English

Resonating Valence-Bond State in an Orbitally Degenerate Quantum Magnet with Dynamical Jahn-Teller Effect

Strongly Correlated Electrons 2015-06-23 v1 Materials Science

Abstract

Short-range resonating-valence bond states in an orbitally degenerate magnet on a honeycomb lattice is studied. A quantum-dimer model is derived from the Hamiltonian which represents the superexchange interaction and the dynamical Jahn-Teller (JT) effect. We introduce two local units termed "spin-orbital singlet dimer", where two spins in a nearest-neighbor bond form a singlet state associated with an orbital polarization along the bond, and "local JT singlet", where an orbital polarization is quenched due to the dynamical JT effect. A derived quantum-dimer model consists of the hopping of the spin-orbital singlet dimers and the JT singlets, and the chemical potential of the JT singlets. We analyze the model by the mean-field approximation, and find that a characteristic phase, termed "JT liquid phase", where both the spin-orbital singlet dimers and the JT singlets move quantum mechanically, is realized. Possible scenarios for the recently observed non magnetic-ordered state in Ba3_3CuSb2_2O9_9 are discussed.

Keywords

Cite

@article{arxiv.1410.6009,
  title  = {Resonating Valence-Bond State in an Orbitally Degenerate Quantum Magnet with Dynamical Jahn-Teller Effect},
  author = {Joji Nasu and Sumio Ishihara},
  journal= {arXiv preprint arXiv:1410.6009},
  year   = {2015}
}

Comments

8 pages, 7 figures