English

High frame rate RIXS spectroscopy using a JUNGFRAU detector with an iLGAD sensor

Instrumentation and Detectors 2025-11-18 v1

Abstract

Resonant inelastic X-ray scattering (RIXS) is a powerful photon-in, photon-out spectroscopy technique for probing electronic, magnetic, and lattice excitations in matter. Time-resolved RIXS extends this capability through a stroboscopic optical pump-probe scheme to characterize the time evolution of the photoexcitation and subsequent relaxation dynamics of a sample. This technique is, however, extremely photon-hungry, requiring high-repetition-rate and intense X-ray facilities. The Heisenberg RIXS (hRIXS) spectrometer at the Spectroscopy and Coherent Scattering (SCS) instrument of the European X-ray Free-Electron Laser (EuXFEL) is designed to exploit high-repetition-rates, while maintaining optimal time and energy resolution. In this work, we demonstrate the successful deployment of a JUNGFRAU detector equipped with an inverse Low Gain Avalanche Diode (iLGAD) sensor for time-resolved RIXS studies in the soft X-ray range, using the hRIXS spectrometer. A spatial resolution of 19.71±0.7 μm19.71 \pm 0.7~\mu\mathrm{m} and a resolving power exceeding 10,000 were achieved at an unprecedented frame rate of 47 kHz. Intra-train resolved data measured with a high FEL peak fluence of 1.8 mJ/cm21.8~\mathrm{mJ/cm^{2}} for a 928.5 eV ph photon energy and 1.1 MHz repetition rate from cupric oxide (CuO) revealed a decrease in the emitted signal by ~10% over a time interval of 340 μs340~\mu\mathrm{s}, indicating FEL-induced effects that require monitoring when conducting high-repetition-rate experiments. These results establish the JUNGFRAU-iLGAD as a promising detector to harvest the full potential of the hRIXS spectrometer, and validate its suitability for soft X-ray applications.

Keywords

Cite

@article{arxiv.2511.12314,
  title  = {High frame rate RIXS spectroscopy using a JUNGFRAU detector with an iLGAD sensor},
  author = {Nuno Duarte and Loïc Le Guyader and Viktoria Hinger and Marco Ramilli and Justine Schlappa and Robert Carley and Maria Carulla and Yi-Ping Chang and Devesh Chopra and Natalia Gerasimova and Michael Grimes and Aldo Mozzanica and Sergii Parchenko and Le Phuong Hoang and Urs Staub and Jiaguo Zhang and Anna Bergamaschi and Andreas Scherz and Bernd Schmitt and Monica Turcato},
  journal= {arXiv preprint arXiv:2511.12314},
  year   = {2025}
}

Comments

30 pages, 13 figures

R2 v1 2026-07-01T07:39:15.486Z