English

Spin Order due to Orbital Fluctuations: Cubic Vanadates

Strongly Correlated Electrons 2009-11-07 v1

Abstract

We investigate the highly frustrated spin and orbital superexchange interactions in cubic vanadates. The fluctuations of t2gt_{2g} orbitals trigger a {\it novel mechanism of ferromagnetic interactions} between spins S=1 of V3+^{3+} ions along one of the cubic directions which operates already in the absence of Hund's rule exchange JHJ_H, and leads to the C-type antiferromagnetic phase in LaVO3_3. The Jahn-Teller effect can stabilize the orbital ordering and the G-type antiferromagnetic phase at low temperatures, but large entropy due to orbital fluctuations favors again the C-phase at higher temperatures, as observed in YVO3_3.

Keywords

Cite

@article{arxiv.cond-mat/0103300,
  title  = {Spin Order due to Orbital Fluctuations: Cubic Vanadates},
  author = {G. Khaliullin and P. Horsch and A. M. Oles},
  journal= {arXiv preprint arXiv:cond-mat/0103300},
  year   = {2009}
}

Comments

4 pages, 3 figures, to appear in Phys. Rev. Lett

R2 v1 2026-07-22T10:18:15.969Z