English

Spin liquid close to a quantum critical point in Na$_4$Ir$_3$O$_8$

Strongly Correlated Electrons 2015-06-18 v1 Materials Science

Abstract

Na4_4Ir3_3O8_8 is a candidate material for a 3-dimensional quantum spin-liquid on the hyperkagome lattice. We present thermodynamic measurements of heat capacity CC and thermal conductivity κ\kappa on high quality polycrystalline samples of Na4_4Ir3_3O8_8 down to T=500T = 500 mK and 7575 mK, respectively. Absence of long-range magnetic order down to T=75T = 75 mK strongly supports claims of a spin-liquid ground state. The constant magnetic susceptibility χ\chi below T25T \approx 25 K and the presence of a small but finite linear-TT term in C(T)C(T) suggest the presence of gapless spin excitations. Additionally, the magnetic Gru¨\ddot{\rm{u}}neisen ratio shows a divergence as T0T \rightarrow 0 K and a scaling behavior which clearly demonstrates that Na4_4Ir3_3O8_8 is situated close to a zero-field QCP.

Keywords

Cite

@article{arxiv.1312.3123,
  title  = {Spin liquid close to a quantum critical point in Na$_4$Ir$_3$O$_8$},
  author = {Yogesh Singh and Y. Tokiwa and J. Dong and P. Gegenwart},
  journal= {arXiv preprint arXiv:1312.3123},
  year   = {2015}
}

Comments

5 pages, 4 figures, PRB rapid, in press