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We numerically analyze the use of intense entangled twin beams for ultra-sensitive spectroscopic measurements in chemical and biological systems. The examined scheme makes use of intense frequency-modulated (chirped) entangled beams to…

Quantum Physics · Physics 2018-05-16 Jiří Svozilík , Jan Peřina , Roberto de J. León-Montiel

Time-resolved spontaneous Raman spectroscopy serves as a probe for incoherent quasiparticle and collective excitation dynamics, and allows to distinguish symmetry changes across a photoinduced phase transition through the inelastic light…

Materials Science · Physics 2019-03-27 J. Zhu , R. B. Versteeg , P. Padmanabhan , P. H. M. van Loosdrecht

Broadband energy-time entanglement can be used to enhance the rate of two-photon absorption (TPA) by combining a precise two-photon resonance with a very short coincidence time. Because of this short coincidence time, broadband TPA is not…

Quantum Physics · Physics 2023-12-04 Baihong Li , Holger F. Hofmann

Super-resolution fluorescence microscopy is of great interest in life science studies for visualizing subcellular structures at the nanometer scale. Among various kinds of super-resolution approaches, image scanning microscopy (ISM) offers…

Infrared (IR) spectroscopy is an indispensable tool for many practical applications including material analysis and sensing. Existing IR spectroscopy techniques face challenges related to the inferior performance and the high cost of…

Optics · Physics 2017-03-13 Anna Paterova , Shaun Lung , Dmitry Kalashnikov , Leonid Krivitsky

We theoretically propose a method to enhance Raman scattering by injecting a seeded light field which is correlated with the initially prepared atomic spin wave. Such a light-atom correlation leads to an interference in the Raman…

Quantum Physics · Physics 2013-05-29 Chun-Hua Yuan , L. Q. Chen , Z. Y. Ou , Weiping Zhang

Particle entanglement is a fundamental resource upon which are based many quantum technologies. However, the up-to-now best sources of entangled photons rely on parametric down-conversion processes, which are optimal only at certain…

We present a novel approach to transient Raman spectroscopy, which combines stochastic probe pulses and a covariance-based detection to measure stimulated Raman signals in alpha-quartz. A coherent broadband pump is used to simultaneously…

Raman scattering signal can be enhanced through localization of incident field into sub-wavelength hot-spots through plasmonic nano-structures (Surface-enhanced Raman scattering-SERS). Recently, further enhancement of SERS signal via…

Path-entangled multi-photon states allow optical phase-sensing beyond the shot-noise limit, provided that an efficient parity measurement can be implemented. Realising this experimentally is technologically demanding, as it requires…

We demonstrate a novel technique of coherent Raman spectroscopy with a femtosecond laser. We apply to a molecular sample a sequence of pairs of ultrashort excitation and probe pulses, with a linearly increasing time delay between the two…

Spectroscopic stimulated Raman scattering (SRS) imaging has become a useful tool finding a broad range of applications. Yet, wider adoption is hindered by the bulky and environmentally-sensitive solid-state optical parametric oscillator…

Optics · Physics 2021-08-20 Hongli Ni , Peng Lin , Yifan Zhu , Meng Zhang , Yuying Tan , Yuewei Zhan , Ji-Xin Cheng

Angle-resolved Raman spectroscopy (ARRS) is an effective method to analyze the symmetry of phonons and other excitations in molecules and solid-state crystals. While there are several configurations of ARRS instruments, the measurement…

Complex 3D integration of photonic and electronic integrated circuits is of particular interest to carry the photonics roadmap and to address challenges but involves mechanical stress, often detrimental for the behavior of optical…

Entangling independent photons is not only of fundamental interest but also of crucial importance for quantum information science. Two-photon interference is a major method to entangle independent identical photons. If two photons are…

Quantum Physics · Physics 2015-01-27 Tian-Ming Zhao , Han Zhang , Jian Yang , Zi-Ru Sang , Xiao Jiang , Xiao-Hui Bao , Jian-Wei Pan

We demonstrate a compact and versatile laser system for stimulated Raman spectroscopy (SRS). The system is based on a tunable continuous wave (CW) probe laser combined with a home-built semi-monolithic nanosecond pulsed pump Nd:YVO4 laser…

Chemical Physics · Physics 2017-03-03 Hugo Kerdoncuff , Mark R. Pollard , Philip G. Westergaard , Jan C. Petersen , Mikael Lassen

Electron and vibrational dynamics of molecules are commonly studied by subjecting them to two interactions with a fast actinic pulse that prepares them in a nonstationary state and after a variable delay period $T$, probing them with a…

Quantum Physics · Physics 2015-03-31 Bijay Kumar Agarwalla , Hideo Ando , Konstantin E. Dorfman , Shaul Mukamel

We demonstrate coincidence measurements of spatially entangled photons by means of a novel type of multi-pixel based detection array. The adopted sensor is a fully digital 8$\times$16 silicon photomultiplier array allowing not only photon…

Instrumentation and Detectors · Physics 2016-12-19 Manuel Unternährer , Bänz Bessire , Leonardo Gasparini , David Stoppa , André Stefanov

The authors demonstrate a form of two-photon-counting interferometry by measuring the coincidence counts between single-photon-counting detectors at an output port of a Mach-Zehnder Interferometer (MZI) following injection of broad-band…

Entangled-photon coincidence imaging is a method to nonlocally image an object by transmitting a pair of entangled photons through the object and a reference optical system, respectively. The image of the object can be extracted from the…

Quantum Physics · Physics 2016-09-08 Jing Cheng , Shensheng Han
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