相关论文: Theory of selective excitation in Stimulated Raman…
The classical stimulated Raman scattering system describing resonant interaction between two electromagnetic waves and a fast relaxing medium wave is studied by introducting a systematic perturbation approach in powers of the relaxation…
The coherence of two, coupled two-level systems, representing vibrational modes in a semiclassical model, is calculated in weak and strong fields for various coupling schemes and for different relative phases between initial state…
The interaction between ultrashort light pulses and non-absorbing materials is dominated by Impulsive Stimulated Raman Scattering (ISRS). The description of ISRS in the context of pump\&probe experiments is based on effective classical…
Interaction of a high intensity short laser pulse with near-critical plasmas allows to achieve extremely high coupling efficiency and transfer laser energy to energetic ions. One dimensional Particle-In-Cell (PIC) simulations are considered…
Stimulated Raman scattering (SRS) in its strongly nonlinear, kinetic regime is controlled by a technique of deterministic, strong temporal modulation and spatial scrambling of laser speckle patterns, called Spike Trains of Uneven Duration…
We explore coherent control of stimulated Raman scattering in the nonimpulsive regime. Optical pulse shaping of the coherent pump field leads to control over the stimulated Raman output. A model of the control mechanism is investigated.
A consistent semiquantitative theoretical analysis of electronic Raman scattering from many-electron quantum dots under resonance excitation conditions has been performed. The theory is based on random-phase-approximation-like wave…
We demonstrate the acquisition of stimulated Raman scattering spectra with the use of a single femtosecond pulse. High resolution vibrational spectra are obtained by shifting the phase of a narrow band of frequencies in the broadband input…
A completely quantum description of Raman process is used to investigate the nonclassical properties of the modes in the stimulated, spontaneous and partially spontaneous Raman process. Both coherent scattering (where all the initial modes…
We explain quantitatively why resonant Raman scattering spectroscopy, an extensively used experimental tool in studying elementary electronic excitations in doped low dimensional semiconductor nanostructures, always produces an observable…
We treat theoretically the two-pulse plane-wave propagation problem associated with the stimulated Raman process. A strong pump pulse and a weak probe pulse interact self-consistently during mutual propagation through a medium in the…
Raman scattering is a chemically selective probing mechanism with diverse applications in industry and clinical settings. Yet, most samples are optically opaque limiting the applicability of Raman probing at depth. Here, we demonstrate…
We present theoretical results concerning inelastic light (Raman) scattering from semiconductor quantum dots. The characteristics of each dot state (whether it is a collective or single-particle excitation, its multipolarity, and its spin)…
Photophysical and photochemical processes are ruled by the interplay between transient vibrational and electronic degrees of freedom, which are ultimately determined by the multidimensional potential energy surfaces (PESs). Differences…
Excited-state vibrational dynamics in molecules can be studied by an electronically off-resonant Raman process induced by a probe pulse with variable delay with respect to an actinic pulse. We establish the connection between several…
Parametric spin wave excitation allows studying a variety of nonlinear phenomena, such as magnon scattering. In patterned micro- and nanostructures the magnon spectra is discrete and translational symmetry is broken, which means allowable…
Excited-state vibrations are crucial for determining photophysical and photochemical properties of molecular compounds. Stimulated Raman scattering can coherently stimulate and probe molecular vibrations with optical pulses, but it is…
Stimulated Raman scattering of a laser pump pulse seeded by a Stokes pulse generically leaves a two-level medium initially at rest in an excited state constituted of static solitons and radiation. The soliton birth manifests as sudden very…
The capability to excite, probe, and manipulate vibrational modes is essential for understanding and controlling chemical reactions at the molecular level. Recent advancements in tip-enhanced Raman spectroscopies have enabled the probing of…
Ultrafast characterization and control of many-body interactions and elementary excitations are critical to understanding and manipulating emergent phenomena in strongly correlated systems. In particular, spin interaction plays an important…