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In time-resolved pump-probe vibrational spectroscopy the internal stretch mode of polar molecules is utilized as a key observable to characterize the ultrafast dynamics of adsorbates on surfaces. The adsorbates non-adiabatic intermode…

材料科学 · 物理学 2023-03-13 Raúl Bombín , Alberto S. Muzas , Dino Novko , J. Iñaki Juaristi , Maite Alducin

In the present work, we give an analytical non-perturbative treatment of mode-mode coupling and anharmonicity occurring in molecular vibrational systems analyzed by 2D-infrared spectroscopy. This analytical description allows a detailed…

化学物理 · 物理学 2013-09-04 Kuo Kan Liang , Albert A. Villaeys

Precise molecular transition frequencies are of great interest in the test of fundamental physics and also in various applications. Two well isolated ro-vibrational transitions of $^{12}$C$^{16}$O at 1.57 $\mu$m, R(9) and R(10) in the…

原子物理 · 物理学 2017-10-11 Jin Wang , Yu R. Sun , Lei-Gang Tao , An-Wen Liu , Shui-Ming Hu

The stretching and bending vibrations of methane are studied in the framework of a symmetry-adapted algebraic model. The model is based on the realization of the one-dimensional Morse potential in terms of a $U(2)$ algebra. For the 44…

化学物理 · 物理学 2017-11-03 R. Lemus , F. Perez-Bernal , A. Frank , R. Bijker , J. M. Arias

Double-$\gamma$ vibrations in deformed nuclei are studied in the context of the interacting boson model with special reference to their anharmonic character. It is shown that large anharmonicities can be obtained with interactions that are…

核理论 · 物理学 2009-10-31 J. E. Garcia-Ramos , C. E. Alonso , J. M. Arias , P. Van Isacker

Recent experimental observations of time-dependent beatings in the two-dimensional echo-spectra of light-harvesting complexes at ambient temperatures have opened up the question whether coherence and wave-like behaviour plays a significant…

生物物理 · 物理学 2012-02-08 Birgit Hein , Christoph Kreisbeck , Tobias Kramer , Mirta Rodríguez

Motivated by recent developments in the experimental study of Bose-Fermi mixtures, we investigate ground-state phase diagrams and excitation spectra for Bose-Fermi mixtures in a three-dimensional (3D) optical lattice. The Gutzwiller…

量子气体 · 物理学 2020-02-19 Rei Hatsuda , Emiko Arahata

We investigate many-body phase diagrams of atomic boson-fermion mixtures loaded in the two-dimensional optical lattice. Bosons mediate an attractive, finite-range interaction between fermions, leading to fermion pairing phases of different…

超导电性 · 物理学 2007-05-23 D. -W. Wang , M. D. Lukin , E. Demler

Terahertz molecular motions are often probed by high-frequency molecular oscillators in different types of non-linear vibrational spectroscopy. Recently developed two-dimensional terahertz-infrared-visible spectroscopy allows direct…

化学物理 · 物理学 2023-04-19 Pankaj Seliya , Mischa Bonn , Maksim Grechko

We study the charge-density dynamics within the two-dimensional extended Hubbard model in the presence of long-range Coulomb interaction across the metal-insulator transition point. To take into account strong correlations we start from…

强关联电子 · 物理学 2014-12-24 E. G. C. P. van Loon , H. Hafermann , A. I. Lichtenstein , A. N. Rubtsov , M. I. Katsnelson

Results are presented for the time evolution of fermions initially in a non-zero temperature normal phase, following the switch on of an attractive interaction. The dynamics are studied in the disordered phase close to the critical point,…

超导电性 · 物理学 2017-09-20 Yonah Lemonik , Aditi Mitra

After a prologue which clarifies some issues left open in my last paper, the main features of the tetron model of elementary particles are discussed in the light of recent developments, in particular the formation of strong and electroweak…

高能物理 - 唯象学 · 物理学 2014-11-18 Bodo Lampe

Interactions between electrons and lattice vibrations are responsible for a wide range of material properties and applications. Recently, there has been considerable interest in the development of resonant inelastic x-ray scattering (RIXS)…

Interacting Bose-Fermi mixtures possess a fermionic (super)symmetry when bosons and fermions in the mixture have equal masses, and when the interaction strengths are appropriately tuned. This symmetry is spontaneously broken in the ground…

量子气体 · 物理学 2016-03-30 Barry Bradlyn , Andrey Gromov

Observed optical reflectivity in the infrared spectral region is compared with theoretical predictions in a strongly coupled electron-phonon system. Starting from a Froehlich Hamiltonian, the spectral functions and their temperature…

超导电性 · 物理学 2007-05-23 H. J. Kaufmann , E. G. Maksimov , E. K. H. Salje

Vibronic spectra of molecules are typically described within the Franck-Condon model. Here, we show that highly resolved vibronic spectra of large organic molecules on a single layer of MoS$_{2}$ on Au(111) show spatial variations in their…

介观与纳米尺度物理 · 物理学 2020-03-24 Gaël Reecht , Nils Krane , Christian Lotze , Lei Zhang , Alejandro L. Briseno , Katharina J. Franke

The multimode Brownian model with nonlinear system-bath coupling offers a flexible framework for studying both intra- and intermolecular vibrational modes in condensed-phase molecular systems. This approach allows us to calculate linear and…

化学物理 · 物理学 2025-12-30 Ryotaro Hoshino , Yoshitaka Tanimura

Conclusive experimental evidence of a supersolid phase in any known condensed matter system is presently lacking. On the other hand, a supersolid phase has been recently predicted for a system of spinless bosons in continuous space,…

量子气体 · 物理学 2012-04-27 Sebastiano Saccani , Saverio Moroni , Massimo Boninsegni

We investigate trapped resonant fermions with unequal populations within the local density approximation above the superfluid transition temperature. By tuning the attractive interaction between fermions via Feshbach resonance, the system…

超导电性 · 物理学 2007-05-23 Chi-Ho Cheng , Sung-Kit Yip

The Boson-Fermion model, describing a mixture of tightly bound electron pairs and quasi-free electrons hybridized with each other via a charge exchange term, is studied in the limit of infinite dimensions, using the Non-Crossing…

超导电性 · 物理学 2009-10-31 J. -M. Robin , A. Romano , J. Ranninger