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Using the stabilized jellium model in two schemes of `relaxed' and `rigid', we have calculated the dissociation energies and the fission barrier heights for the binary fragmentations of singly-ionized and doubly-ionized Ag clusters. In the…

材料科学 · 物理学 2009-11-10 M. Payami

We construct a meta-generalized-gradient approximation which properly balances the nonlocality contributions to the exchange and correlation at the semilocal level. This non-empirical functional shows good accuracy for a broad palette of…

化学物理 · 物理学 2013-05-17 L. A. Constantin , E. Fabiano , F. Della Sala

The theoretical formalism of the local density approximation (LDA) to density functional theory (DFT) has been used to study the electronic and geometric structures of SimCn (1<=m, n<=4;n<=m) clusters. An all electron 6-311++G** basis set…

原子与分子团簇 · 物理学 2007-05-23 Prachi Pradhan , Asok K. Ray

Laboratory experiments and particle-resolved simulations are employed to investigate the settling dynamics of a pair of rigidly connected spherical particles of unequal size. They yield a detailed picture of the transient evolution and the…

流体动力学 · 物理学 2024-06-18 Zachary Maches , Morgane Houssais , Alban Sauret , Eckart Meiburg

We study static, spherically symmetric, self-gravitating systems minimally coupled to a scalar field with U(1) gauge symmetry: charged boson stars. We find numerical solutions to the EinsteinMaxwell equations coupled to the relativistic…

高能天体物理现象 · 物理学 2013-08-05 Daniela Pugliese , Hernando Quevedo , Jorge A. Rueda H. , Remo Ruffini

We prove a threshold-sharp stability theory for the conformal scalar-curvature sector on zero-curvature Carter backgrounds. The main result is a fully closed bounded-slab theorem: the reflecting evolution is constructed, the conserved…

偏微分方程分析 · 数学 2026-05-19 Bobby Eka Gunara

The macroscopic properties of compact stars in modified gravity theories can be significantly different from the general relativistic (GR) predictions. Within the gravitational context of scalar-tensor theories, with a scalar field $\phi$…

广义相对论与量子宇宙学 · 物理学 2023-12-05 Juan M. Z. Pretel , Sergio E. Jorás , Ribamar R. R. Reis , Sergio B. Duarte , José D. V. Arbañil

Recently, we have demonstrated that the problems finding a suitable adiabatic approximation in time-dependent one-body reduced density matrix functional theory can be remedied by introducing an additional degree of freedom to describe the…

化学物理 · 物理学 2014-03-10 Klaas J. H. Giesbertz , Oleg V. Gritsenko , Evert Jan Baerends

By using the quantum Ising chain as a test bed and treating the spin polarization along the external transverse field as the "generalized density", we examine the performance of different levels of density functional approximations parallel…

计算物理 · 物理学 2021-10-27 Jiahao Mao , Haifeng Tang , Wenhui Duan , Zheng Liu

Using first-principles density functional theory based calculations, we analyze the structural stability of small clusters of 3$d$ late transition metals. We consider the relative stability of the two structures - layer-like structure with…

介观与纳米尺度物理 · 物理学 2011-08-15 Soumendu Datta , Mukul Kabir , Tanusri Saha-Dasgupta

The effective response depends sensitively on composite microstructure due to large fluctuations in the local electric field. For metallic clusters embedded in a dielectric host, the local field distributions are extremely inhomogeneous in…

软凝聚态物质 · 物理学 2007-05-23 Ying Gu , K. W. Yu , Hong Sun

In this work, we have used the exchange-only optimized effective potential in the self-consistent calculations of the density functional Kohn-Sham equations for simple metal clusters in stabilized jellium model with self-compression. The…

原子与分子团簇 · 物理学 2009-11-11 M. Payami

We determine the structure and melting behavior of supported metallic clusters using an ab initio density-functional-based treatment of intracluster interactions and an approximate treatment of the surface as an idealized smooth plane…

介观与纳米尺度物理 · 物理学 2012-10-02 S. A. Blundell , Soumyajyoti Haldar , D. G. Kanhere

Previously, the authors reported direct evidence of channel saturation and conductance quantization in atomic-sized gold constrictions through mechanical perturbation studies, and also showed that peaks in conductance histograms are…

介观与纳米尺度物理 · 物理学 2011-04-07 Jason N. Armstrong , Susan Z. Hua , Harsh Deep Chopra

We have calculated the absorption characteristics of different hybrid systems consisting of Ag, Ag2 or Ag3 atomic clusters and poly(methacrylic acid) (PMAA) using the time-dependent density-functional theory. The polymer is found to have an…

材料科学 · 物理学 2015-05-18 Laura Koponen , Lasse O. Tunturivuori , Martti J. Puska , Y. Hancock

The Ionization Potentials of small Li_N clusters are calculated with a Shell Correction Method. They are used to illustrate that, within the jellium approximation, deformed cluster shapes provide an adequate description of the observed…

原子与分子团簇 · 物理学 2009-10-31 Constantine Yannouleas , Uzi Landman

We present a comparative study of metal-organic interface properties obtained from dispersion corrected density functional theory calculations based on two different approaches: the periodic slab supercell technique and cluster models with…

The strong-coupling perturbation theory (SCPT) for correlated electron systems is extended to the case of full Coulomb interaction. The Coulomb mechanism of the orbital polarization is discussed and attention is paid to the importance of…

强关联电子 · 物理学 2007-05-23 I. Sandalov , U. Lundin , O. Eriksson

The static electric dipole polarizability of $\mathrm{Na_N}$ clusters with even N has been calculated in a collective, axially averaged and a three-dimensional, finite-field approach for $2\le N \le 20$, including the ionic structure of the…

原子与分子团簇 · 物理学 2009-10-31 S. Kümmel , T. Berkus , P. -G. Reinhard , M. Brack

Topologically stable structures include vortices in a wide variety of matter, such as skyrmions in ferro- and antiferromagnets, and hedgehog point defects in liquid crystals and ferromagnets. These are characterized by integer-valued…