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Spin correlations of the frustrated pyrochlore oxide Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been investigated by using inelastic neutron scattering on single crystalline samples ($x=-0.007, 0.000,$ and $0.003$), which have the putative…

Strongly Correlated Electrons · Physics 2019-01-08 Hiroaki Kadowaki , Mika Wakita , Björn Fåk , Jacques Ollivier , Seiko Ohira-Kawamura , Kenji Nakajima , Jeffrey W. Lynn

Magnetic properties of the natural mineral Cu$_2$(OH)$_2$CO$_3$ (malachite) were investigated through DC and AC susceptibility measurements. The analysis of the low-temperature part reveals a quantum spin-gap behavior with $\Delta \approx…

Strongly Correlated Electrons · Physics 2009-10-31 E. Janod , L. Leonyuk , V. Maltsev

LuCuGaO4 has magnetic Cu2+ and diamagnetic Ga3+ ions distributed on a triangular bilayer and is suggested to undergo a spin-glass transition with T_g approximately 0.4 K. Using muSR and neutron scattering measurements, we show that at low…

Materials Science · Physics 2013-05-29 S Calder , SR Giblin , DR Parker , PP Deen , C Ritter , JR Stewart , S Rols , T Fennell

Geometrical frustration among interacting spins combined with strong quantum fluctuations destabilize long-range magnetic order in favour of more exotic states such as spin liquids. By following this guiding principle, a number of spin…

Quantum spin liquids attract great interest due to their exceptional magnetic properties characterized by the absence of long-range order down to low temperatures despite the strong magnetic interaction. Commonly, these compounds are…

Strongly Correlated Electrons · Physics 2018-05-01 Martin Dressel , Andrej Pustogow

Conventional crystalline magnets are characterized by symmetry breaking and normal modes of excitation called magnons with quantized angular momentum $\hbar$. Neutron scattering correspondingly features extra magnetic Bragg diffraction at…

Strongly Correlated Electrons · Physics 2018-10-31 K. W. Plumb , Hitesh J. Changlani , A. Scheie , Shu Zhang , J. W. Kriza , J. A. Rodriguez-Rivera , Yiming Qiu , B. Winn , R. J. Cava , C. L. Broholm

The search for the experimental evidence of quantum spin liquid (QSL) states is critical but extremely challenging, as the quenched interaction randomness introduced by structural imperfection is usually inevitable in real materials.…

Strongly Correlated Electrons · Physics 2022-11-08 Fangjun Lu , Long Yuan , Jian Zhang , Boqiang Li , Yongkang Luo , Yuesheng Li

Using thermodynamic measurements, neutron diffraction, nuclear magnetic resonance, and muon spin relaxation, we establish putative quantum spin-liquid behavior in Ba$_3$InIr$_2$O$_9$, where unpaired electrons are localized on mixed-valence…

Using the density-matrix renormalization group method for the ground state and excitations of the Shastry- Sutherland spin model, we demonstrate the existence of a narrow quantum spin liquid phase between the previously known…

Strongly Correlated Electrons · Physics 2022-03-01 Jianwei Yang , Anders W. Sandvik , Ling Wang

We report 17O NMR measurements in the S=1/2 Cu2+ kagome antiferromagnet Herbertsmithite ZnCu3(OH)6Cl2 down to 45mK in magnetic fields ranging from 2T to 12T. While Herbertsmithite displays a gapless spin-liquid behavior in zero field, we…

Strongly Correlated Electrons · Physics 2013-09-09 M. Jeong , F. Bert , P. Mendels , F. Duc , J. C. Trombe , M. A. de Vries , A. Harrison

Experimental quest for the hypothetical "quantum spin liquid" state has recently met a few promising candidate materials including organic salts \kappa-(ET)2Cu2(CN)3 and EtMe3Sb[Pd(dmit)2]2, S=1/2 triangular-lattice Heisenberg…

Strongly Correlated Electrons · Physics 2015-06-17 Ken Watanabe , Hikaru Kawamura , Hiroki Nakano , Toru Sakai

The two-dimensional (2D) spin-1/2 kagome Heisenberg antiferromagnet is believed to host quantum spin liquid (QSL) states with no magnetic order, but its ground state remains largely elusive. An important outstanding question concerns the…

Strongly Correlated Electrons · Physics 2024-05-30 S. Suetsugu , T. Asaba , Y. Kasahara , Y. Kohsaka , K. Totsuka , B. Li , Y. Zhao , Y. Li , M. Tokunaga , Y. Matsuda

We report that a possible Z2 quantum spin liquid (QSL) can be observed in a new class of frustrated system: spinor bosons subject to a pi flux in a square lattice. We construct a new class of Ginsburg-Landau (GL) type of effective action to…

Strongly Correlated Electrons · Physics 2020-05-12 Fadi Sun , Jinwu Ye

Based on analytical and numerical approaches, we investigate thermodynamic properties of CuSe2O5 at high magnetic fields which is a candidate for the strong intra-chain interaction in quasi one-dimensional (1D) quantum magnets. Magnetic…

Strongly Correlated Electrons · Physics 2015-09-14 Z. Saghafi , J. Jahangiri , S. Mahdavifar , H. Hadipour , S. Farjami Shayesteh

YbZn$_2$GaO$_5$ is a promising candidate for realizing a quantum spin liquid (QSL) state, particularly owing to its lack of significant site disorder. Pulsed-field magnetometry at 0.5 K shows magnetization saturating near 15 T, with a…

The quantum spin liquid (QSL) state is an exotic state of matter featuring a high degree of entanglement and lack of long-range magnetic order in the zero-temperature limit. The triangular antiferromagnet YbMgGaO4 is a candidate QSL host,…

Spin liquid is a state of electron spins in which quantum fluctuation breaks magnetic ordering while maintaining spin correlation. It has been a central topic in magnetism because of its relevance to high-Tc superconductivity and…

Strongly Correlated Electrons · Physics 2016-09-28 Daichi Hirobe , Masahiro Sato , Takayuki Kawamata , Yuki Shiomi , Ken-ichi Uchida , Ryo Iguchi , Yoji Koike , Sadamichi Maekawa , Eiji Saitoh

Despite possessing a local spin $2$ moment on the iron site and a Curie-Weiss temperature of $45K$, the A site spinel FeSc$_2$S$_4$ does not magnetically order down to 50mK. Previous theoretical work by Chen and Balents advanced an…

Strongly Correlated Electrons · Physics 2015-10-28 Daniel Ish , Leon Balents

The existance of a spin disordered ground state for the frustrated Quantum Heisenberg Antiferromagnet on a square lattice is reconsidered. It is argued that there is a unique action which is continuous through the whole phase diagram,…

Condensed Matter · Physics 2009-10-22 Jaime Ferrer

Spin liquids are quantum phases of matter that exhibit a variety of novel features associated with their topological character. These include various forms of fractionalization - elementary excitations that behave as fractions of an…

Strongly Correlated Electrons · Physics 2020-01-20 C. Broholm , R. J. Cava , S. A. Kivelson , D. G. Nocera , M. R. Norman , T. Senthil
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