相关论文: Nonlinear interferometric vibrational imaging

Molecular ions can be held in a chain of laser-cooled atomic ions by sympathetic cooling. This system is ideal for performing high-precision molecular spectroscopy with applications in astrochemistry and fundamental physics. Here we show…

Information from frequency bands in biomedical time series provides useful summaries of the observed signal. Many existing methods consider summaries of the time series obtained over a few well-known, pre-defined frequency bands of…

We present an approach for improving spatial frequency sampling in active incoherent millimeter-wave (AIM) imaging systems using frequency diversity. AIM imaging relies on active transmission of spatio-temporally incoherent signals to…

Raman scattering is the inelastic process where photons bounce off molecules, losing energy and becoming red-shifted. This weak effect is unique to each molecular species, making it an essential tool in e.g. spectroscopy and label-free…

We develop a computational framework to examine the factors responsible for scattering-induced distortions of coherent anti-Stokes Raman scattering (CARS) signals in turbid samples. We apply the Huygens-Fresnel Wave-based Electric Field…

Interferometry can measure the shape or the material density of a system that could not be measured otherwise by recording the difference between the phase change of a signal and a reference phase. This difference is always between $-\pi$…

We have developed a modified Michelson interferometer type Raman laser system to manipulate cold 87 Rb atoms to interfere. A frequency modulated continuous wave technique was introduced to determine the optical path difference, thus…

We demonstrate how a narrowband pump and a broadband spectrum can be spatially multiplexed by selective coupling them in two distinct modes of a few-mode microstructure fiber. The first mode carries most of the input pump energy, and…

Transmission electron microscopy and spectroscopy currently enable the acquisition of spatially resolved spectral information from a specimen by focusing electron beams down to a sub-Angstrom spot and then analyzing the energy of the…

Experimental Stokes vector spectroscopy characterizes polarization state noise in nonlinear fiber transmission. Noise bandwidths of a few MHz are observed from XPM-blurred receive SOPs using a polarization scrambling interferometer. This…

We present measurements of the complete spatio-temporal Fourier spectrum of Faraday waves. The Faraday waves are generated at the interface of two immiscible index matched liquids of different density. By use of a new absorption technique…

Raman scattering signal can be enhanced through localization of incident field into sub-wavelength hot-spots through plasmonic nano-structures (Surface-enhanced Raman scattering-SERS). Recently, further enhancement of SERS signal via…

Quantum entanglement has emerged as a great resource for interactions between molecules and radiation. We propose a new paradigm of stimulated Raman scattering with entangled photons. A quantum ultrafast Raman spectroscopy is developed for…

Nonlinear interferometry with entangled photons allows for characterizing a sample without detecting the photons interacting with it. This method enables highly sensitive optical sensing in the wavelength regions where efficient detectors…

Measuring an electric field waveform beyond radio frequencies is often accomplished via a second-order nonlinear interaction with a laser pulse shorter than half of the field's oscillation period. However, synthesizing such a gate pulse is…

We use both simulated and real quasar light curves to explore modeling photometric reverberation-mapping (RM) data as a stochastic process. We do this using modifications to our previously developed RM method based on modeling quasar…

Many reports on stimulated Raman scattering in mixtures of Raman-active and noble gases indicate that the addition of a dispersive buffer gas increases the phase-mismatch to higher-order Stokes and antiStokes sidebands, resulting in…

Existing permanental processes often impose constraints on kernel types or stationarity, limiting the model's expressiveness. To overcome these limitations, we propose a novel approach utilizing the sparse spectral representation of…

Nonlinear radio waves modulate the plasma, scatter on the modulations, and develop an intermittent power spectrum -- perhaps. Rudiments of theory, numerical simulations, and qualitative modeling of nonlinear scattering are presented.…

We provide conclusive demonstration of vibrational pumping under Surface Enhanced Raman Scattering (SERS) conditions by performing anti-Stokes/Stokes ratio measurements down to 10 K using dried silver colloids, the dye rhodamine 6G and 676…