相关论文: Photoinduced optical rotation in a racemic mixture…
Most large molecules are chiral in their structure: they exist as two enantiomers, which are mirror images of each other. Whereas the rovibronic sublevels of two enantiomers are almost identical, it turns out that the photoelectric effect…
It has been long recognized that the spatial polarization of the electronic clouds in molecules, and the spatial arrangements of atoms into chiral molecular structures, play crucial roles in physics, chemistry and biology. However, these…
We consider the optical dipole potential energy, which arises from the interaction of a two-level atom with a circularly polarized Laguerre-Gaussian laser beam of small waist. The beam is characterized by the existence of a longitudinal…
Enantiomers are chiral molecules that exist in right-handed and left-handed conformations. Optical techniques of enantiomers detection are widely employed to discriminate between left- and right-handed molecules. However, identical spectra…
The creation and detection of atomic polarization is examined theoretically, through the study of basic optical-pumping mechanisms and absorption and fluorescence measurements, and the dependence of these processes on the size of ground-…
Chirality causes symmetry breaks in a large variety of natural phenomena ranging from particle physics to biochemistry. We investigate one of the simplest conceivable chiral systems, a laser-excited, oriented, effective one-electron Li…
Chirality is a pervasive form of symmetry that is intimately connected to the physical properties of solids, as well as the chemical and biological activity of molecular systems. However, its control with light is challenging, because…
It has been assumed that optical activity can be measured by illuminating alternatively a material with left- and right- handed circular polarized light and analyzing the differential response. This simple and intuitive approach is in…
Optical chiral properties of a resonant hybrid photonic crystal (RHPC) are computed taking into account spin-orbit effect due to light-hole excitons perfectly confined in 2D quantum wells. The trends of the optical activity, expressed as a…
A highly-efficient method for optical detection and separation of left- and right-handed chiral molecules is presented. The method utilizes a closed-loop three-state system in which the population dynamics depends on the phases of the three…
Quantum entanglement has emerged as a great resource for interactions between molecules and radiation. We propose a new paradigm of stimulated Raman scattering with entangled photons. A quantum ultrafast Raman spectroscopy is developed for…
Measuring and controlling the ionization dynamics by intense laser fields has recently led to important breakthroughs, from the investigation of tunneling time delays to attosecond molecular imaging by electron holography. In these…
Quantifying the optical chirality of a sample requires the precise measurement of the rotation of the plane of linear polarisation of the transmitted light. Central to this notion is that the sample needs to be exposed to light of a defined…
The topological response of matter to electromagnetic fields is a property in high demand in materials design and metrology due to its robustness against noise and decoherence, stimulating recent advances in ultrafast photonics. Embedding…
Light interacts differently with left and right handed three dimensional chiral objects, like helices, and this leads to the phenomenon known as optical activity. Here, by applying a polarization tomography, we show experimentally, for the…
Optical chirality (OC) - one of the fundamental quantities of electromagnetic fields - corresponds to the instantaneous chirality of light. It has been utilized for exploring chiral light-matter interactions in linear optics, but has not…
Chirality is ubiquitous in nature and fundamental in science, from particle physics to metamaterials.The most established technique of chiral discrimination - photoabsorption circular dichroism - relies on the magnetic properties of a…
The evolution versus pump power of the spectrum of a singly resonant optical parametric oscillator based on an MgO-doped periodically poled stoichiometric lithium tantalate crystal is observed. The onset of cascade Raman lasing due to…
This is a sequel to an earlier article on the theory of angular correlation for double photoionization. Here we consider the two-step double photoionization of a rare gas atom under the influence of a polarized photon beam described by…
We suggest a novel mechanism to induce the motion of a chiral material body towards an optical source. Our solution is based on the interference between a chiral light beam and its reflection on an opaque mirror. Surprisingly, it is…