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We closely replicated and extended a recent experiment ("Spatial properties of entangled two-photon absorption," Phys. Rev. Lett. 129, 183601, 2022) that reportedly observed enhancement of two-photon absorption rates in molecular samples by…

Quantum Physics · Physics 2024-04-26 Tiemo Landes , Brian J. Smith , Michael G. Raymer

The faithful distribution of entanglement in continuous variable systems is essential to many quantum information protocols. As such, entanglement distillation and enhancement schemes are a cornerstone of many applications. The photon…

Quantum Physics · Physics 2018-06-07 Zacharie M. Leger , Aharon Brodutch , Amr S. Helmy

In this work we extend low frequency impulsive stimulated Raman microspectroscopy to the pre-electronic resonance regime. We use a broadband two color collinear pump probe scheme which can be readily extended to imaging. We discuss the…

Optics · Physics 2020-07-10 Yahel Soffer , Dekel Raanan , Dan Oron

The random lasing (RL) emission of dyed vesicular polymeric films in diffusive regime of light propagation was investigated under helium temperature. It represents itself the coupling effect of stimulated emission and stimulated Raman…

Optics · Physics 2010-08-27 V. P. Yashchuk , E. A. Tikhonov , O. A. Prygodiuk

Entangled photons can be used to make measurements with an accuracy beyond that possible with classical light. While most implementations of quantum metrology have used states made up of a single colour of photons, we show that entangled…

Traditionally, spectroscopy is performed by examining the position of absorption lines. However, at frequencies near the transition frequency, additional information can be obtained from the phase shift. In this work we consider the…

Quantum Physics · Physics 2016-06-14 Hossein T. Dinani , Manish K. Gupta , Jonathan P. Dowling , Dominic W. Berry

Wide field Raman imaging using the integral field spectroscopy approach was used as a fast, one shot imaging method for the simultaneous collection of all spectra composing a Raman image. For the suppression of autofluorescence and…

Fluorescence lifetime experiments are a standard approach for measuring excited state dynamics and local environment effects. Here, we show that entangled photon pairs produced from a continuous-wave (CW) laser diode can replicate pulsed…

Quantum Physics · Physics 2023-05-15 Nathan Harper , Bryce P. Hickam , Manni He , Scott K. Cushing

Two-photon processes are crucial in applications like microscopy and microfabrication, but their low cross-section requires intense illumination and limits, e.g., the penetration depth in nonlinear microscopy. Entangled states have been…

The coupling evolutions of stimulated Raman scattering (SRS) and Raman rescattering (re-SRS) are studied under the parameter conditions of relevance to the gas-filled hohlraum experiments at the National Ignition Facility by a nonenveloped…

Plasma Physics · Physics 2019-04-26 Liang Hao , Wenyi Huo , Zhanjun Liu , Chunyang Zheng , Chuang Ren

Quantum correlation, such as entanglement and squeezing have shown to improve phase estimation in interferometric setups on one side, and non-interferometric imaging scheme of amplitude object on the other. In the last case, quantum…

Stimulated Raman scattering (SRS) has played an increasingly pivotal role in chemistry and photonics. Recently, understanding of light-molecule interaction during SRS was brought to a new quantitative level through the introduction of…

Chemical Physics · Physics 2023-12-13 Wei Min , Xin Gao

The ability to identify the contents of a sealed container, without the need to extract a sample, is desirable in applications ranging from forensics to product quality control. One technique suited to this is inverse spatially offset Raman…

In virtual-state spectroscopy, information about the energy-level structure of an arbitrary sample is retrieved by Fourier transforming sets of measured two-photon absorption probabilities of entangled photon pairs where the degree of…

Quantum Physics · Physics 2021-08-04 Lutz Mertenskötter , Kurt Busch , Roberto de J. León-Montiel

This paper presents a study on quantum radar technology developments, design Consideration for its integration, and quantum radar cross-section, QRCS based on quantum electrodynamics and interferometric considerations. Quantum radar systems…

Quantum Physics · Physics 2022-05-30 Manoj Mathews

We employed femtosecond pump probe technique to investigate the dynamics of coherent optical phonons in iron garnet. A phenomenological symmetry-based consideration reveals that oscillations of the terahertz T2g mode are excited. Selective…

In this paper we study the resolution of images illuminated by sources composed of $N+1$ photons in which one non-degenerate photon is entangled with $N$ degenerate photons. The $N$ degenerate photons illuminate an object and are collected…

Quantum Physics · Physics 2008-12-12 Jianming Wen , Morton H. Rubin , Yanhua Shih

We describe two-photon absorption processes excited by entangled pairs, but not by non-entangled pairs of the same energy and polarization. Photon states are selected for destructive interference in the non-entangled process between…

Quantum Physics · Physics 2010-12-21 Keith Kastella , Ralph S. Conti

Improving the resolution of fluorescence microscopy beyond the diffraction limit can be achievedby acquiring and processing multiple images of the sample under different illumination conditions.One of the simplest techniques, Random…

Two-photon excited fluorescence (TPEF) is a standard technique in modern microscopy but still affected by photo-damage of the probe. It was proposed that TPEF can be enhanced by using entangled photons, but has proven to be challenging.…

Quantum Physics · Physics 2013-10-17 Andreas Jechow , Michael Seefeldt , Henning Kurzke , Axel Heuer , Ralf Menzel
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