相关论文: Pump and Probe nonlinear processes: new modified s…
The nonlinear oscillator model allows a basic understanding of all nonlinear processes and can be adopted to analyse optical vibrational modes and electronic transition in molecules and crystals, in order to derive general properties of…
Along the lines of the nonlinear response theory developed by Ruelle, in a previous paper we have proved under rather general conditions that Kramers-Kronig dispersion relations and sum rules apply for a class of susceptibilities describing…
Using sum rules, the dipolar terms can be eliminated from the commonly-used sum-over-states (SOS) expression for nonlinear susceptibilities. This new dipole-free expression is more compact, converges to the same results as the common SOS…
The nonlinear response of stochastic models obeying a master equation is calculated up to fifth-order in the external field thus extending the third-order results obtained earlier (G. Diezemann, Phys. Rev. E{\bf 85}, 051502 (2012)). For…
A generic physical situation is considered where Im $\Pi$, the imaginary part of polarization operator (generalized susceptibility), can be measured on a finite interval and the high frequency asymptotics (up to a few orders) of $\Pi$ can…
Generally, natural scientific problems are so complicated that one has to establish some effective perturbation or nonperturbation theories with respect to some associated ideal models. In this Letter, a new theory that combines…
To add the detailed information to the existed knowledge of nonlinear optics field, the nonlinear optical processes of the second and third order have been discussed in their respective susceptibility tensors in the presence of degenerate…
Partial sum rules are widely used in physics to separate low- and high-energy degrees of freedom of complex dynamical systems. Their application, though, is challenged in practice by the always finite spectrometer bandwidth and is often…
Pump-probe microscopy is an emerging nonlinear imaging technique based on high repetition rate lasers and fast intensity modulation. Here we present new methods for pump-probe microscopy that keep the beam intensity constant and instead…
The linear and nonlinear dynamical susceptibilities of a two level system are calculated as it undergoes a transition to a decoherent state. Analogously to the Glover-Tinkham-Ferrell sum rule of superconductivity, spectral weight in the…
Accurate knowledge of absorption coefficient of a sample is a prerequisite for measuring the third order optical nonlinearity of materials, which could become a serious limitation for unknown samples. We introduce a new method, which…
A general non-linear response theory is derived for an arbitrary time-dependent Hamiltonian, not necessarily obeying time-reversal symmetry. This allows us to obtain a greatly generalized Kubo type formula. Applied to a mesoscopic system…
While nonlinear optical spectroscopy is becoming more commonly used to study the excited states of nonlinear-optical systems, a general theory of inhomogeneous broadening is rarely applied in lieu of either a simple Lorentzian or Gaussian…
The optical conductivity is the basic defining property of materials characterizing the current response toward time-dependent electric fields. In this work, following the approach of Kubo's response theory, we study the general properties…
Using matrix product state techniques we study the nonequilibrium dynamical response of the half-filled Hubbard ladder when subject to an optical pump. Optical pumping offers a way of producing and manipulating new strongly correlated…
The Kramers-Kronig relations and various oscillator strength sum rules represent strong constraints on the physical response of materials. In this work, taking inspiration from the well-established equivalence between $f-$sum rules and…
Stable limit cycle as a stabilized mechanical oscillation is the primary result of the dynamical evolution of an optomechanical system under sufficiently powerful pump. Because this dynamical process is highly nonlinear, it was not clear…
Upon excitation by a laser pulse, broken-symmetry phases of a wide variety of solids demonstrate similar order parameter dynamics characterized by a dramatic slowing down of relaxation for stronger pump fluences. Motivated by this recurrent…
It is explicitly shown, for optical processes arbitrarily comprising two-, three- or four-photon interactions, that the sum over all matter states of any optical susceptibility is exactly zero. The result remains true even in frequency…
Nonlinear effects are crucial in order to compute the cosmological matter power spectrum to the accuracy required by future generation surveys. Here, a new approach is presented, in which the power spectrum, the bispectrum and higher order…