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The spectral dynamics of a mid-infrared multimode Cr^2+:ZnSe laser located in a vacuum sealed chamber containing acetylene at low pressure is analyzed by a stepping-mode high-resolution time-resolved Fourier transform interferometer.…

Supercontinua generated in highly non-linear fibers by ultrashort-pulse lasers can be used for high resolution Fourier transform absorption spectroscopy. The practical advantages of these bright ultrabroadband light sources for spectroscopy…

Spectra comprised of hundreds of time-components for absorption path lengths up to 130 km have been recorded around 1050 nm by combining two recent techniques, intracavity laser spectroscopy with vertical external cavity surface emitting…

光学 · 物理学 2009-11-13 Nathalie Picqué , Guy Guelachvili , Alexander A. Kachanov

Optical frequency-comb-based-high-resolution spectrometers offer enormous potential for spectroscopic applications. Although various implementations have been demonstrated, the lack of suitable mid-infrared comb sources has impeded…

An ultrashort-pulse Cr^{2+}:ZnSe laser is a novel broadband source for sensitive high resolution molecular spectroscopy. A 130-fs pulse allows covering of up to 380 cm^-1 spectral domain around 2.4 $\mu$m which is analyzed simultaneously…

Intracavity laser absorption spectroscopy (ICLAS) with an evacuated Cr2+: ZnSe laser is performed with a high-resolution time-resolved Fourier transform interferometer with a minimum detectable absorption coefficient equal to 4 10-9 cm-1…

We perform femtosecond frequency comb vernier spectroscopy in the near infrared with a femtosecond Er doped fiber laser, a scanning high-finesse cavity and an InGaAs camera. By utilizing the properties of a frequency comb and a scanning…

We present a system for molecular spectroscopy using a broadband mid-infrared laser with near infrared detection. Difference frequency generation of a Yb:fiber femtosecond laser produced a mid-infrared (MIR) source tunable from 2100-3700…

光学 · 物理学 2015-05-30 Todd A. Johnson , Scott A. Diddams

Improving spectral acquisition rate of broadband mid-infrared spectroscopy promises further advancements of molecular science and technology. Unlike the pump-probe spectroscopy that requires repeated measurements with different pump-probe…

In this paper, the photoacoustic spectroscopy technique based on lithium niobate crystals is initially reported, to our knowledge. A novel dual-cantilever tuning fork structure and new electrodes have been designed using Y-cut 128{\deg}…

应用物理 · 物理学 2023-12-20 Haoyang Lin , Wenguo Zhu , Yongchun Zhong , Jieyuan Tang , Huihui Lu , Jianhui Yu , Huadan Zheng

We developed a novel technique for frequency measurement and synthesis, based on the operation of a femtosecond comb generator as transfer oscillator. The technique can be used to measure frequency ratios of any optical signals throughout…

光学 · 物理学 2009-11-07 Jörn Stenger , Harald Schnatz , Christian Tamm , Harald R. Telle

We demonstrate a new simple technique to measure IR frequencies near 30 THz using a femtosecond (fs) laser optical comb and sum-frequency generation. The optical frequency is directly compared to the distance between two modes of the fs…

A novel mid-infrared/near-infrared double resonant absorption setup for studying infrared-inactive vibrational states is presented. A strong vibrational transition in the mid-infrared region is excited using an idler beam from a singly…

化学物理 · 物理学 2016-07-21 J. Karhu , J. Nauta , M. Vainio , M. Metsälä , S. Hoekstra , L. Halonen

X-ray absorption spectroscopy (XAS) is a powerful and well established technique with sensitivity to elemental and chemical composition. Despite these advantages, its implementation has not kept pace with the development of ultrafast pulsed…

The first comprehensive high-resolution photoabsorption spectrum of 14N15N has been recorded using the Fourier-transform spectrometer attached to the Desirs beamline at the Soleil synchrotron. Observations are made in the extreme…

原子与分子团簇 · 物理学 2012-01-25 A. N. Heays , G. D. Dickenson , E. J. Salumbides , N. de Oliveira , D. Joyeux , L. Nahon , B. R. Lewis , W. Ubachs

Several ways to electronically synchronize different types of amplified femtosecond laser systems are presented, based on a single freely programmable electronics hardware: Arbitrary-detuning asynchronous optical sampling, as well as…

光学 · 物理学 2023-07-06 Jan Helbing , Peter Hamm

High-resolution absorption spectra of \NH\ in the region 2100 - 5500 \cm\ at 1027 $^{\circ}$C and atmospheric pressure (1045 $\pm$ 3 mbar) are measured. An \NH\ concentration of 10\% in volume fraction is used in the measurements. Spectra…

Time-resolved femtosecond stimulated Raman spectroscopy (FSRS) is a powerful tool for investigating ultrafast structural and vibrational dynamics in light absorbing systems. However, the technique generally requires exposing a sample to…

仪器与探测器 · 物理学 2018-07-10 Matthew N. Ashner , William A. Tisdale

A room temperature operating Vertical External Cavity Surface Emitting Laser is applied around 1550 nm to intracavity laser absorption spectroscopy analyzed by time-resolved Fourier transform interferometry. At an equivalent pathlength of…

A source of ultrashort pulses of light in the 2 {\mu}m region was constructed using supercontinuum broadening from an erbium mode-locked laser. The output spectrum spanned 1000 nm to 2200 nm with an average power of 250 mW. A pulse width of…

光学 · 物理学 2017-07-26 Andrew Klose , Gabriel Ycas , Daniel L. Maser , Scott A. Diddams
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