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The honeycomb-lattice cobaltate Na$_3$Co$_2$SbO$_6$ has recently been proposed to be a proximate Kitaev quantum spin liquid~(QSL) candidate. However, non-Kitaev terms in the Hamiltonian lead to a zigzag-type antiferromagnetic~(AFM) order at…

Frustrated quantum magnets are expected to host many exotic quantum spin states like quantum spin liquid (QSL), and have attracted numerous interest in modern condensed matter physics. The discovery of the triangular lattice spin liquid…

Strongly Correlated Electrons · Physics 2018-10-02 Weiwei Liu , Zheng Zhang , Jianting Ji , Yixuan Liu , Jianshu Li , Xiaoqun Wang , Hechang Lei , Gang Chen , Qingming Zhang

A quantum spin liquid is an exotic quantum state of matter in which spins are highly entangled and remain disordered down to zero temperature. Such a state of matter is potentially relevant to high-temperature superconductivity and…

Recently, several putative quantum spin liquid (QSL) states were discovered in ${\tilde S} = 1/2$ rare-earth based triangular-lattice antiferromagnets (TLAF) with the delafossite structure. A way to clarify the origin of the QSL state in…

Yb-based magnets, with a perfect triangular lattice of pseudospin-$1/2$ Yb$^{3+}$ ions, have emerged as candidates for realizing a quantum spin-liquid state, with NaYbS$_2$ being a prominent example. Here we present the solid-solution…

Strongly Correlated Electrons · Physics 2022-06-09 Ellen Häußler , Jörg Sichelschmidt , Michael Baenitz , Eric C. Andrade , Matthias Vojta , Thomas Doert

We have investigated the thermodynamic and local magnetic properties of the Mott insulating system Ag$_{3}$LiRu$_{2}$O$_{6}$ containing Ru$^{4+}$ (4$d$$^{4}$) for novel magnetism. The material crystallizes in a monoclinic $C2/m$ structure…

Spin liquids are highly correlated yet disordered states formed by the entanglement of magnetic dipoles$^1$. Theories typically define such states using gauge fields and deconfined quasiparticle excitations that emerge from a simple rule…

$\rm Sr_2IrO_4$ is an archetypal spin-orbit-coupled Mott insulator and has been extensively studied in part because of a wide range of predicted novel states. Limited experimental characterization of these states thus far brings to light…

Strongly Correlated Electrons · Physics 2020-09-14 Feng Ye , Christina Hoffmann , Wei Tian , Hengdi Zhao , G. Cao

We report the crystal growth and structural and magnetic properties of quasi two-dimensional $S=1/2$ quantum magnet Cu[C$_6$H$_2$(COO)$_4$][H$_3$N-(CH$_2$)$_2$-NH$_3$]$\cdot$3H$_2$O. It is found to crystallize in a monoclinic structure with…

Materials Science · Physics 2021-05-26 S. Guchhait , S. Baby , M. Padmanabhan , A. Medhi , R. Nath

Geometric frustration of magnetic ions can lead to a quantum spin liquid ground state where long range magnetic order is avoided despite strong exchange interactions. The physical realization of quantum spin liquids comprises a major…

Strongly Correlated Electrons · Physics 2023-06-07 Alex Hallett , Catalina Avarvarei , John W. Harter

We study the 3D Kitaev and Kitaev-Heisenberg models respectively on the hyperhoneycomb and hyperoctagon lattices, both at zero and finite-temperature, in the thermodynamic limit. Our analysis relies on advanced tensor network (TN)…

Strongly Correlated Electrons · Physics 2021-09-08 Saeed S. Jahromi , Hadi Yarloo , Roman Orus

Quantum spin liquid (QSL) is an exotic quantum phase of matter whose ground state is quantum-mechanically entangled without any magnetic ordering. A central issue concerns emergent excitations that characterize QSLs, which are…

Strongly Correlated Electrons · Physics 2018-05-08 Y. Tokiwa , T. Yamashita , D. Terazawa , K. Kimura , Y. Kasahara , T. Onishi , Y. Kato , M. Halim , P. Gegenwart , T. Shibauchi , S. Nakatsuji , E. -G. Moon , Y. Matsuda

We explore the potential experimental realization of the mixed-spin Kitaev model in materials such as Zr$_{0.5}$Ru$_{0.5}$Cl$_3$, where spin-1/2 and spin-3/2 ions occupy distinct sublattices of a honeycomb lattice. By developing a…

Strongly Correlated Electrons · Physics 2025-05-09 Willian Natori , Yang Yang , Hui-Ke Jin , Johannes Knolle , Natalia B. Perkins

The Kitaev model predicts that quantum spin liquids (QSLs) will form at low temperatures under certain special conditions, and materials hosting the QSL state are frequently sought. The layered honeycomb lattice material {\alpha}-RuCl3 has…

Materials Science · Physics 2022-01-24 Danrui Ni , Xin Gui , Kelly M. Powderly , R. J. Cava

We discuss the finite-temperature phase diagram of the Heisenberg-Kitaev model on the hexagonal lattice, which has been suggested to describe the spin-orbital exchange of the effective spin-1/2 momenta in the Mott insulating Iridate…

Strongly Correlated Electrons · Physics 2011-09-26 Johannes Reuther , Ronny Thomale , Simon Trebst

Spin-liquid behavior was recently suggested experimentally in the moderately one-dimensional organic compound $\kappa$-H$_3$(Cat-EDT-TTF)$_2$. This compound can be modeled by the one-band Hubbard model on the anisotropic triangular lattice…

Strongly Correlated Electrons · Physics 2016-12-28 S. Acheche , A. Reymbaut , M. Charlebois , D. Sénéchal , A. -M. S. Tremblay

The insulating honeycomb magnet $\alpha$-RuCl$_{3}$ exhibits fractionalized excitiations that signal its proximity to a Kitaev quantum spin liquid (QSL) state, however, at $T=0$, fragile long-range magnetic order arises from non-Kitaev…

Strongly Correlated Electrons · Physics 2017-12-12 P. Lampen-Kelley , A. Banerjee , A. A. Aczel , H. B. Cao , M. B. Stone , C. A. Bridges , J. -Q. Yan , S. E. Nagler , D. Mandrus

The three-dimensional frustrated spin lattice in MgCrGaO4, where Cr3+ ions occupy a pyrochlore-like network, exemplifies a quantum magnet with competing interactions, macroscopic degeneracy, and exotic low-energy excitations. Using…

Strongly Correlated Electrons · Physics 2026-03-17 U. Jena , S. Kundu , Suheon Lee , Q. Faure , F. Damay , S. Rols , Adam Berlie , S. Petit , Kwang-Yong Choi , P. Khuntia

Quantum spin liquids can arise from Kitaev magnetic interactions, and exhibit fractionalized excitations with the potential for a topological form of quantum computation. This review surveys recent experimental and theoretical progress on…

A quantum spin liquid (QSL) would be an exotic stage for superconductivity. A promising candidate for a doped QSL is the organic triangular-lattice system, kappa-(BEDT-TTF)4Hg2:89Br8, which hosts a non-Fermi liquid and magnetism of a QSL…

Superconductivity · Physics 2022-06-16 K. Wakamatsu , Y. Ueno , K. Miyagawa , H. Taniguchi , K. Kanoda