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Dynamical Jahn-Teller Effect in Spin-Orbital Coupled System

Strongly Correlated Electrons 2015-06-11 v2 Materials Science

Abstract

Dynamical Jahn-Teller (DJT) effect in a spin-orbital coupled system on a honeycomb lattice is examined, motivated from recently observed spin-liquid behavior in Ba3_3CuSb2_2O9_9. An effective vibronic Hamiltonian, where the superexchange interaction and the DJT effect are taken into account, is derived. We find that the DJT effect induces a spin-orbital resonant state where local spin-singlet states and parallel orbital configurations are entangled with each other. This spin-orbital resonant state is realized in between an orbital ordered state, where spin-singlet pairs are localized, and an antiferromagnetic ordered state. Based on the theoretical results, a possible scenario for Ba3_3CuSb2_2O9_9 is proposed.

Keywords

Cite

@article{arxiv.1209.0239,
  title  = {Dynamical Jahn-Teller Effect in Spin-Orbital Coupled System},
  author = {Joji Nasu and Sumio Ishihara},
  journal= {arXiv preprint arXiv:1209.0239},
  year   = {2015}
}

Comments

13 pages, 8 figures, to be published in PRB

R2 v1 2026-06-21T21:58:43.310Z