相关论文: Ultrafast Dynamics for Electron Photodetachment fr…
Understanding the nature of solvated electrons is important in studying a range of chemical and biological phenomena. This study investigates the structural and dynamical behavior of an excess electron in water, examining different…
Optimising the photoelectrochemical performance of hematite photoanodes for solar water splitting requires better understanding of the relationships between dopant distribution, structural defects and photoelectrochemical properties. Here,…
Data for inelastic processes due to hydrogen atom collisions with manganese and titanium are needed for accurate modeling of the corresponding spectra in late-type stars. In this work excitation and charge transfer in low-energy Mn+H and…
Electrolyte decomposition reactions on Li-ion battery electrodes contribute to the formation of solid electrolyte interphase (SEI) layers. These SEI layers are one of the known causes for the loss in battery voltage and capacity over…
Ultrafast laser ablation is an extremely precise and clean method of removing material, applied in material processing as well as medical applications. And due to its violent nature, it tests our understanding of the interplay between…
Gas phase ultrafast electron diffraction (GUED) has become a powerful technique to directly observe the structural dynamics of photoexcited molecules. GUED reveals information about the nuclear motions that is complementary to the…
The advent of powerful laser sources has made it possible to observe a relatively large cross section of the excited state of Hydrogen atom. This is due to the effect of joint collisions of a linearly polarized $N$-photon and high-energy…
To undergo diffusive shock acceleration, electrons need to be pre-accelerated to increase their energies by several orders of magnitude, else their gyro-radii are smaller than the finite width of the shock. In oblique shocks, where the…
Ultrafast photocurrent measurements are performed on individual carbon nanotube PN junction photodiodes. The photocurrent response to sub-picosecond pulses separated by a variable time delay {\Delta}t shows strong photocurrent suppression…
The dynamics of the electron impact multiphoton ionization of a hydrogen atom in the presence of an intense laser field has been studied theoretically, with a view to comparing (qualitatively) the results with the recent kinematically…
The dipole strength of the nuclide $^{76}$Ge was studied in photon-scattering experiments using bremsstrahlung produced with electron beams of energies of 7.8 and 12.3 MeV at the $\gamma$ELBE facility. We identified 210 levels up to an…
An excitonic insulator phase is expected to arise from the spontaneous formation of electron-hole pairs (excitons) in semiconductors where the exciton binding energy exceeds the size of the electronic band gap. At low temperature, these…
The evolution of charge carriers in photoexcited room temperature ZnO nanoparticles in solution is investigated using ultrafast ultraviolet photoluminescence spectroscopy, ultrafast Zn K-edge absorption spectroscopy and ab-initio molecular…
The design of better heterogeneous catalysts for applications such as fuel cells and electrolyzers requires a mechanistic understanding of electrocatalytic reactions and the dependence of their activity on operating conditions such as pH. A…
The photoelectric effect established by Einstein is well known, which indicates that electrons on lower energy levels can jump up to higher levels by absorbing photons, or jump down from higher levels to lower levels and give out…
Using the photon-ion merged-beams technique at the PETRA\,III synchrotron light source, we have measured cross sections for double and up to tenfold photoionization of La$^{+}$ ions by a single photon in the energy range 820--1400~eV, where…
The solvation structure of protons in aqueous media is highly relevant to electric properties and to proton transport in liquids and membranes. At ambient temperature, polar liquids display structural fluctuations on femto- to picosecond…
Using molecular dynamics simulations, we reveal emergent properties of hydrated electrode interfaces that while molecular in origin are integral to the behavior of the system across long times scales and large length scales. Specifically,…
We present ab initio studies of photoelectron spectra for above threshold detachment (ATD) of F$^-$ anions in short, 1300 nm and 1800 nm laser pulses. We identify and assess the importance of electron rescattering in strong-field…
Discharge and electron-impact excitation lead to the production of metastable helium atoms in two metastable states, 2$^1$S$_0$ and 2$^3$S$_1$. However, many applications require pure beams of one of these species or at least a detailed…