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The magnetic susceptibility of the gapped quantum spin liquid compound (C$_4$H$_{12}$N$_2$)Cu$_2$Cl$_6$ and its chemically disordered derivatives (C$_4$H$_{12}$N$_2$)Cu$_2$(Cl$_{1-x}$Br$_{x}$)$_6$ are systematically studied in magnetic…

Strongly Correlated Electrons · Physics 2015-06-16 D. Hüvonen , G. Ballon , A. Zheludev

We report a neutron scattering study of the spin-1/2 alternating bond antiferromagnet Cu(NO_3)_2. 2.5D_2O for 0.06<k_BT/J_1<1.5. For k_BT/J_1 << 1 the excitation spectrum is dominated by a coherent singlet-triplet mode centered at…

Strongly Correlated Electrons · Physics 2009-10-31 Guangyong Xu , C. Broholm , Daniel H. Reich , M. A. Adams

Numerous experiments on pyrochlore oxides Pr$_2$(Zr, Sn, Hf, Ir)$_2$O$_7$ with non-Kramers Pr$^{3+}$ ions suggest that they support a quantum spin liquid (QSL) ground state, but the precise nature of the QSL remains unclear. Quantum spin…

Strongly Correlated Electrons · Physics 2025-12-15 Tony An , Félix Desrochers , Yong Baek Kim

A quantum spin liquid (QSL) is an exotic state of matter in which electrons' spins are quantum entangled over long distances, but do not show symmetry-breaking magnetic order in the zero-temperature limit. The observation of QSL states is a…

Strongly Correlated Electrons · Physics 2017-03-08 J. A. M. Paddison , M. Daum , Z. L. Dun , G. Ehlers , Y. Liu , M. B. Stone , H. D. Zhou , M. Mourigal

By performing time-of-flight neutron scattering measurements on a large amount of single crystals of Sr$_2$RuO$_4$, we studied detailed structure of the imaginary part of the dynamic spin susceptibility over a wide range of phase space. In…

Strongly Correlated Electrons · Physics 2015-05-28 K. Iida , M. Kofu , N. Katayama , J. Lee , R. Kajimoto , Y. Inamura , M. Nakamura , M. Arai , Y. Yoshida , M. Fujita , K. Yamada , S. -H. Lee

Frustrated pyrochlore lattices in transition-metal oxides provide an ideal platform for realizing exotic quantum states, including spin liquids with unconventional low-energy excitations arising from the macroscopic ground-state degeneracy…

Strongly Correlated Electrons · Physics 2026-05-26 Satish Kumar , U. Jena , A. Bandhopadhay , G. B. G. Stenning , D. T. Adroja , S. Petit , P. Khuntia

The ground states of the frustrated pyrochlore oxide Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been studied by inelastic neutron scattering experiments. Three single-crystal samples are investigated; one shows no phase transition…

CeTa$_7$O$_{19}$ is a recently found two-dimensional triangular lattice antiferromagnet without showing magnetic order. We grew high-quality CeTa$_7$O$_{19}$ single crystals and studied the low-temperature magnetic susceptibility, specific…

Strongly Correlated Electrons · Physics 2025-03-06 N. Li , A. Rutherford , Y. Y. Wang , H. Liang , Y. Zhou , Y. Sun , D. D. Wu , P. F. Chen , Q. J. Li , H. Wang , W. Xie , E. S. Choi , S. Z. Zhang , M. Lee , H. D. Zhou , X. F. Sun

A quantum spin liquid is a novel ground state that can support long-range entanglement between magnetic moments, resulting in exotic spin excitations involving fractionalized $S=\frac{1}{2}$ spinons. Here, we measure the excitations in…

We study the spin stiffness of a one-dimensional quantum antiferromagnet in the whole range of system sizes $L$ and temperatures $T$. We show that for integer and half-odd integer spin case the stiffness differs fundamentally in its $L$ and…

Condensed Matter · Physics 2009-10-22 Daniel Loss , Dmitrii L. Maslov

We report magnetization and specific heat measurements in the 2D frustrated spin-1/2 Heisenberg antiferromagnet Cs2CuCl4 at temperatures down to 0.05 K and high magnetic fields up to 11.5 T applied along a, b and c-axes. The low-field…

Strongly Correlated Electrons · Physics 2013-06-25 Y. Tokiwa , T. Radu , R. Coldea , H. Wilhelm , Z. Tylczynski , F. Steglich

We used 17O NMR to probe the uniform (wavevector q=0) electron spin excitations up to 800 K in Sr2CuO3 and separate the q=0 from the q=\pm\pi/a staggered components. Our results support the logarithmic decrease of the uniform spin…

Strongly Correlated Electrons · Physics 2009-11-07 K. R. Thurber , A. W. Hunt , T. Imai , F. C. Chou

In conventional spin glasses, the magnetic interaction is not strongly anisotropic and the entire spin system freezes at low temperature. In La2(Cu,Li)O4, for which the in-plane exchange interaction dominates the interplane one, only a…

Disordered Systems and Neural Networks · Physics 2015-06-25 Y. Chen , Wei Bao , Y. Qiu , J. E. Lorenzo , J. L. Sarrao , D. L. Ho , Min Y. Lin

This chapter is intended as a brief overview of some of the quantum spin liquid phases with unbroken SU(2) spin symmetry available in one dimension. The main characteristics of these phases are discussed by means of the bosonization…

Strongly Correlated Electrons · Physics 2007-05-23 P. Lecheminant

Quantum spin liquids are exotic states of matter which form when strongly frustrated magnetic interactions induce a highly entangled quantum paramagnet far below the energy scale of the magnetic interactions. Three-dimensional cases are…

Sr_2Cu_3O_4Cl_2 is an antiferromagnet consisting of weakly coupled CuO planes which comprise two weakly interacting antiferromagnetic subsystems, I and II, which order at respective temperatures T_I \approx 390K and T_{II} \approx 40K.…

Strongly Correlated Electrons · Physics 2009-10-31 A. B. Harris , A. Aharony , O. Entin-Wohlman , I. Ya. Korenblit , R. J. Birgeneau , Y. J. Kim

Quantum fluctuations are expected to lead to highly entangled spin-liquid states in certain two-dimensional spin-1/2 compounds. We have synthesized and measured thermodynamic properties and muon spin relaxation rates in the copper-based…

We report proximate quantum spin liquid behavior in K$_2$Co$_2$(SO$_4$)$_3$ with the magnetic Co$^{2+}$ ions embedded on a highly frustrated three-dimensional double trillium lattice. Single-crystal and high-resolution synchrotron powder…

The layered spiral magnet Cs2CuCl4 displays several interesting properties that have been suggested as evidence of proximity to a two dimensional quantum spin liquid. In this paper we study a concrete version of this proposal and suggest…

Strongly Correlated Electrons · Physics 2009-11-11 S. V. Isakov , T. Senthil , Yong Baek Kim

Na$_4$Ir$_3$O$_8$ is a candidate material for a 3-dimensional quantum spin-liquid on the hyperkagome lattice. We present thermodynamic measurements of heat capacity $C$ and thermal conductivity $\kappa$ on high quality polycrystalline…

Strongly Correlated Electrons · Physics 2015-06-18 Yogesh Singh , Y. Tokiwa , J. Dong , P. Gegenwart
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