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Slow dynamics of difluorotetrachloroethane in both supercooled plastic crystal and supercooled liquid states have been investigated from Molecular Dynamics simulations. The temperature and wave-vector dependence of collective dynamics in…

Soft Condensed Matter · Physics 2009-11-11 F. Affouard , M. Descamps

Glasses derive their functional properties from complex relaxation dynamics that remain enigmatic under extreme conditions. While the temperature dependence of these relaxation processes is well-established, their behavior under…

There is a long-standing technological problem in which a stress dwell during cyclic loading at room temperature in Ti causes a significant fatigue life reduction. It is thought that localised time dependent plasticity in soft grains…

Dielectric measurements on molecular liquids just above the glass transition indicate that alpha relaxation is characterized by a generic high-frequency loss varying as $\omega^{-1/2}$, whereas deviations from this come from one or more…

Soft Condensed Matter · Physics 2009-11-11 Jeppe C. Dyre

We propose a dynamic structure of coupled dynamic molecular strings for supercooled small polar molecule liquids and accordingly we obtain the Hamiltonian of the rotational degrees of freedom of the system. From the Hamiltonian, the…

Disordered Systems and Neural Networks · Physics 2009-11-10 Y. N. Huang , C. J. Wang , E. Riande

The glass transition temperature and relaxation dynamics of the segmental motions of thin films of polystyrene labeled with a dye, 4-[N-ethyl-N-(hydroxyethyl)]amino-4-nitraozobenzene (Disperse Red 1, DR1) are investigated using dielectric…

Soft Condensed Matter · Physics 2009-11-13 Rodney D. Priestley , Linda J. Broadbelt , John M. Torkelson , Koji Fukao

The fragilities (Tg-normalized temperature dependence of alpha-relaxation times) of 33 glass-forming liquids and polymers are compared for isobaric, mP, and isochoric, mV, conditions. We find that the two quantities are linearly correlated,…

Soft Condensed Matter · Physics 2009-11-11 R. Casalini , C. M. Roland

Relaxation processes significantly influence the properties of glass materials. However, understanding their specific origins is difficult, even more challenging is to forecast them theoretically. In this study, using microseconds molecular…

Materials Science · Physics 2019-09-09 Yang Sun , Si-Xu Peng , Qun Yang , Feng Zhang , Meng-Hao Yang , Cai-Zhuang Wang , Kai-Ming Ho , Hai-Bin Yu

We present a thorough characterization of the glassy dynamics of three propylene glycols (mono-, di- and trimer) by broadband dielectric spectroscopy. By covering a frequency range of more than 15 decades, we have access to the entire…

Soft Condensed Matter · Physics 2015-05-13 M. Köhler , P. Lunkenheimer , Y. Goncharov , R. Wehn , A. Loidl

With gradual temperature increase in premelting regions of solid phase of methanol and high pressure phase of ethanol, and using novel procedure of separation of electrode polarization effects, we are able to register the contribution of…

Materials Science · Physics 2022-05-11 M. V. Kondrin , A. A. Pronin , Y. B. Lebed , V. V. Brazhkin

Relaxor behavior and lattice dynamics have been studied for a single crystal of K$_{1-x}$Li$_x$TaO$_3$ $(x=0.05)$, where a small amount of a Ca impurity ($\sim 15$~ppm) was incorporated. The dielectric measurements revealed Debye-like…

Materials Science · Physics 2009-11-11 S. Wakimoto , G. A. Samara , R. K. Grubbs , E. L. Venturini , L. A. Boatner , G. Xu , G. Shirane , S. -H. Lee

The incoherent dynamic structure factor of ortho-terphenyl has been measured by neutron time-of-flight and backscattering technique in the pressure range from 0.1 MPa to 240 MPa for temperatures between 301 K and 335 K. Tagged-particle…

Statistical Mechanics · Physics 2011-04-05 A. Toelle , H. Schober , J. Wuttke , F. Fujara

The frequency and temperature dependence of the dielectric constant and the electrical conductivity of the transparent glasses in the composition Li2O-3B2O3 (LBO) were investigated in the 100 Hz- 10 MHz frequency range. The dielectric…

Materials Science · Physics 2015-05-19 Rahul Vaish , K. B. R. Varma

The polymer relaxation dynamic of a sample, stretched up to the stress hardening regime, is measured, at room temperature, as a function of the strain $\lambda$ for a wide range of the strain rate $\dot\gamma$, by an original dielectric…

Soft Condensed Matter · Physics 2020-03-11 R. Sahli , J. Hem , C. Crauste-Thibierge , F. Clément , D Long , S. Ciliberto

Ion conducting $(CaO)_x(SiO_2)_{1-x}$ glasses and melts show a threshold behaviour in dc conductivity near $x=x_t=0.50$, with conductivities increasing linearly at $x>x_t$. We show that the behaviour can be traced to a rigid ($x<0.50$) to…

Materials Science · Physics 2009-11-10 M. Malki , M. Micoulaut , F. Chaimbault , Y. Vaills , P. Simon

We present a dielectric study on the dynamics of supercooled glycerol during crystallization. We explore the transformation into a solid phase in real time by monitoring the temporal evolution of the amplitude of the dielectric signal.…

Soft Condensed Matter · Physics 2017-03-01 Alejandro Sanz , Kristine Niss

We present a molecular dynamics study of the liquid and plastic crystalline phases of CCl$_3$Br. We investigated the short-range orientational order using a recently developed classification method and we found that both phases behave in a…

Chemical Physics · Physics 2015-06-16 Nirvana Caballero , Mariano Zuriaga , Marcelo Carignano , Pablo Serra

We investigate the relaxation behavior of thin films of a polyamide random copolymer, PA66/6I, with various film thicknesses using dielectric relaxation spectroscopy. Two dielectric signals are observed at high temperatures, the…

Soft Condensed Matter · Physics 2015-06-11 Natsumi Taniguchi , Koji Fukao , Paul Sotta , Didier R. Long

The molecular dynamics in the ambient-pressure solid phase of (1,1,2)-trichloroethane is studied by means of broadband dielectric spectroscopy and molecular dynamics simulations. The dielectric spectra of polycrystalline samples obtained by…

The out-of-equilibrium excess conductance of electron-glasses typically relaxes with a logarithmic time-dependence. Here it is shown that the log(t) relaxation of a weakly-disordered amorphous indium-oxide films crosses-over asymptotically…

Disordered Systems and Neural Networks · Physics 2018-06-04 Z. Ovadyahu