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Frequency-stabilized mid-infrared lasers are valuable tools for precision molecular spectroscopy. However, their implementation remains limited by complicated stabilization schemes. Here we achieve optical self-locking of a quantum cascade…

光学 · 物理学 2021-06-29 Gang Zhao , Jianfei Tian , Joseph T. Hodges , Adam J. Fleisher

We report shifting of the frequency of an 850 nm laser with an instantaneous bandwidth of (350-1650), MHz and an efficiency between 35% (minimum) to 80% (best at frequencies around 600 and 1500, MHz) by phase modulation with a sawtooth…

光学 · 物理学 2009-10-10 Rachel Houtz , Cheong Chan , Holger Mueller

We report the development of a new instrument for cavity-enhanced absorption spectroscopy of the fundamental rovibrational transitions of molecules in the long-wave mid-infrared (LWIR) region from 6500 to 10000 nm. Our setup combines a LWIR…

Spatial resolution of most imaging devices is fundamentally restricted by diffraction. This limitation is manifested in the loss of high spatial frequency information contained in evanescent waves. As a result, conventional far-field optics…

光学 · 物理学 2010-03-16 Leonid Alekseyev , Evgenii Narimanov , Jacob Khurgin

Phase noise or frequency noise is a key metrics to evaluate the short term stability of a laser. This property is of a great interest for the applications but delicate to characterize, especially for narrow line-width lasers. In this…

We present an ultrafast fiber laser system delivering 4.6 W average power at 258 nm based on two-stage fourth-harmonic generation in beta barium borate (BBO). The beam quality is close to diffraction limited with an M2- value of 1.3 x 1.6.…

We combine a tunable continuous-wave optical parametric oscillator and a femtosecond Ti:Sapphire laser frequency comb to provide a phase-coherent bridge between the visible and mid-infrared spectral ranges. As a first demonstration of this…

光学 · 物理学 2009-11-11 Evgeny Kovalchuk , Thilo Schuldt , Achim Peters

Single-shot ultrafast absorbance spectroscopy based on the frequency encoding of the kinetics is analyzed theoretically and implemented experimentally. In Part II of the series, arbitrary thickness sample is analysed theroretically. The…

We demonstrate a remarkably effective single-stage compression technique for ultrafast pulses in the visible electromagnetic spectrum using second-harmonic pulses at 515 nmderived from a 1030 nm Yb-based femtosecond regenerative amplifier.…

We present high spectral resolution (~3 km/s) observations of the nu_2 ro-vibrational band of H2O in the 6.086--6.135 micron range toward the massive protostar AFGL 2591 using the Echelon-Cross-Echelle Spectrograph (EXES) on the…

Femtosecond carrier recombination in PbI2 is measured using tabletop high-harmonic extreme ultraviolet (XUV) transient absorption spectroscopy and ultrafast electron diffraction. XUV absorption from 45 eV to 62 eV measures transitions from…

We report an approach for high-resolution spectroscopy using a widely tunable laser emitting in the molecular fingerprint region. The laser is based on difference-frequency generation (DFG) in a nonlinear orientation-patterned GaAs crystal.…

The motion of electrons in or near solids, liquids and gases can be tracked by forcing their ejection with attosecond x-ray pulses, derived from femtosecond lasers. The momentum of these emitted electrons carries the imprint of the…

介观与纳米尺度物理 · 物理学 2017-06-14 C. W. Barlow-Myers , N. J. Pine , W. A. Bryan

We present a modified approach to laser optical-feedback cavity-enhanced absorption spectroscopy. The technique involves continuously scanning the length of a high-finesse cavity to periodically lock a diode laser to the cavity resonance,…

光学 · 物理学 2024-09-04 Christopher A. Curwen , Mathieu Fradet , Ryan M. Briggs

Photoacoustic imaging can achieve high-resolution three-dimensional visualization of optical absorbers at penetration depths ~ 1 cm in biological tissues by detecting optically-induced high ultrasound frequencies. Tomographic acquisition…

光学 · 物理学 2015-05-15 Jérôme Gateau , Marc Gesnik , Jean-Marie Chassot , Emmanuel Bossy

We have used injection locking to multiply the repetition rate of a passively mode-locked femtosecond fiber laser from 40 MHz to 1 GHz while preserving optical phase coherence between the master laser and the slave output. The system is…

光学 · 物理学 2015-06-03 D. Kielpinski , O. Gat

We measure molecular vibrations with femtometer precision using time-resolved x-ray absorption spectroscopy. For a demonstration, a Raman process excites the A$_{1g}$ mode in gas-phase SF$_6$ molecules with an amplitude of $\approx50$ fm,…

The serrodyne principle enables shifting the frequency of an electromagnetic signal by applying a linear phase ramp in the time domain [1]. This phenomenon has been exploited to frequency-shift signals in the radiofrequency (RF), microwave…

We demonstrate Faraday spectroscopy with high duty cycle and sampling rate using atoms confined to a blue-detuned optical trap. Our trap consists of a crossed pair of high-charge-number hollow laser beams, which forms a dark, box-like…

量子物理 · 物理学 2009-11-13 Matthew L. Terraciano , Mark Bashkansky , Fredrik Fatemi

When optically excited, iodine absorbs in the 490- to 650-nm visible region of the spectrum and, after radiative relaxation, it displays an emission spectrum of discrete vibrational bands at moderate resolution. This makes laser-induced…

物理教育 · 物理学 2015-07-10 S. B. Bayram , M. V. Freamat