We report a systematic study of coherent spin precession and spin dephasing in electron-doped monolayer MoS2. Using time-resolved Kerr rotation spectroscopy and applied in-plane magnetic fields, a nanosecond-timescale Larmor spin precession signal commensurate with g-factor ∣g0∣≃1.86 is observed in several different MoS2 samples grown by chemical vapor deposition. The dephasing rate of this oscillatory signal increases linearly with magnetic field, suggesting that the coherence arises from a sub-ensemble of localized electron spins having an inhomogeneously-broadened distribution of g-factors, g0+Δg. In contrast to g0, Δg is sample-dependent and ranges from 0.042 to 0.115.
@article{arxiv.1511.03255,
title = {Spin coherence and dephasing of localized electrons in monolayer MoS$_2$},
author = {Luyi Yang and Weibing Chen and Kathleen M. McCreary and Berend T. Jonker and Jun Lou and Scott A. Crooker},
journal= {arXiv preprint arXiv:1511.03255},
year = {2016}
}
Comments
5 pages, 4 figures. Accepted and in press, Nano Letters