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We present quantitative results for the drift velocity of a polymer in a gel if a force (e.g. through an electric or magnetic field) acts on a tag, attached to one of its ends. This is done by introducing a modification of the…

凝聚态物理 · 物理学 2009-10-28 G. T. Barkema , G. M. Schütz

We investigate the translocation of rods with different charge distributions using hybrid Langevin Dynamics and Lattice Boltzmann (LD-LB) simulations. Electrostatic interactions are added to the system using the $P^3M$ algorithm to model…

软凝聚态物质 · 物理学 2022-05-24 Le Qiao , Gary W. Slater

Confinement strongly influences electrochemical systems, where structural control has enabled advances in nanofluidics, sensing, and energy storage. In electric double-layer capacitors (EDLCs), or supercapacitors, energy density is governed…

化学物理 · 物理学 2026-01-30 Bryce Rives , Filipe Henrique , Pawel Zuk , Ankur Gupta

We develop a diffuse-interface continuum model for membrane electroporation that couples a phase field for pore geometry to a quasi-static electrolyte potential and a spatially varying leaky-dielectric model for the transmembrane voltage.…

软凝聚态物质 · 物理学 2026-02-10 Saman Seifi , David Salac

Tunable nanopores in elastomeric membranes have been used to study the dependence of ionic current blockade rate on the concentration and electrophoretic mobility of particles in aqueous suspensions. A range of nanoparticle sizes, materials…

软凝聚态物质 · 物理学 2010-05-25 G R Willmott , R Vogel , S S C Yu , L G Groenewegen , G S Roberts , D Kozak , W Anderson , M Trau

Molecular dynamics simulation is utilized to investigate the ionic transport of NaCl in solution through a graphene nanopore under an applied electric field. Results show the formation of concentration polarization layers in the vicinity of…

生物物理 · 物理学 2013-01-10 Guohui Hu , Mao Mao , Sandip Ghosal

Coarse-grained simulations are often employed to study the translocation of DNA through a nanopore. The majority of these studies investigate the translocation process in a relatively generic sense and do not endeavour to match any…

软凝聚态物质 · 物理学 2015-03-05 Hendrick W. de Haan , David Sean , Gary W. Slater

Using Langevin dynamics simulations, we investigate the dynamics of polymer translocation into a circular nanocontainer through a nanopore under a driving force $F$. We observe that the translocation probability initially increases and then…

软凝聚态物质 · 物理学 2012-12-06 Kehong Zhang , Kaifu Luo

The translocation time of a polymer chain through an interaction energy gradient nanopore was studied by Monte Carlo simulations and the Fokker-Planck equation with double-absorbing boundary conditions. Both the simulation and calculation…

软凝聚态物质 · 物理学 2017-01-04 Meng-Bo Luo , Shuang Zhang , Fan Wu , Li-Zhen Sun

The transport of polyelectrolytes confined by oppositely charged surfaces and driven by a constant electric field is of interest in studies of DNA separation according to size. Using molecular dynamics simulations that include surface…

软凝聚态物质 · 物理学 2020-09-15 Debarshee Bagchi , Monica Olvera de la Cruz

Run-and-tumble motility is widely used by swimming microorganisms including numerous prokaryotic eukaryotic organisms. Here, we experimentally investigate the run-and-tumble dynamics of the bacterium E. coli in polymeric solutions. We find…

流体动力学 · 物理学 2015-11-04 A. E. Patteson , A. Gopinath , M. Goulian , P. E. Arratia

We study the mean velocity and diffusion constant in three related models of molecular Brownian ratchets. Brownian ratchets can be used to describe translocation of biopolymers like DNA through nanopores in cells in the presence of…

统计力学 · 物理学 2018-08-08 Matthias Uhl , Udo Seifert

Dynamic processes in dispersions of charged spherical particles are of importance both in fundamental science, and in technical and bio-medical applications. There exists a large variety of charged-particles systems, ranging from…

软凝聚态物质 · 物理学 2013-11-25 G. Nägele , M. Heinen , A. J. Banchio , C. Contreras-Aburto

Nanoporosity in silicon results in an interface-dominated mechanics, fluidics and photonics that are often superior to the ones of the bulk material. However, their active control, e.g. as a response to electronic stimuli, is challenging…

材料科学 · 物理学 2022-11-29 Manuel Brinker , Patrick Huber

Water electrolysis in a microsystem is observed and analyzed on a short-time scale ~10 us. Very unusual properties of the process are stressed. An extremely high current density is observed because the process is not limited by the…

软凝聚态物质 · 物理学 2013-07-18 Vitaly B. Svetovoy , Remco G. P. Sanders , Miko C. Elwenspoek

Analyte translocation involves three phases: (i) diffusion in the loading solution; (ii) capture by the pore; (iii) threading. The capture process remains poorly characterized because it cannot easily be visualized or inferred from indirect…

生物物理 · 物理学 2020-08-10 Le Qiao , Maxime Ignacio , Gary W. Slater

We propose a numerical method to simulate electrohydrodynamic phenomena in charged colloidal dispersions. This method enables us to compute the time evolutions of colloidal particles, ions, and host fluids simultaneously by solving Newton,…

软凝聚态物质 · 物理学 2007-05-23 Kang Kim , Yasuya Nakayama , Ryoichi Yamamoto

The velocity of polaron migration in the long poly-DNA chain (~40 base pairs) in an applied electric field has been studied within a polaron model. We found that the polaron velocity strongly depends on the polaron size. A small polaron…

软凝聚态物质 · 物理学 2007-09-11 Julia A. Berashevich , Adam D. Bookatz , Tapash Chakraborty

We present a numerical study of forced polymer translocation by using two separate pore models. Both of them have been extensively used in previous forced translocation studies. We show that variations in the pore model affect the forced…

生物物理 · 物理学 2015-05-19 V. V. Lehtola , K. Kaski , R. P. Linna

The locomotion of swimming bacteria in simple Newtonian fluids can successfully be described within the framework of low Reynolds number hydrodynamics. The presence of polymers in biofluids generally increases the viscosity, which is…

软凝聚态物质 · 物理学 2019-08-12 Andreas Zöttl , Julia M. Yeomans