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By resorting to measurements of physically characterizing observables of water samples perturbed by the presence of Nafion and by iterative filtration processes, we discuss their scale free, self-similar fractal properties. By use of…

综合物理 · 物理学 2013-12-31 A. Capolupo , E. Del Giudice , V. Elia , R. Germano , E. Napoli , M. Niccoli , A. Tedeschi , G. Vitiello

We study the response of a spherical colloid under alternating electric fields (AC-fields) by mesoscopic simulation method, accounting in full for hydrodynamic and electrostatic interactions. We focus on a special case of uncharged…

软凝聚态物质 · 物理学 2013-04-17 Jiajia Zhou , Friederike Schmid

We present a comprehensive computational framework for reproducing the full X-ray absorption fine structure (XAFS) through quantum-chemical simulations. The near-edge region is accurately captured using an efficient implementation of…

材料科学 · 物理学 2025-12-04 Philipp Hönicke , Yves Kayser , Pouya Partovi-Azar

Effects of presence of ions, at moderate to high concentrations, on dynamical properties of water molecules are investigated through classical molecular dynamics simulations using two well known non-polarizable water models. Simulations…

软凝聚态物质 · 物理学 2015-01-14 Upayan Baul , Satyavani Vemparala

We briefly review recent theoretical and simulation studies of charged colloidal dispersions in alternating electric fields (AC fields). The response of single colloid to an external field can be characterized by a complex polarizability,…

软凝聚态物质 · 物理学 2014-01-09 Jiajia Zhou , Friederike Schmid

A good representation of mesoscopic fluids is required to combine with molecular simulations at larger length and time scales (De Fabritiis {\it et. al}, Phys. Rev. Lett. 97, 134501 (2006)). However, accurate computational models of the…

流体动力学 · 物理学 2015-06-26 G. De Fabritiis , M. Serrano , R. Delgado-Buscalioni , P. V. Coveney

Electrolyte solutions at high concentration are indispensable and yet poorly understood. In particular, the extent of speciation -- the formation of complexes composed of multiple species -- in concentrated ionic solutions is very…

In Molecular Dynamics (MD) simulations, interactions between water molecules and graphitic surfaces are often modeled as a simple Lennard-Jones potential between oxygen and carbon atoms. A possible method for tuning this parameter consists…

介观与纳米尺度物理 · 物理学 2015-06-03 Giulio Scocchi , Danilo Sergi , Claudio D'Angelo , Alberto Ortona

The study of the modification of interfacial properties between an organic solvent and aqueous electrolyte solutions is presented by using electrostatic Dissipative Particle Dynamics (DPD) simulations. In this article the parametrization…

化学物理 · 物理学 2012-11-29 E. Mayoral , E. Nahmad-Achar

Alkali halide (100) crystal surfaces are poorly wetted by their own melt at the triple point. We carried out simulations for NaCl(100) within the well tested BMHFT model potential. Calculations of the solid-vapor, solid-liquid and…

材料科学 · 物理学 2008-09-25 D. Ceresoli , T. Zykova-Timan , U. Tartaglino , E. Tosatti

Diamondoids are promising materials for applications in catalysis and nanotechnology. Since many of their applications are in aqueous environments, to understand their function it is essential to know the structure and dynamics of the water…

介观与纳米尺度物理 · 物理学 2022-11-29 Karol Palczynski , Thorren Kirschbaum , Annika Bande , Joachim Dzubiella

Knowledge of the vapor-liquid equilibrium (VLE) properties of molten salts is important in the design of thermal energy storage systems for solar power and nuclear energy production applications. The high temperatures involved make their…

统计力学 · 物理学 2024-06-19 Leann Tran , Jiri Skvara , William R. Smith

A novel atomistic-continuum method (ACM) based on finite element method (FEM) is proposed to numerically simulate the nano-scaled Poisson's ratio and Young's modulus effect of Lithium (Li) body-centered cubic (BCC) structure. The potential…

材料科学 · 物理学 2016-09-08 C. -Y. Chou , C. Yuan , Chung-Jung Wu , K. -N. Chiang

The interaction of mass-selected atomic clusters and nanoparticles with surfaces attracts strong interest in view of fundamental research and technological applications. Understanding dynamics of the deposition process is important for…

原子与分子团簇 · 物理学 2021-07-12 Yannick Fortouna , Pablo de Vera , Alexey Verkhovtsev , Andrey V. Solov'yov

Although electrolyte density measurements have been reported for over a century, employing them to obtain accurate partial molar volume (PMV) profiles as a function of salt concentration has remained elusive. Obtaining such curves requires…

The Angstrom-scale transport characteristics of water and six different solutes, methanol, ethanol, 2-propanol, urea, Na+, and Cl-, were studied for a polyamide reverse osmosis (RO) membrane, FT-30, using non-equilibrium molecular dynamics…

计算物理 · 物理学 2016-07-18 Meng Shen , Sinan Keten , Richard M. Lueptow

Water scarcity is a reality in our world, and scenarios predicted by leading scientists in this area indicate that it will worsen in the next decades. However, new technologies based in low-cost seawater desalination can prevent the worst…

软凝聚态物质 · 物理学 2020-06-24 João P. K. Abal , José Rafael Bordin , Marcia C. Barbosa

Platinum-water interfaces underpin many electrochemical energy conversion processes. However, despite decades of research, the real-space liquid structure of these interfaces remains elusive. Using three-dimensional atomic force microscopy…

材料科学 · 物理学 2025-09-09 Yitong Li , Qian Ai , Lalith Krishna Samanth Bonagiri , Yingjie Zhang

Molecular dynamics simulations of water with both multi-Kr and single Kr atomic solutes are carried out to implement quasi-chemical theory evaluation of the hydration free energy of Kr(aq). This approach obtains free energy differences…

化学物理 · 物理学 2014-11-07 M. I. Chaudhari , D. Sabo , L. R. Pratt , S. B. Rempe

We studied the interaction between salts and surfactants on the water surface using heterodyne-detected vibrational sum frequency generation (HD-VSFG) spectroscopy. We used sodium dodecyl sulfate (SDS) as a prototype surfactant system at 75…

软凝聚态物质 · 物理学 2025-08-15 Sanghamitra Sengupta , Jan Versluis , Huib J. Bakker