English

Spin coherence and dephasing of localized electrons in monolayer MoS$_2$

Materials Science 2016-02-11 v1 Mesoscale and Nanoscale Physics

Abstract

We report a systematic study of coherent spin precession and spin dephasing in electron-doped monolayer MoS2_2. Using time-resolved Kerr rotation spectroscopy and applied in-plane magnetic fields, a nanosecond-timescale Larmor spin precession signal commensurate with gg-factor g01.86|g_0|\simeq 1.86 is observed in several different MoS2_2 samples grown by chemical vapor deposition. The dephasing rate of this oscillatory signal increases linearly with magnetic field, suggesting that the coherence arises from a sub-ensemble of localized electron spins having an inhomogeneously-broadened distribution of gg-factors, g0+Δgg_0 + \Delta g. In contrast to g0g_0, Δg\Delta g is sample-dependent and ranges from 0.042 to 0.115.

Keywords

Cite

@article{arxiv.1511.03255,
  title  = {Spin coherence and dephasing of localized electrons in monolayer MoS$_2$},
  author = {Luyi Yang and Weibing Chen and Kathleen M. McCreary and Berend T. Jonker and Jun Lou and Scott A. Crooker},
  journal= {arXiv preprint arXiv:1511.03255},
  year   = {2016}
}

Comments

5 pages, 4 figures. Accepted and in press, Nano Letters