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Related papers: RIXS and excited states calculation with the Xclai…

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We develop a framework to evaluate the time-dependent resonant inelastic X-ray scattering (RIXS) signal with the use of non-equilibrium dynamical mean field theory simulations. The approach is based on the solution of a time-dependent…

Strongly Correlated Electrons · Physics 2021-03-24 Martin Eckstein , Philipp Werner

We analyze theoretically the resonant inelastic x-ray scattering (RIXS) at the Ni K edge in the stripe-ordered state of La_{2-x}Sr_xNiO_4 at x=1/3. In the calculation of RIXS spectra, the stripe-ordered ground state is described within the…

Strongly Correlated Electrons · Physics 2012-01-18 Takuji Nomura , Eiji Kaneshita

We present a theoretical investigation of the origin of Raman-like and fluorescencelike (FL) features of resonant inelastic x-ray scattering (RIXS) spectra. Using a combination of local-density approximation + dynamical mean-field theory…

Strongly Correlated Electrons · Physics 2018-09-26 Atsushi Hariki , Mathias Winder , Jan Kuneš

Recent improvements in instrumentation have established resonant inelastic x-ray scattering (RIXS) as a valuable new probe of the magnetic excitations in the cuprates. This article introduces RIXS, focusing on the Cu $L_3$ resonance, and…

Superconductivity · Physics 2015-02-17 M. P. M. Dean

Ru M$_3$-edge resonant inelastic x-ray scattering (RIXS) measurements of RuCl$_3$ with 27 meV resolution reveals a spin-orbit exciton without noticeable splitting. We extract values for the spin-orbit coupling constant ($\lambda=154\pm2$…

Strongly Correlated Electrons · Physics 2020-01-29 Blair W Lebert , Subin Kim , Valentina Bisogni , Ignace Jarrige , Andi M Barbour , Young-June Kim

We theoretically analyze the intensity of the resonant inelastic X-ray scattering (RIXS) based on Ansatz that the electron is fractionalized into two components. By fitting the angle resolved photoemission spectroscopy (ARPES) data of a…

Strongly Correlated Electrons · Physics 2021-07-26 Masatoshi Imada

Results of model calculations using exact diagonalization reveal the orbital character of states associated with different Raman loss peaks in Cu $K$-edge resonant inelastic X-ray scattering (RIXS) from La$_{2}$CuO$_{4}$. The model includes…

We present a formalism for the resonant inelastic x-ray scattering (RIXS) cross section. The resulting compact expression in terms of polarizability matrix elements, particularly lends itself to the implementation in an all-electron…

Materials Science · Physics 2022-08-17 Christian Vorwerk , Francesco Sottile , Claudia Draxl

We present an ab initio study of neutral core and valence electronic excitations in {\alpha}-Al2O3 by solving the Bethe-Salpeter equation (BSE) of many-body perturbation theory within an all-electron framework. Calculated spectra at the Al…

Materials Science · Physics 2024-01-26 M. Laura Urquiza , Matteo Gatti , Francesco Sottile

We analyze resonant inelastic x-ray scattering (RIXS) at the Cu K edge in a typical orbital-ordered compound KCuF3 on the basis of a microscopic theory. Spectral shape and its dependence on polarization direction and momentum transfer of…

Strongly Correlated Electrons · Physics 2014-06-20 Takuji Nomura

Young's archetypal double-slit experiment forms the basis for modern diffraction techniques: the elastic scattering of waves yields an interference pattern that captures the real-space structure. Here, we report on an inelastic incarnation…

We show that high resolution Resonant Inelastic X-ray Scattering (RIXS) provides direct, element-specific and momentum-resolved information on the electron-phonon (e-p) coupling strength. Our theoretical analysis demonstrates that the e-p…

Strongly Correlated Electrons · Physics 2012-12-03 Luuk J. P. Ament , Michel van Veenendaal , Jeroen van den Brink

We report a comprehensive resonant inelastic x-ray scattering (RIXS) study of various iridate materials focusing on core-level excitations and transitions between crystal-field split d-levels. The 2p core hole created at the Ir $L_3$…

Strongly Correlated Electrons · Physics 2018-05-10 Young-June Kim , J. P. Clancy , H. Gretarsson , G. Cao , Yogesh Singh , Jungho Kim , M. H. Upton , D. Casa , T. Gog

Resonant Inelastic X-ray scattering (RIXS) is a synchrotron-based spectroscopy that has seen growing interest across a range of scientific disciplines beyond fundamental physics. The interpretation of experimental RIXS data requires…

This paper provides a brief overview of applications of advanced X-ray spectroscopic techniques that take advantage of the resonant inelastic X-ray scattering (RIXS) in the hard and tender x-ray range and have recently become available for…

Materials Science · Physics 2014-01-08 K. O. Kvashnina , S. M. Butorin

We present an ab initio theory of core- and valence resonant inelastic x-ray scattering (RIXS) based on a real-space multiple scattering Green's function formalism and a quasi-boson model Hamiltonian. Simplifying assumptions are made which…

Materials Science · Physics 2011-01-25 J. J. Kas , J. J. Rehr , J. A. Soininen , P. Glatzel

Herein we show that non-resonant inelastic x-ray scattering involving an $s$ core level is a powerful spectroscopic method to characterize the excited states of transition metal compounds. The spherical charge distribution of the $s$ core…

We study two-magnon excitations in resonant inelastic x-ray scattering (RIXS) at the transition-metal $K$-edge. Instead of working with effective Heisenberg spin models, we work with a Hubbard-type model ($d$-$p$ model) for a typical…

Strongly Correlated Electrons · Physics 2017-10-18 Takuji Nomura

We have performed resonant inelastic x-ray scattering (RIXS) near the Cu-K edge on cuprate superconductors La(2-x)Sr(x)CuO(4), La(2-x)Ba(x)CuO(4), La(2-x)Sr(x)Cu(1-y)Fe(y)O(4) and Bi(1.76)Pb(0.35)Sr(1.89)CuO(6+d), covering underdoped to…

Superconductivity · Physics 2015-06-15 S. Wakimoto , K. Ishii , H. Kimura , K. Ikeuchi , M. Yoshida , T. Adachi , D. Casa , M. Fujita , Y. Fukunaga , T. Gog , Y. Koike , J. Mizuki , K. Yamada

We analyze the resonant inelastic x-ray scattering (RIXS) spectra at the Cu and Ni K edges in La2CuO4 and La2NiO4, respectively. We make use of the Keldysh-Green-function formalism, in which the RIXS intensity is described by a product of…

Strongly Correlated Electrons · Physics 2009-11-13 Manabu Takahashi , Junichi Igarashi , Taeko Semba