相关论文: How harmonic is dipole resonance of metal clusters…
Multipole electric and magnetic giant resonances in metal clusters are reviewed and compared with their counterparts in atomic nuclei. The main attention is paid to E1 resonance (dipole plasmon).
We derive large-amplitude collective equations of motion from the variational principle for the time-dependent Schroedinger equation. These equations reduce to the well-known diabatic formulas for vibrational frequencies in the small…
The periods of the harmonic oscillations of the ion core of charged sodium clusters around the equilibrium shapes are considered. It is found that these periods are of the order of magnitude of the experimentally measured relaxation times…
Multipolar plasmon oscillation frequencies and corresponding damping rates for nanospheres formed of the simplest free-electron metals are studied. The possibility of controlling plasmon features by choosing the size and dielectric…
We study the effect of the electromagnetic environment on the resonance frequency of plasmonic excitations in dimers of interacting metallic nanoparticles. The coupling between plasmons and vacuum electromagnetic fluctuations induces a…
In this paper, we investigate the hybridization theory of plasmon resonance in metallic nanostructures, which has been validated by the authors in [31] through a series of experiments. In an electrostatic field, we establish a mathematical…
We develop a theoretical framework, based on a multipole, quasi-static approach, for the prediction of the localized surface plasmon resonances in Fanoshells formed via geometrical symmetry-breaking in multilayer nanoshells consisting of a…
A systematic microscopic study of the anharmonic properties of the double giant dipole resonance (DGDR) has been carried out, for the first time, for nuclei with mass number $A$ spanning the whole mass table. It is concluded that the…
The idea of utilizing the second-order plasmon resonance of the gold nanorod {\pi}-dimers for plasmon rulers is introduced. We report on a qualitatively different dependence of the plasmon resonance shift on the interparticle distance for…
The role of anharmonic effects on the excitation of the double giant dipole resonance is investigated in a simple macroscopic model.Perturbation theory is used to find energies and wave functions of the anharmonic ascillator.The cross…
Theoretical description of oscillations of electron liquid in large metallic nanospheres (with radius of few tens nm) is formulated within random-phase-approximation semiclassical scheme. Spectrum of plasmons is determined including both…
We investigate the influence of morphology and size on the vibrational properties of disordered clusters of colloidal particles with attractive interactions. From measurements of displacement correlations between particles in each cluster,…
We have developed a microscopic theory on phonon energy dispersion in chiral crystals within a harmonic approximation. One of the main issues is about the splitting of sound velocity of acoustic phonons with opposite ``crystal'' angular…
A nonperturbative theory of multiphonon anharmonic transitions between energy levels of a local mode is presented. It is shown that the rate of transitions rearranges near the critical level number $n_{cr}$: at smaller $n$ the process slows…
We investigate the effect of anharmonicity on the one-dimensional half-filled Holstein model by using the determinant quantum Monte Carlo method. By calculating the order parameters we find that with and without anharmonicity there is…
Material losses in metals are a central bottleneck in plasmonics for many applications. Here we propose and theoretically demonstrate that metal losses can be successfully mitigated with dielectric particles on metallic films, giving rise…
Two possible mechanisms of surface plasmon (SP) oscillations damping in metallic nanoparticles (MNPs), not connected with electron-phonon interaction are investigated theoretically: a) the radiation damping of SP, b) resonant coupling of SP…
We show that second harmonic generation can be enhanced by Fano resonant coupling of asymmetric plasmonic metal nanostructures. We develop a theoretical model examining the effects of electromagnetic interaction between two metal…
We study the linewidth of the surface plasmon resonance in the optical absorption spectrum of metallic nanoparticles, when the decay into electron-hole pairs is the dominant channel. Within a semiclassical approach, we find that the…
Two phonon-states of alkali-metal clusters (treated as jellium spheres) are calculated by using a method based on a perturbative construction of periodic orbits of the time-dependent mean-field equations. Collective vibrations with various…