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Dynamical decoupling pulse sequences have been used to extend coherence times in quantum systems ever since the discovery of the spin-echo effect. Here we introduce a method of recursively concatenated dynamical decoupling pulses, designed…

量子物理 · 物理学 2007-05-23 K. Khodjasteh , D. A. Lidar

Nuclear spins are promising candidates for quantum information processing because their good isolation from the environment precludes the rapid loss of quantum coherence. Many strategies have been developed to further extend their…

Dynamic nuclear polarisation (DNP) refers to a class of techniques used to increase the signal in nuclear magnetic resonance measurements by transferring spin polarisation from ensembles of highly polarised electrons to target nuclear…

量子物理 · 物理学 2020-12-24 L. T. Hall , D. A. Broadway , A. Stacey , D. A. Simpson , J-P. Tetienne , L. C. L. Hollenberg

We introduce a method to rotate arbitrarily the excitation profile of universal broadband composite pulse sequences for robust high-fidelity population inversion. These pulses compensate deviations in any experimental parameter (e.g. pulse…

量子物理 · 物理学 2020-02-20 Genko T. Genov , Marcel Hain , Nikolay V. Vitanov , Thomas Halfmann

We present a study of the prospects for coherence preservation in solid-state spin qubits using dynamical decoupling protocols. Recent experiments have provided the first demonstrations of multipulse dynamical decoupling sequences in this…

介观与纳米尺度物理 · 物理学 2013-05-29 M. J. Biercuk , H. Bluhm

Dynamical decoupling multipulse sequences can be applied to solid state spins for sensing weak oscillating fields from nearby single nuclear spins. By periodically reversing the probing system's evolution, other noises are counteracted and…

We discuss the implementation of arbitrary precision composite pulses developed using the methods of Brown et al. [Phys. Rev. A 70 (2004) 052318]. We give explicit results for pulse sequences designed to tackle both the simple case of pulse…

量子物理 · 物理学 2007-11-05 William G. Alway , Jonathan A. Jones

Hyperpolarisation using Signal Amplification By Reversible Exchange (SABRE) is a convenient method for high repeatability studies. The core of this technique is polarisation transfer to the target substrate during an on-going chemical…

Asymmetrical horizontal interdot coupling was demonstrated to exist in a system of a single plane of self-assembled CdTe/ZnTe quantum dots. Photoluminescence excitation (PLE), second order photon correlation and optical orientation were…

其他凝聚态物理 · 物理学 2009-06-12 T. Kazimierczuk , J. Suffczynski , P. Wojnar , A. Golnik , J. A. Gaj , P. Kossacki

We investigate the dynamic nuclear polarization process by frequently injecting polarized electron spins into a quantum dot. Due to the suppression of the direct dipolar and indirect electron-mediated nuclear spin interactions, by the…

介观与纳米尺度物理 · 物理学 2016-07-26 Na Wu , Wenkui Ding , Anqi Shi , Wenxian Zhang

Taking inspiration from NMR spectroscopy, periodic irradiation schemes have recently shown remarkable performance when implemented into pulsed dynamic nuclear polarization (DNP) sequences. This has prompted considerable interest in…

We demonstrate a new resonance condition that obeys the relation ${\Delta}{\delta}=n{\nu}_{R}/2$, where ${\Delta}{\delta}$ is the chemical shift difference between two homonuclear-coupled spins, ${\nu}_{R}$ is the magic-angle spinning speed…

化学物理 · 物理学 2022-04-06 Orr Simon Lusky , Amir Goldbourt

We introduce a theoretical framework for computaions of anisotropic multipolar exchange interactions found in many spin--orbit coupled magnetic systems and propose a method to extract these coupling constants using a density functional…

强关联电子 · 物理学 2014-08-01 Shu-Ting Pi , Ravindra Nanguneri , Sergey Savrasov

Inverse problems, where the goal is to recover an unknown signal from noisy or incomplete measurements, are central to applications in medical imaging, remote sensing, and computational biology. Diffusion models have recently emerged as…

机器学习 · 计算机科学 2026-01-15 Shayan Mohajer Hamidi , En-Hui Yang , Ben Liang

Finding control fields (pulse sequences) that can compensate for the dispersion in the parameters governing the evolution of a quantum system is an important problem in coherent spectroscopy and quantum information processing. The use of…

量子物理 · 物理学 2007-05-23 Navin Khaneja , Jr-Shin Li

General analytical expressions for Double Quantum Nuclear Magnetic Resonance (NMR) kinetic curves of many-spin I=1/2 systems are derived with an accuracy of the second cumulant approximation. The expressions obtained exactly describe the…

软凝聚态物质 · 物理学 2015-06-17 N. Fatkullin , C. Mattea , S. Stapf

Pulsed Dynamic Nuclear Polarization (DNP) is currently receiving substantial interest as a means to enhance the sensitivity of nuclear magnetic resonance (NMR) and magnetic resonance imaging (MRI) by orders of magnitude. It has also…

Due to their nonlinear properties, spin transfer nano-oscillators can easily adapt their frequency to external stimuli. This makes them interesting model systems to study the effects of synchronization and brings some opportunities to…

Recently, Pang et al reported a novel polarization transfer scheme applicable to three-spin systems, whereby a rotating-frame NMR analogue of the cross effect could transfer polarization between; e.g., two 13Cs and an 15N in a single…

量子物理 · 物理学 2026-04-21 Sundaresan Jayanthi , Adonis Lupulescu , Julia Grinshtein , Lucio Frydman

This paper employs the general time-space fractional diffusion equation to derive correlation time function for analyzing nuclear magnetic resonance (NMR) relaxation. Both the anomalous rotational and translational diffusion are treated.…

化学物理 · 物理学 2018-12-31 Guoxing Lin