English

Classical dimers and dimerized superstructure in orbitally degenerate honeycomb antiferromagnet

Strongly Correlated Electrons 2008-04-12 v2 Statistical Mechanics

Abstract

We discuss the ground state of the spin-orbital model for spin-one ions with partially filled t2gt_{2g} levels on a honeycomb lattice. We find that the orbital degrees of freedom induce a spontaneous dimerization of spins and drive them into nonmagnetic manifold spanned by hard-core dimer (spin-singlet) coverings of the lattice. The cooperative ``dimer Jahn-Teller'' effect is introduced through a magnetoelastic coupling and is shown to lift the orientational degeneracy of dimers leading to a peculiar valence bond crystal pattern. The present theory provides a theoretical explanation of nonmagnetic dimerized superstructure experimentally seen in Li2_2RuO3_3 compound at low temperatures.

Keywords

Cite

@article{arxiv.0802.2692,
  title  = {Classical dimers and dimerized superstructure in orbitally degenerate honeycomb antiferromagnet},
  author = {G. Jackeli and D. I. Khomskii},
  journal= {arXiv preprint arXiv:0802.2692},
  year   = {2008}
}

Comments

to appear in Phys. Rev. Lett

R2 v1 2026-06-21T10:13:53.666Z