Related papers: Stimulated Raman Spectroscopy with Entangled Light…
Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…
We present experimental demonstration of a recently predicted path interference phenomenon [Nanophotonics 7, 1687 (2018)]. A SERS process becomes resonant when both incident and the converted frequencies match with two plasmon resonances --…
Today's cutting-edge optical spectroscopic exploratory tools, such as Raman or infrared spectroscopy, rely on methods of signal enhancement as a route for their development. These methods are indispensable for substance identification and…
Entangled photons, generated by spontaneous parametric down-conversion from a second-order nonlinear crystal, present a rich potential for imaging and image-processing applications. Since this source is an example of a three-wave mixing…
We extend entangled coincidence (ghost) imaging to fluorescent samples. Given the entangled photon correlation, one photon of the pair carries information on where the other photon has been absorbed and has produced fluorescence in a…
Nonlinear optical methods, such as coherent anti-Stokes Raman scattering (CARS) and stimulated Raman scattering (SRS), are able to perform label free imaging, with chemical bonds specificity. Here, we demonstrate that the use of circularly…
We analyze theoretically and experimentally cases of asymmetric detection, stimulation, and loss within a quantum nonlinear interferometer of entangled pairs. We show that the visibility of the SU(1,1) interference directly discerns between…
Raman-based technologies have enabled many ground-breaking scientific discoveries related to surface science, single molecule chemistry and biology. For example, researchers have identified surface bound molecules by their Raman vibrational…
Photo-Induced Enhanced Raman Spectroscopy (PIERS) is a new surface enhanced Raman spectroscopy (SERS) modality with an order-of-magnitude Raman signal enhancement of adsorbed analytes over that of typical SERS substrates. Despite the…
We introduce Biphoton Entanglement Light Spectroscopy (BELS), a quantum spectroscopic technique that employs polarization entangled Bell pairs and two photon interference to probe material properties. In BELS, the measured signal arises not…
Quantum-enhanced sensing promises to improve the performance of sensing tasks using non-classical probes and measurements that require far fewer scene-modulated photons than the best classical schemes, thereby granting…
Nanofibers functionalized by metal nanostructures and particles are exploited as effective flexible substrates for SERS analysis. Their complex three-dimensional structure may provide Raman signals enhanced by orders of magnitude compared…
Infrared optical measurement has a wide range of applications in industry and science, but infrared light detectors suffer from high costs and inferior performance than visible light detectors. Four-wave mixing (FWM) process allows…
Acoustic-Resolution Photoacoustic Microscopy (AR-PAM) is promising for subcutaneous vascular imaging, but its spatial resolution is constrained by the Point Spread Function (PSF). Traditional deconvolution methods like Richardson-Lucy and…
This article reviews the new developments in Tip-enhanced Raman scattering (TERS). The fundamental mechanisms underlying the Raman enhancement are discussed, including the role of the plasmonic character of the metallic tips, the nature of…
Non-line-of-sight (NLOS) optical imaging and sensing of objects imply new capabilities valuable to autonomous technology, machine vision, and other applications. Existing NLOS imaging methods rely heavily on the prowess of computational…
Raman scattering spectroscopy is widely used as an analytical technique in various fields, but its measurement process tends to be slow due to the low scattering cross-section. In the last decade, various broadband coherent Raman scattering…
Photon entanglement is an important state of light that is at the basis of many protocols in photonic quantum technologies, from quantum computing, to simulation and sensing. The capability to generate entangled photons in integrated…
Infrared light scattering methods have been developed and employed to non-invasively monitor human cerebral blood flow (CBF). However, the number of reflected photons that interact with the brain is low when detecting blood flow in deep…
Spectroscopy with entanglement has shown great potential to break limitations of traditional spectroscopic measurements, yet the role of entanglement in spectroscopic multi-parameter joint measurement, particularly in the infrared optical…