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Possible quantum spin liquid state of CeTa$_7$O$_{19}$

Strongly Correlated Electrons 2025-03-06 v2 Materials Science

Abstract

CeTa7_7O19_{19} is a recently found two-dimensional triangular lattice antiferromagnet without showing magnetic order. We grew high-quality CeTa7_7O19_{19} single crystals and studied the low-temperature magnetic susceptibility, specific heat and thermal conductivity. The dc magnetic susceptibility and magnetization reveal its nature of effective spin-1/2, easy axis anisotropy, and antiferromagnetic spin coupling. The ultralow-temperature ac susceptibility and specific heat data indicate the absence of any phase transition down to 20 mK. The ultralow-temperature thermal conductivity (κ\kappa) at zero magnetic field exhibits a non-zero residual term κ0/T=\kappa_0/T = 0.0056 W/K2^2m. Although the magnetic field dependence of κ\kappa is rather weak, the 14 T thermal conductivity shows an essential zero residual term. All these results point to a possible ground state of quantum spin liquid.

Keywords

Cite

@article{arxiv.2503.00752,
  title  = {Possible quantum spin liquid state of CeTa$_7$O$_{19}$},
  author = {N. Li and A. Rutherford and Y. Y. Wang and H. Liang and Y. Zhou and Y. Sun and D. D. Wu and P. F. Chen and Q. J. Li and H. Wang and W. Xie and E. S. Choi and S. Z. Zhang and M. Lee and H. D. Zhou and X. F. Sun},
  journal= {arXiv preprint arXiv:2503.00752},
  year   = {2025}
}

Comments

8 pages, 6 figures, accepted for publication in Phys. Rev. B