jin , Youguo Shi , Qingming Zhang

In the quest for materials hosting Kitaev spin liquids, much of the efforts have been focused on the fourth- and fifth-row transition metal compounds, which are spin-orbit coupling assisted Mott insulators. Here, we study the structural and…

Strongly Correlated Electrons · Physics 2022-12-20 Shishir Kumar Pandey , Ji Feng

We report on the magnetic properties of four isomorphous compounds of a family of quinternary oxalates down to 60 mK. In all these materials, the magnetic FeII ions with a strong magneto-crystalline anisotropy form a distorted kagome…

Strongly Correlated Electrons · Physics 2013-06-24 E. Lhotel , V. Simonet , J. Ortloff , B. Canals , C. Paulsen , E. Suard , T. Hansen , D. J. Price , P. T. Wood , A. K. Powell , R. Ballou

The quest for entangled spin excitations has stimulated intense research on frustrated magnetic systems. For almost two decades, the triangular-lattice Mott insulator $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ has been the hottest candidate for…

Strongly Correlated Electrons · Physics 2023-06-06 A. Pustogow , Y. Kawasugi , H. Sakurakoji , N. Tajima

The family of edge-sharing tri-coordinated iridates and ruthenates has emerged in recent years as a major platform for Kitaev spin liquid physics, where spins fractionalize into emergent magnetic fluxes and Majorana fermions with Dirac-like…

Quantum fluctuations enhanced by frustration and subtle interplay between competing degrees of freedom offer an ideal ground to realize novel states with fractional quantum numbers in quantum materials that defy standard theoretical…

A new quantum spin liquid (QSL) candidate material H$_{3}$LiIr$_{2}$O$_{6}$ was synthesized recently and was found not to show any magnetic order or phase transition down to low temperatures. In this work, we study the quantum dynamics of…

Strongly Correlated Electrons · Physics 2020-08-17 Shuai Wang , Long Zhang , Fa Wang
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