相关论文: Two-Pulse Atomic Coherent Control (2PACC) Spectros…
Attosecond pulses can ionize atoms in a coherent process. Since the emerging fragments are entangled, however, each preserves only a fraction of the initial coherence, thus limiting the chance of guiding the ion subsequent evolution. In…
The rotational echo response of molecules is found to strongly depend on the delay between the two ultrashort laser pulses, as opposed to two-level systems. We study this dependence experimentally and theoretically and show that by…
In this work we report ab initio calculations for the $H_2^+$ molecule interacting with ultrashort intense laser pulses. We analyse several observables that can, in principle, be available experimentally, in order to get a deeper…
Understanding and controlling the electronic as well as ro-vibrational motion and, thus, the entire chemical dynamics in molecules is the ultimate goal of ultrafast laser and imaging science. In photochemistry, laser-induced dissociation…
A high sensitivity atom flux sensor based on atomic absorption spectroscopy has been designed and implemented to control electron beam evaporators and effusion cells in a molecular beam epitaxy system. Using a high-resolution spectrometer…
Coherence among rotational ion channels during photoionization is exploited to control the anisotropy of the resulting photoelectron angular distributions at specific photoelectron energies. The strategy refers to a robust and single…
The coherent dipole-dipole interactions of atoms in an atomic array are studied. It is found that the excitation probability of an atom in an array parallel to the direction of laser propagation ($\boldsymbol{\hat{k}}$) will either grow or…
In recent years it became possible to align molecules in free space using ultrashort laser pulses. Here we explore two schemes for controlling molecule-surface scattering process, which are based on the laser-induced molecular alignment. In…
Today's high-intensity laser facilities produce short pulses can, in tight focus, reach peak intensities of $10^{22}\,\mathrm{Wcm}^{-2}$ and, in long focus, wakefield-accelerate electrons to GeV energies. The radiation-reaction--dominated…
We theoretically propose a multidimensional high-harmonic echo spectroscopy technique which utilizes strong optical fields to resolve coherent electron dynamics spanning an energy range of multiple electron Volts. Using our recently…
A Computationally Assisted Spectroscopic Technique to measure secondary electron emission coefficients ($\gamma$-CAST) in capacitively-coupled radio-frequency plasmas is proposed. This non-intrusive, sensitive diagnostic is based on a…
Interactions between particles in quantum many-body systems play a crucial role in determining the electric, magnetic, optical, and thermal properties of the system. The recent progress in the laser-pulse technique has enabled the…
Coherent control of the atomic two-photon absorption with shaped single-cycle pulses is examined theoretically in the weak-field regime. The control over the stabilized carrier-envelope phase (CEP) of the pulses is determined as a key…
We present an analysis of atomic diffraction due to the interaction of an atomic beam with a pair of Gaussian light pulses. We derive a simple analytical expression for the populations in different diffraction orders. The validity of the…
We theoretically study a pulsed stimulated two-photon Raman outcoupler for an atom laser using a full three-dimensional description. A finite-temperature trapped Bose-condensed atomic gas is treated self-consistently by the…
Optimal control experiments can readily identify effective shaped laser pulses, or "photonic reagents", that achieve a wide variety of objectives. For many practical applications, an important criterion is that a particular photonic reagent…
By analyzing ``exact'' theoretical results from solving the time-dependent Schr\"odinger equation of atoms in few-cycle laser pulses, we established the general conclusion that differential elastic scattering and photo-recombination cross…
We observed two-photon emission signals from the first vibrationally excited state of parahydrogen gas excited coherently by counter-propagating laser pulses. A single narrow-linewidth laser source was used to excite the parahydrogen…
We investigate theoretically the optical properties of an atomic gas which has been cooled by the laser cooling method velocity-selective coherent population trapping. We demonstrate that the application of a weak laser pulse gives rise to…
Coherent control, a central concept in physics and chemistry, has sparked significant interest due to its ability to fine-tune interference effects in atoms and individual molecules for applications ranging from light-harvesting complexes…