English

Interplay of the Jahn--Teller Effect and Spin-Orbit Coupling: The Case of Trigonal Vibronic Modes

Materials Science 2022-07-26 v2

Abstract

We study an interplay between the orbital degeneracy and spin-orbit coupling giving rise to spin-orbital entangled states. As a specific example, we analyze the interaction of electrons occupying triply degenerate single-ion t2gt_{2g} levels with trigonal vibronic modes (the tTt\otimes T problem). A more general problem of the electron-lattice interaction involving both tetragonal and trigonal vibrations is also considered. It is shown that the result of such interaction crucially depends on the occupation of t2gt_{2g} levels leading to either the suppression or enhancement of the Jahn-Teller effect by the spin-orbit coupling.

Keywords

Cite

@article{arxiv.2203.02243,
  title  = {Interplay of the Jahn--Teller Effect and Spin-Orbit Coupling: The Case of Trigonal Vibronic Modes},
  author = {S. V. Streltsov and F. V. Temnikov and K. I. Kugel and D. I. Khomskii},
  journal= {arXiv preprint arXiv:2203.02243},
  year   = {2022}
}

Comments

11 pages, 10 figures