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We develop a formalism to study the Resonant Inelastic X-ray Scattering (RIXS) response in metals based on the diagrammatic expansion for its cross section. The standard approach to the solution of the RIXS problem relies on two key…

Strongly Correlated Electrons · Physics 2019-11-20 A. M. Tsvelik , R. M. Konik , N. V. Prokof'ev , I. S. Tupitsyn

Resonant inelastic X-ray scattering (RIXS) has become an important scientific tool. Nonetheless, conventional high-resolution RIXS measurements (<100 meV), especially in the soft x-ray range, require large and low-throughput grating…

Materials Science · Physics 2020-06-22 Daniel J. Higley , Hirohito Ogasawara , Sioan Zohar , Georgi L. Dakovski

We develop a formalism to calculate the L-edge resonant x-ray scattering (RIXS) spectra from transition-metal compounds. Using a multi-orbital tight-binding model, we derive useful formulas to calculate the spectra by collecting up the…

Strongly Correlated Electrons · Physics 2015-06-16 Jun-ichi Igarashi , Tatsuya Nagao

A new method is presented for describing vibrational effects in x-ray absorption spectroscopy (XAS) and resonant inelastic x-ray scattering (RIXS) using a combination of the classical Franck-Condon (FC) approximation and classical…

Materials Science · Physics 2017-12-20 Mathias P. Ljungberg

Resonant inelastic x-ray scattering (RIXS) is a spectroscopic technique which has been widely used to study various elementary excitations in correlated and other condensed matter systems. For strongly correlated materials, besides boosting…

Strongly Correlated Electrons · Physics 2012-12-27 C. J. Jia , C. -C. Chen , A. P. Sorini , B. Moritz , T. P. Devereaux

An easily accessible method is presented that permits to calculate spectra involving atomic multiplets relevant to X-ray Absorption Spectroscopy (XAS) and Resonant Inelastic X-ray Scattering (RIXS) experiments. We present specific examples…

Strongly Correlated Electrons · Physics 2009-03-16 F. Vernay , B. Delley

Resonant inelastic x-ray scattering (RIXS) is an extremely valuable tool for the study of elementary, including magnetic, excitations in matter. Latest developments of this technique mostly aimed at improving the energy resolution and…

The study of elementary bosonic excitations is essential toward a complete description of quantum electronic solids. In this context, resonant inelastic X-ray scattering (RIXS) has recently risen to becoming a versatile probe of electronic…

Strongly Correlated Electrons · Physics 2019-01-23 M. Kang , J. Pelliciari , Y. Krockenberger , J. Li , D. E. McNally , E. Paris , R. Liang , W. N. Hardy , D. A. Bonn , H. Yamamoto , T. Schmitt , R. Comin

Resonant inelastic X-ray scattering (RIXS) is a powerful photon-in, photon-out spectroscopy technique for probing electronic, magnetic, and lattice excitations in matter. Time-resolved RIXS extends this capability through a stroboscopic…

We propose a general scheme for the derivation of the signals resonant inelastic (and elastic) x-ray scattering (RIXS) gives access to. In particular, we find that RIXS should allow to directly detect many hidden orders, such as spin…

Strongly Correlated Electrons · Physics 2015-06-17 Lucile Savary , T. Senthil

The resonant inelastic x-ray scattering (RIXS) was measured in an insulating SrCuO$_{2}$ with changing the incident photon energy ($h\nu$) near the Cu $1s$ absorption edge (K-edge). Complex structures and their dependences on the momentum…

We present calculations for resonant inelastic x-ray scattering (RIXS) in edge-shared copper oxide systems, such as CuGeO$_{3}$ and Li$_{2}$CuO$_{2}$, appropriate for hard x-ray scattering where the photoexcited electron lies above oxygen…

Strongly Correlated Electrons · Physics 2009-11-13 F. Vernay , B. Moritz , I. Elfimov , J. Geck , D. Hawthorn , T. P. Devereaux , G. A. Sawatzky

Resonant inelastic x-ray scattering (RIXS) tuned for the Cu L edge is a possible tool to detect charge excitations in cuprate superconductors. We theoretically investigate the possibility for observing a collective charge excitation by the…

Strongly Correlated Electrons · Physics 2015-08-03 Takami Tohyama , Kenji Tsutsui , Michiyasu Mori , Shigetoshi Sota , Seiji Yunoki

Resonant inelastic X-ray scattering (RIXS) spectra of model copper- and nickel-based transition metal oxides are measured over a wide range of energies near the M-edge (h$\nu$=60-80eV) to better understand the properties of resonant…

Strongly Correlated Electrons · Physics 2012-11-20 L. Andrew Wray , Wanli Yang , Hiroshi Eisaki , Zahid Hussain , Yi-De Chuang

We investigate theoretically the resonant inelastic x-ray scattering (RIXS) at the $K$ edge of Si on the basis of an ab initio calculation. We calculate the RIXS spectra with systematically varying transfered-momenta, incident-photon energy…

Materials Science · Physics 2007-05-23 Yunori Nisikawa , Manabu Usuda , Jun-ichi Igarashi

We examine the momentum-dependent excitation spectra of indirect as well as direct resonant inelastic x-ray scattering (RIXS) processes in half-filled (extended) Hubbard rings. We determine the fundamental features of the groundstate RIXS…

Strongly Correlated Electrons · Physics 2012-03-02 Stefanos Kourtis , Jeroen van den Brink , Maria Daghofer

We theoretically examine the momentum dependence of resonant inelastic x-ray scattering (RIXS) spectrum for one-dimensional and two-dimensional cuprates based on the single-band Hubbard model with realistic parameter values. The spectrum is…

Strongly Correlated Electrons · Physics 2007-05-23 T. Tohyama , K. Tsutsui , S. Maekawa

In indirect resonant inelastic X-ray scattering (RIXS) an intermediate state is created with a core-hole that has a ultrashort lifetime. The core-hole potential therefore acts as a femtosecond pulse on the valence electrons. We show that…

Strongly Correlated Electrons · Physics 2009-11-11 Luuk J. P. Ament , Filomena Forte , Jeroen van den Brink

X-ray cavity quantum optics with inner-shell transitions has been hindered by the overlap between resonant and continuum states. Here, we report the first experimental demonstration of cavity-controlled co-to-core resonant inelastic x-ray…