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Despite decades of studies on the grand problem of the glass transition the question of well-defined universal patterns, including the key problem of the previtreous behavior of the primary (structural) relaxation time, remains elusive.…

Soft Condensed Matter · Physics 2018-09-18 Aleksandra Drozd-Rzoska

Brillouin scattering has been used to measure the dynamic structure factor of glycerol as a function of temperature from the high temperature liquid to the glassy state. Our investigation aims at understanding the number and the nature of…

Soft Condensed Matter · Physics 2009-11-10 Lucia Comez , Daniele Fioretto , Filippo Scarponi , Giulio Monaco

We present the results of broadband dielectric spectroscopy on two glass formers with strong Johari-Goldstein beta-relaxations. In addition to the alpha- and beta-relaxation dynamics, the extension of the spectra up to 1 THz also allows…

Soft Condensed Matter · Physics 2011-02-16 S. Kastner , M. Köhler , Y. Goncharov , P. Lunkenheimer , A. Loidl

Low-frequency Raman and inelastic neutron scattering of amorphous bis-phenol A polycarbonate is measured at low temperature, and compared. The vibrational density of states and light-vibration coupling coefficient are determined. The…

Disordered Systems and Neural Networks · Physics 2009-10-31 L. Saviot , E. Duval , J. F. Jal , A. J. Dianoux

Electrical conductivity of dry, slow cooled (AgPO$_3$)$_{1-x}$(AgI)$_x$ glasses is examined as a function of temperature, frequency and glass composition. From these data compositional trends in activation energy for conductivity E$_A$(x),…

Materials Science · Physics 2015-05-14 M. Micoulaut , M. Malki , D. I. Novita , P. Boolchand

Using molecular dynamics simulation we examine dynamics in sheared polycrystal states in a binary mixture containing 10% larger particles in two dimensions. We find large stress fluctuations arising from sliding motions of the particles at…

Soft Condensed Matter · Physics 2009-11-13 Toshiyuki Hamanaka , Akira Onuki

The detailed nature of spatially heterogeneous dynamics of glycerol-silica nanocomposites is unraveled by combining dielectric spectroscopy with atomistic simulation and statistical mechanical theory. Analysis of the spatial mobility…

We demonstrate that plastic deformation in solids is associated with a dynamic transition that is reminiscent to the transition from a superconducting to a mixed phase in Type II superconductors. We report analytic calculations, extensive…

Soft Condensed Matter · Physics 2016-12-06 Saswati Ganguly , Juergen Horbach , Peter Sollich , Smarajit Karmakar , Surajit Sengupta

Microscopic relaxation timescales are estimated from the autocorrelation functions obtained by dynamic light scattering experiments for Laponite suspensions with different concentrations ($C_{L}$), added salt concentrations ($C_{S}$) and…

Soft Condensed Matter · Physics 2016-01-20 Debasish Saha , Yogesh M. Joshi , Ranjini Bandyopadhyay

We investigate the Johari-Goldstein (JG) $\beta$-relaxation process in a model metallic glass-forming (GF) material (Al90Sm10), previously studied extensively by both frequency-dependent mechanical measurements and simulation studies…

Materials Science · Physics 2021-03-09 Hao Zhang , Xinyi Wang , Hai-Bin Yu , Jack F. Douglas

Results of broadband dielectric spectroscopy and rheological studies of poly(propylene glycol) + SiO${_2}$ nanocomposites are presented. They show that the dynamics in high-concentrated composite is determined by confinement and adsorption…

Soft Condensed Matter · Physics 2017-02-24 M. Głuszek , A. Antosik , R. Żurowski , M. Szafran , S. J. Rzoska , M. Zalewski , E. Pawlikowska , S. Starzonek

An analysis of the glass transition of four materials with similar chemical structures is performed: PET, PEN and two PET/PEN blends (90/10 and 70/30 w/w). During the melt processing of the blends transesterification reactions yield block…

Materials Science · Physics 2015-06-05 J. Sellares , J. A. Diego , J. C. Canadas , M. Mudarra , J. Belana , P. Colomer , F. Roman , Y. Calventus

Advances in high-precision dielectric spectroscopy has enabled access to non-linear susceptibilities of polar molecular liquids. The observed non-monotonic behavior has been claimed to provide strong support for theories of dynamic arrest…

Soft Condensed Matter · Physics 2021-07-07 Thomas Speck

We present a mean-field theory of a coarse-grained model of a super-cooled liquid in which relaxation occurs via local plastic rearrangements. Local relaxation can be induced by thermal fluctuations or by the long-range elastic consequences…

Soft Condensed Matter · Physics 2023-12-07 Joseph W. Baron , Giulio Biroli

Plastic rearrangements play a crucial role in the characterization of soft-glassy materials, such as emulsions and foams. Based on numerical simulations of soft-glassy systems, we study the dynamics of plastic rearrangements at the…

Soft Condensed Matter · Physics 2014-10-27 R. Benzi , M. Sbragaglia , A. Scagliarini , P. Perlekar , M. Bernaschi , S. Succi , F. Toschi

As a nontrivial solid state of matter, the glassy-crystal state embraces physical features of both crystalline and amorphous solids, where a long-range ordered periodic structure formed by the mass centers of constituent molecules…

Molecular dynamics simulations are performed to investigate heterogeneous dynamics in amorphous glassy materials under oscillatory shear strain. We consider three-dimensional binary Lennard-Jones mixture well below the glass transition…

Soft Condensed Matter · Physics 2013-05-10 Nikolai V. Priezjev

The relaxation dynamics of glass-forming systems shows a multitude of features that are absent in normal liquids, such as non-exponential relaxation and a strong temperature-dependence of the relaxation time. Connecting these dynamic…

Disordered Systems and Neural Networks · Physics 2019-04-03 Zhen Wei Wu , Walter Kob , Wei-Hua Wang , Limei Xu

Present paper reports, the structural, microstructural, electrical, dielectric properties and ion dynamics of a sodium based solid polymer electrolyte films comprising of PEO8-NaPF6+ x wt. % SN. The structural and surface morphology…

Materials Science · Physics 2018-07-12 Anil Arya , A. L. Sharma*

Relaxor ferroelectrics are difficult to study and understand. The experiment shows that at low energy scattering there is an acoustic mode, an optic mode, dynamic quasi-elastic scattering and strictly elastic scattering as well as Bragg…

Materials Science · Physics 2008-08-29 R. A. Cowley , S. N. Gvasaliya , B. Roessli
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