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Resonant inelastic x-ray scattering (RIXS) is an evolving tool for investigating spin dynamics of strongly correlated materials, which complements inelastic neutron scattering. Both techniques have found that non-spin-conserving (NSC)…

We present a microscopic theory of resonant soft x-ray scattering (RSXS) that accounts for the delocalized character of valence electrons. Unlike past approaches defined in terms of form factors for atoms or clusters, we develop a…

Strongly Correlated Electrons · Physics 2013-04-08 David Benjamin , Dmitry Abanin , Peter Abbamonte , Eugene Demler

We report resonant inelastic x-ray measurements of insulating La$_2$CuO$_4$ and Sr$_2$CuO$_2$Cl$_2$ taken with the incident energy tuned near the Cu K absorption edge. We show that the spectra are well described in a shakeup picture in 3rd…

Strongly Correlated Electrons · Physics 2009-10-31 P. Abbamonte , C. A. Burns , E. D. Isaacs , P. M. Platzman , L. L. Miller , S. W. Cheong , M. V. Klein

X-ray absorption spectroscopy (XAS) is an explicit probe of the unoccupied electronic structure of materials and an invaluable tool for fingerprinting various electronic properties and phenomena. Computational methods capable of simulating…

Materials Science · Physics 2023-02-07 Subhayan Roychoudhury , David Prendergast

The electronic structure of CuIr$_2$S$_4$ has been investigated using various bulk-sensitive x-ray spectroscopic methods near the Ir $L_3$-edge: resonant inelastic x-ray scattering (RIXS), x-ray absorption spectroscopy in the partial…

Strongly Correlated Electrons · Physics 2012-06-18 H. Gretarsson , Jungho Kim , D. Casa , T. Gog , K. R. Choi , S. W. Cheong , Young-June Kim

We report a Cu $K$-edge resonant inelastic x-ray scattering (RIXS) study of charge-transfer excitations in the 2-8 eV range in the structurally simple compound HgBa$_2$CuO$_{4+\delta}$ at optimal doping ($T_{\rm c} = 96.5 $ K). The spectra…

Strongly Correlated Electrons · Physics 2009-11-11 L. Lu , X. Zhao , G. Chabot-Couture , J. N. Hancock , N. Kaneko , O. P. Vajk , G. Yu , S. Grenier , Y. J. Kim , D. Casa , T. Gog , M. Greven

We examine the effect of core-hole lifetime on the spectral weight of resonant inelastic x-ray scattering (RIXS) in hole-doped cuprates. We calculate the spectral weight by using exact diagonalization technique for a 4x4 doped Hubbard…

Strongly Correlated Electrons · Physics 2018-08-01 Takami Tohyama , Kenji Tsutsui

Resonant inelastic x-ray scattering (RIXS) has become a prominent technique to study quasiparticle excitations. With advances in polarization analysis capabilities at different facilities, RIXS offers exceptional potential for investigating…

Taking spinon excitations in the quantum antiferromagnet CaCu2O3 as an example, we demonstrate that femtosecond dynamics of magnetic excitations can be probed by direct resonant inelastic x-ray scattering (RIXS). To this end, we isolate the…

Recent improvements in the energy resolution of resonant inelastic x-ray scattering experiments (RIXS) at the Cu-L$_3$ edge have enabled the study of lattice, spin, and charge excitations. Here, we report on the detection of a low intensity…

We used resonant inelastic x-ray scattering (RIXS) with and without analysis of the scattered photon polarization, to study dispersive spin excitations in the high temperature superconductor YBa2Cu3O6+x over a wide range of doping levels…

In strongly correlated systems the complete determination of the dynamical susceptibility $\chi(\textbf{q}, \omega)$ is of special relevance because of the entwinement of the spin and charge components. Although Resonant Inelastic X-Ray…

Identifying model Hamiltonians is a vital step toward creating predictive models of materials. Here, we combine Bayesian optimization with the EDRIXS numerical package to infer Hamiltonian parameters from resonant inelastic X-ray scattering…

Strongly Correlated Electrons · Physics 2025-10-30 Marton K. Lajer , Xin Dai , Kipton Barros , Matthew R. Carbone , S. Johnston , M. P. M. Dean

We present a new approach to computing multiplets for core spectroscopies, whereby the crystal field is constructed explicitly from the positions and charges of surrounding atoms. The simplicity of the input allows the consideration of…

Other Condensed Matter · Physics 2012-03-30 A. Uldry , F. Vernay , B. Delley

A resonant inelastic x-ray scattering study of the electronic structure of the semiconductor cuprous oxide, $\rm Cu_2O$, is reported. When the incident x-ray energy is tuned to the Cu K-absorption edge, large enhancements of the spectral…

Materials Science · Physics 2012-06-18 Young-June Kim , J. P. Hill , H. Yamaguchi , T. Gog , D. Casa

High-resolution resonant inelastic X-ray scattering (RIXS) at the oxygen K-edge has been used to study the orbital excitations of Ca2RuO4 and Sr2RuO4. In combination with linear dichroism X-ray absorption spectroscopy, the ruthenium…

Resonance anomalous surface x-ray scattering (RASXS) technique was applied to electrochemical interface studies. It was used to determine the chemical states of electrochemically formed anodic oxide monolayers on platinum surface. It is…

We study the magnetic resonant x-ray scattering (RXS) spectra around the $K$ edge of Cu in KCuF$_3$ on the basis of an {\em ab initio} calculation. We use the full-potential linearlized augmented plane wave method in the LDA$+U$ scheme, and…

Strongly Correlated Electrons · Physics 2009-11-07 M. Takahashi , M. Usuda , J. Igarashi

Understanding the electronic structure of actinide materials is crucial for both fundamental research and nuclear applications. The partially filled 5f shells exhibit complex behavior due to strong correlations and ligand hybridization,…

We have developed a scattering-matrix approach for numerical calculation of resonant states and Q-values of a nonideal optical disk cavity of an arbitrary shape and of an arbitrary varying refraction index. The developed method has been…

Optics · Physics 2009-11-10 A. I. Rahachou , I. V. Zozoulenko
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