相关论文: Photoinduced optical rotation in a racemic mixture…
We study optical excitations of an ultracold gas in an optical lattice in the Mott insulator case and with anisotropic properties. The anisotropy is induced by an oriented transition dipole generated by optical pumping and external static…
Optical activity is the ability of chiral materials to rotate linearly-polarized (LP) electromagnetic waves. Because of their intrinsic asymmetry, traditional chiral molecules usually lack isotropic performance, or at best only possess a…
We study the dynamics of paramagnetic molecular superrotors in an external magnetic field. Optical centrifuge is used to create dense ensembles of oxygen molecules in ultra-high rotational states. It is shown for the first time, that the…
Photoelectron circular dichroism refers to the forward/backward asymmetry in the photoelectron angular distribution with respect to the propagation axis of circularly polarized light. It has recently been demonstrated in femtosecond…
In this paper, we discuss the possibility of imaging molecular orbitals from photoelectron spectra obtained via Laser Induced Electron Diffraction (LIED) in linear molecules. This is an extension of our work published recently in Physical…
We consider optical properties of a gas of molecules that are brought to fast unidirectional spinning by a pulsed laser field. It is shown that a circularly polarized probe light passing through the medium inverts its polarization…
Chirality is a highly important topic in modern chemistry, given the dramatically different pharmacological effects that enantiomers can have on the body. Chirality of natural molecules can be controlled by reconfiguration of molecular…
Using an example of a Raman active medium we describe how a common nonlinear process of four-wave mixing can be used to induce strong coupling between the spatial and temporal degrees of freedom in optical waves. This coupling produces…
Charge and spin dynamics is addressed in chiral molecules immediately after the instantaneous coupling to an external metallic reservoir. It is shown how a spin-polarization is induced in the chiral structure as a response to the charge…
The incorporation of structured light techniques into vision science has enabled more selective probes of polarization related entoptic phenomena. Diverse sets of stimuli have become accessible in which the spatially dependant optical…
We theoretically introduce a scheme to perform Ramsey spectroscopy on a racemic mixture of chiral molecules, simultaneously extracting the transition frequencies of the left- and right-handed molecules, known as enantiomers. By taking the…
Orbital angular momentum (OAM) carried by helical light beams is an unbounded degree of freedom of photons that offers a promising playground in modern photonics. So far, integrated sources of coherent light carrying OAM are based on…
Chirality describes the asymmetry between an object and its mirror image and manifests itself in diverse functionalities across all scales of matter - from molecules and aggregates to thin films and bulk chiral materials. A particularly…
Photoelectron circular dichroism results from one-photon ionization of chiral molecules by circularly polarized light and manifests itself in forward-backward asymmetry of electron emission in the direction orthogonal to the light…
Drawing inspiration from a remarkable chiral force found in nature, we show that a static electric field combined with an optical lin$\perp$lin polarization standing wave can exert a chiral optical force on a small chiral molecule that is…
We calculate optical forces and torques exerted on a chiral dipole by chiral light fields and reveal genuinely chiral forces in combining the chiral contents of both light field and dipolar matter. Here, the optical chirality is…
Following excitation by a strong ultra-short laser pulse, molecules develop coordinated rotational motion, exhibiting transient alignment along the direction of the laser electric field, followed by periodic full and fractional revivals…
Dynamic hybrid optical pumping effects with a radio-frequency-field-driven nonlinear magneto-optical rotation (RF NMOR) scheme are studied in a dual-species paraffin coated vapor cell. By pumping K atoms and probing $^{87}$Rb atoms, we…
Enantioselective photochemistry provides access to unique molecular structures and functions, with deep implications for fundamental science and industrial applications. Current methods for highly enantioselective photochemistry critically…
We present a combined theoretical and experimental work investigating the angle-resolved phases of the photoionization process driven by a two-color field consisting of an attosecond pulse train and an infrared pulse in an ensemble of…