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Single-shot ultrafast absorbance spectroscopy based on the frequency encoding of the kinetics is analyzed theoretically and implemented experimentally. The kinetics are sampled in the frequency domain using linearly chirped, amplified 33 fs…

"Single-shot" ultrafast spectroscopy based on the frequency encoding of transient absorbance kinetics using chirped probe pulses is analyzed theoretically. FDSS has an advantage over pump-probe spectroscopy in a situation where the "noise"…

光学 · 物理学 2007-05-23 Ilya A. Shkrob , Stanislas Pommeret

Single-shot ultrafast spectroscopy based on the frequency encoding of transient absorbance kinetics (FDSS) is demonstrated. These kinetics are sampled spectrally using linearly chirped pulses derived from a Ti:sapphire laser. A variable…

光学 · 物理学 2007-05-23 Ilya A. Shkrob , Dmitri A. Oulianov , Robert A. Crowell

A new method, FM-FTS, combining Frequency Modulation heterodyne laser spectroscopy and Fourier Transform Spectroscopy is presented. It provides simultaneous sensitive measurement of absorption and dispersion profiles with broadband spectral…

光学 · 物理学 2007-09-24 Julien Mandon , Guy Guelachvili , Nathalie Picqué

Ultrafast single-shot imaging techniques now reach frame rates of tens of tera-frame-per-second (Tfps) and long sequence depths but are often too complex for large-scale use, both in terms of image acquisition and reconstruction. We propose…

We present a new technique using a frequency comb laser and optical cavities for performing ultrafast transient absorption spectroscopy with improved sensitivity. Resonantly enhancing the probe pulses, we demonstrate a sensitivity of…

光学 · 物理学 2016-04-05 Melanie A. R. Reber , Yuning Chen , Thomas K. Allison

Despite the decades that have passed since the discovery of ultrafast transient absorption spectroscopy and its apparent simplicity, this method is still often subject to experimental errors and misinterpretations when applied to 2D…

介观与纳米尺度物理 · 物理学 2025-12-05 Yuri D. Glinka

An ultrafast single-pixel optical 2D imaging system using a single multimode fiber (MF) is proposed. The MF acted as the all-optical random pattern generator. Light with different wavelengths pass through a single MF will generator…

Ultrafast spectroscopy is an important tool for studying photoinduced dynamical processes in atoms, molecules, and nanostructures. Typically, the time to perform these experiments ranges from several minutes to hours depending on the choice…

The possibility of spatially resolving the optical properties of atomically thin materials is especially appealing as they can be modulated at the micro- and nanoscale by reducing their thickness, changing the doping level or applying a…

介观与纳米尺度物理 · 物理学 2016-03-23 Andres Castellanos-Gomez , Jorge Quereda , Herko P. van der Meulen , Nicolás Agraït , Gabino Rubio-Bollinger

Presented is a novel way to combine snapshot compressive imaging and lateral shearing interferometry in order to capture the spatio-spectral phase of an ultrashort laser pulse in a single shot. A deep unrolling algorithm is utilised for the…

We have developed a single-shot imaging technique that can capture ultrafast events occurring on femtosecond to picosecond time scales. The technique is based on an optical pump-probe method, in which multiple time-delayed femtosecond…

仪器与探测器 · 物理学 2018-11-14 Sarang Yeola , Donghoon Kuk , Ki-Yong Kim

Recording of transient absorption microscopy images requires fast detection of minute optical density changes, which is typically achieved with high-repetition-rate laser sources and lock-in detection. Here, we present a highly flexible and…

We have developed a single-shot terahertz time-domain spectrometer to perform optical-pump/terahertz-probe experiments in pulsed, high magnetic fields up to 30 T. The single-shot detection scheme for measuring a terahertz waveform…

An apporach for the sensing of small amounts of chemical and biochemical material is presented. A frequency selective surface (FSS) made from asymmetric split ring resonators (aDSR) is excited with free space radiation. Due to interference…

应用物理 · 物理学 2021-04-13 Christian Debus , Peter Haring Bolívar

Single-shot characterization techniques are crucial when dealing with shot-to-shot pulse-shape fluctuations (e.g., unstable laser systems, high-power, or with low repetition rate) since the scanning configurations cannot measure single…

光学 · 物理学 2025-07-23 Cristian Barbero , Íñigo J. Sola , Benjamín Alonso

The surface morphology of metal influences its optical absorptivity. Recent experiments have demonstrated that the femtosecond laser induced surface structures on metals could be dynamically controlled by the fluence of laser and the number…

应用物理 · 物理学 2018-11-14 Muhammad Zubair , Yee Sin Ang , Kelvin J. A. Ooi , L. K. Ang

High-Impedance Surfaces (HIS) comprising lossy Frequency Selective Surfaces (FSS) are employed to design thin electromagnetic absorbers. The structure, despite its typical resonant behavior, is able to perform a very wideband absorption in…

经典物理 · 物理学 2010-07-27 Filippo Costa , Agostino Monorchio , Giuliano Manara

The realm of classical phase retrieval concerns itself with the arduous task of recovering a signal from its Fourier magnitude measurements, which are fraught with inherent ambiguities. A single-exposure intensity measurement is commonly…

计算机视觉与模式识别 · 计算机科学 2023-11-21 Yixiao Yang , Ran Tao , Kaixuan Wei , Jun Shi

Hyperspectral imaging is an important tool having been applied in various fields, but still limited in observation of dynamic scenes. In this paper, we propose a snapshot hyperspectral imaging technique which exploits both spectral and…

仪器与探测器 · 物理学 2018-12-26 Chao Deng , Xuemei Hu , Jinli Suo , Yuanlong Zhang , Zhili Zhang , Qionghai Dai
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