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Motivated by recent experiments on $\alpha$-RuCl$_3$, we investigate a possible quantum spin liquid ground state of the honeycomb-lattice spin model with bond-dependent interactions. We consider the $K-\Gamma$ model, where $K$ and $\Gamma$…

Strongly Correlated Electrons · Physics 2018-02-15 Matthias Gohlke , Gideon Wachtel , Youhei Yamaji , Frank Pollmann , Yong Baek Kim

Continuous spin excitations are widely recognized as one of the hallmarks of novel spin states in quantum magnets, such as quantum spin liquids (QSLs). Here, we report the observation of such kind of excitations in K2Ni2(SO4)3, which…

The exploration of quantum spin liquids (QSLs) has been guided by different approaches including the resonating valence bond (RVB) picture, deconfined lattice gauge theories and the Kitaev model. More recently, a spin liquid ground state…

Strongly Correlated Electrons · Physics 2022-12-19 Ruben Verresen , Ashvin Vishwanath

Experimental quest for the hypothetical "quantum spin liquid" state has recently met a few promising candidate materials including organic salts \kappa-(ET)2Cu2(CN)3 and EtMe3Sb[Pd(dmit)2]2, S=1/2 triangular-lattice Heisenberg…

Strongly Correlated Electrons · Physics 2015-06-17 Ken Watanabe , Hikaru Kawamura , Hiroki Nakano , Toru Sakai

We combine ultra-high-resolution inelastic neutron scattering and quantum Monte Carlo simulations to study thermodynamics and spin excitations in the spin-supersolid phase of the triangular lattice XXZ antiferromagnet K$_2$Co(SeO$_3$)$_2$…

A quantum spin liquid (QSL) is an exotic quantum state of matter characterized by fluctuating spins which may exhibit long-range entanglement. Among the possible host candidates for a QSL ground state, the $S$=1/2 kagome lattice…

The two-dimensional Hubbard model on the anisotropic triangular lattice, with two different hopping amplitudes $t$ and $t^\prime$, is relevant to describe the low-energy physics of $\kappa$-(ET)$_2$X, a family of organic salts. The…

Strongly Correlated Electrons · Physics 2015-05-13 Luca F. Tocchio , Alberto Parola , Claudius Gros , Federico Becca

In frustrated Ising magnets, classical spin liquids (CSLs) with macroscopic ground-state degeneracy can survive against conventional magnetic order, as exemplified by systems on triangular, kagome and pyrochlore lattices at zero field. Here…

We report the thermodynamic and muon spin relaxation ($\mu$SR) evidences for a possible gapless spin liquid in Tm$_{3}$Sb$_{3}$Zn$_{2}$O$_{14}$, with the rare-earth ions Tm$^{3+}$ forming a two-dimensional kagom\'{e} lattice. We extract the…

Strongly Correlated Electrons · Physics 2018-11-09 Zhaofeng Ding , Yanxing Yang , Jian Zhang , Cheng Tan , Zihao Zhu , Gang Chen , Lei Shu

We present a theory of spin and orbital states in Mott insulator $LaTiO_3$. The spin-orbital superexchange interaction between $d^1(t_{2g})$ ions in cubic crystal suffers from a pathological degeneracy of orbital states at classical level.…

Strongly Correlated Electrons · Physics 2009-10-31 G. Khaliullin , S. Maekawa

Quantum spin liquids (QSLs) are an exotic state of matter that is subject to extensive research. However, the relationship between the ubiquitous disorder and the QSL behaviors is still unclear. Here, by performing comparative experimental…

We report the magnetic, magnetodielectric, and electric polarization properties of single crystals of the Co-based Kitaev Spin Liquid (KSL) candidate Na$_2$Co$_2$TeO$_6$ (NCTO). The sample shows magnetic transitions at 26 K, 16 K, and 5 K,…

Recently, the bi-layer Kagome lattice material Ca$_{10}$Cr$_7$O$_{28}$ has been shown to be a quasi-two-dimensional quantum spin liquid (QSL) where the frustration arises from a balance between competing ferromagnetic and antiferromagnetic…

Strongly Correlated Electrons · Physics 2020-05-27 A. Balodhi , A. Ali , Yogesh Singh

We have performed thermodynamic and neutron scattering measurements on the S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is observed…

Strongly Correlated Electrons · Physics 2007-05-23 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Yoshida , Y. Takano , A. Suslov , Y. Qiu , J. -H. Chung , D. G. Nocera , Y. S. Lee

We present a thorough experimental study of the three-dimensional hyperhoneycomb Kitaev magnet $\beta$-Li$_2$IrO$_3$, using a combination of inelastic neutron scattering (INS), time-domain THz spectroscopy, and heat capacity measurements.…

Materials that realize Kitaev spin models with bond-dependent anisotropic interactions have long been searched for, as the resulting frustration effects are predicted to stabilize novel forms of magnetic order or quantum spin liquids. Here…

Strongly Correlated Electrons · Physics 2014-11-11 A. Biffin , R. D. Johnson , I. Kimchi , R. Morris , A. Bombardi , J. G. Analytis , A. Vishwanath , R. Coldea

Quantum fluctuations originating phase competition or geometrical frustration of spins lead to novel states such as a quantum critical point and a quantum spin liquid where the strong quantum fluctuations suppress any ordered states even at…

Strongly Correlated Electrons · Physics 2019-11-28 Y. Saito , H. Nakamura , M. Sawada , T. Yamazaki , S. Fukuoka , N. Matsunaga , K. Nomura , M. Dressel , A. Kawamoto

A quantum spin liquid (QSL) is a state of matter where unpaired electrons' spins in a solid are quantum entangled, but do not show magnetic order in the zero-temperature limit. Because such a state may be important to the microscopic origin…

Motivated by recent experiments on the quantum-spin-liquid candidate material LiZn2Mo3O8, we study a single-band extended Hubbard model on an anisotropic Kagome lattice with the 1/6 electron filling. Due to the partial filling of the…

Strongly Correlated Electrons · Physics 2016-06-16 Gang Chen , Hae-Young Kee , Yong Baek Kim

The honeycomb magnet $\alpha-$RuCl$_3$ is a prime candidate material for realizing the Kitaev quantum spin liquid (QSL), but it shows long-range magnetic order at low temperature. Nevertheless, its broad inelastic neutron scattering (INS)…

Strongly Correlated Electrons · Physics 2022-11-23 Oliver Franke , Dumitru Călugăru , Andreas Nunnenkamp , Johannes Knolle