Related papers: Stimulated Raman Spectroscopy with Entangled Light…
In this contribution we analyze virtual-state spectroscopy --- a unique tool for extracting information about the virtual states that contribute to the two-photon excitation of an absorbing medium --- as implemented by means of intense…
Imaging Raman spectroscopy can be used to identify cancerous tissue. Traditionally, a step-by-step scanning of the sample is applied to generate a Raman image, which, however, is too slow for routine examination of patients. By transferring…
We extend the Purcell's original idea [Phys. Rev. \textbf{69}, 682 (1946)] on modification of photon spontaneous \textit{emission} rate to modification of photon spontaneous \textit{scattering} rate. We find the interplay of local incident…
In the quantum process of stimulated Raman scattering (SRS), a laser photon propagating in a resonance medium undergoes multifold conversions into a Stokes photon and back. The nontrivial ``cooperative'' behavior of the Stokes component of…
Fluorescence imaging is an essential diagnostic tool in many fields, but diffraction-limited optical imaging at depth is limited by scattering. Here, we present a method based on multiple random illuminations, combined with a computational…
We review an on-chip approach for spontaneous Raman spectroscopy and Surface Enhanced Raman Spectroscopy (SERS) based on evanescent excitation of the analyte as well as evanescent collection of the Raman signal using Complementary Metal…
We calculate the rate of two-photon absorption for frequency entangled photons in a tapered optical fiber whose diameter is comparable to the wavelength of the light. The confinement of the electric field in the transverse direction…
By measuring the thermal effects resulting from stimulated Raman excitations, stimulated Raman photothermal (SRP) microscope offers a new access to spatially and temporally resolved Raman signatures across various sample types. Unlike…
We propose a class of path-entangled photon Fock states for robust quantum optical metrology, imaging, and sensing in the presence of loss. We model propagation loss with beam-splitters and derive a reduced density matrix formalism from…
Spectroscopy is an important tool for probing the properties of materials, chemicals and biological samples. We design a practical transmitter-receiver system that exploits entanglement to achieve a provable quantum advantage over all…
A monochromatic laser pumping a parametric down conversion crystal generates frequency entangled photon pairs. We study this experimentally by addressing such frequency entangled photons at telecommunication wavelengths (around 1550 nm)…
Spontaneous Raman spectroscopy (SRS) is a conventional in-situ laser diagnostic method that has been widely used for measurements of temperature and major species. However, SRS in sooting flames suffers from strong interference including…
Stimulated Raman scattering (SRS) in plasma in the degenerate regime is studied theoretically and numerically. Different from normal SRS with the non-degenerate eigen electrostatic mode excited, the degenerate SRS is developed at plasma…
Entangled photons exhibit non-classical light-matter interactions that create new opportunities in materials and molecular science. For example, in entangled two-photon absorption, the intensity-dependence scales linearly as if only one…
Single-shot ultrafast absorbance spectroscopy based on the frequency encoding of the kinetics is analyzed theoretically and implemented experimentally. The kinetics are sampled in the frequency domain using linearly chirped, amplified 33 fs…
Quantum spectroscopy was performed using the frequency-entangled broadband photon pairs generated by spontaneous parametric down-conversion. An absorptive sample was placed in front of the idler photon detector, and the frequency of signal…
Entanglement has been known to boost target detection, despite it being destroyed by lossy-noisy propagation. Recently, [Phys. Rev. Lett. 128, 010501 (2022)] proposed a quantum pulse-compression radar to extend entanglement's benefit to…
Single photon avalanche diode arrays can provide both the spatial and temporal information of each detected photon. We present here the characterization of entangled light with a sensor specifically designed for quantum imaging…
The Fano lineshape arises from the interference of two excitation pathways to reach a continuum. Its generality has resulted in a tremendous success in explaining the lineshapes of many one-dimensional spectroscopies - absorption, emission,…
Step-frequency radar (SFR) is a high resolution radar approach, where multiple pulses are transmitted at different frequencies, covering a wide spectrum. The obtained resolution directly depends on the total bandwidth used, or equivalently,…