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We consider several fundamental optical phenomena involving single molecules in biased metal-molecule-metal junctions. The molecule is represented by its highest occupied and lowest unoccupied molecular orbitals, and the analysis involves…

介观与纳米尺度物理 · 物理学 2007-05-23 Michael Galperin , Abraham Nitzan

The influence of an intramolecular proton transfer reaction on the conductance of a molecular junction is investigated employing a generic model, which includes the effects of the electric field of the gate and leads electrodes and the…

介观与纳米尺度物理 · 物理学 2017-03-08 Chriszandro Hofmeister , Pedro B. Coto , Michael Thoss

With a specific choice of laser parameters resulting into a so-called exceptional point in the wavelength-intensity plane, it is possible to produce the coalescence of two Floquet resonances describing the photodissociation of the molecule…

量子物理 · 物理学 2010-11-12 Osman Atabek , Roland Lefebvre , M. Lepers , Amine Jaouadi , Olivier Dulieu , V. Kokoouline

Molecular spintronics is made possible by the coupling between electronic configuration and magnetic po- larization of the molecules. For control and application of the individual molecular states it is necessary to both read and write…

介观与纳米尺度物理 · 物理学 2016-04-27 T. Saygun , J. Bylin , H. Hammar , J. Fransson

Nanoscale molecular-electronic devices and machines are emerging as promising functional elements, naturally flexible and efficient, for next generation technologies. A deeper understanding of carrier dynamics in molecular junctions is…

介观与纳米尺度物理 · 物理学 2018-04-04 K. Beltako , F. Michelini , N. Cavassilas , L. Raymond

We investigate the influence of external laser excitations on the average current through bridged molecules. For the computation of the current, we use a numerically very efficient formalism that is based on the Floquet solutions of the…

化学物理 · 物理学 2007-05-23 Sigmund Kohler , Jörg Lehmann , Sébastien Camalet , Peter Hänggi

Intense time-periodic laser fields can transform the electronic structure of a solid into strongly modified Floquet-Bloch bands. While this suggests multiple pathways to induce electronic orders such as superconductivity or charge density…

强关联电子 · 物理学 2019-01-14 Nagamalleswararao Dasari , Martin Eckstein

We demonstrate experimentally a method of varying the degree of directionality in laser-induced molecular rotation. To control the ratio between the number of clockwise and counter-clockwise rotating molecules (with respect to a fixed…

化学物理 · 物理学 2021-05-05 Alexander A. Milner , Valery Milner

While experiments with one or two quantum emitters have become routine in various laboratories, scalable platforms for efficient optical coupling of many quantum systems remain elusive. To address this issue, we report on chip-based systems…

We introduce a new scheme for controlling the sense of molecular rotation. By varying the polarization and the delay between two ultrashort laser pulses, we induce unidirectional molecular rotation, thereby forcing the molecules to rotate…

量子物理 · 物理学 2015-05-13 Sharly Fleischer , Yuri Khodorkovsky , Yehiam Prior , Ilya Sh. Averbukh

Recent studies have attracted widespread attention on magnet-superconductor hybrid systems with emergent topological superconductivity. Here, we present the Floquet engineering of realistic two-dimensional topological nodal-point…

超导电性 · 物理学 2024-04-12 Zhen Ning , Junjie Zeng , Da-Shuai Ma , Dong-Hui Xu , Rui Wang

To develop active nanomaterials that can instantly respond to external stimuli with designed mechanical motions is an important step towards the realization of nanomachines and nanorobots. Herein, we present our finding of a versatile…

应用物理 · 物理学 2020-01-08 Zexi Liang , Daniel Teal , Donglei Fan

Many types of molecular motors have been proposed and synthesized in recent years, displaying different kinds of motion, and fueled by different driving forces such as light, heat, or chemical reactions. We propose a new type of molecular…

介观与纳米尺度物理 · 物理学 2010-11-24 Johannes S. Seldenthuis , Ferry Prins , Joseph M. Thijssen , Herre S. J. van der Zant

In recent experiments on ultracold matter, molecules have been produced from ultracold atoms by photoassociation, Feshbach resonances, and three-body recombination. The created molecules are translationally cold, but vibrationally highly…

量子物理 · 物理学 2007-05-23 Christiane P. Koch , José P. Palao , Ronnie Kosloff , Françoise Masnou-Seeuws

A new mechanism of longitudinal confinement of optical energy via coupled plasmon modes is proposed in chains of noble metal nanoparticles embedded in a graded dielectric medium, which is analogous to the confinement of electrons in…

材料科学 · 物理学 2007-05-23 J. J. Xiao , K. Yakubo , K. W. Yu

We report on a theoretical study of a Cs$_2$ molecule illuminated by two lasers and show how it can result in novel quantum dynamics. We reveal that these interactions facilitate the bypass of the non-crossing rule, forming Light-Induced…

化学物理 · 物理学 2024-05-21 Edgar Barriga , Luis E. F. Foa Torres , Carlos Cárdenas

We study how fermions in molybdenum disulfide MoS$_2$ interact with a laser field and a static potential barrier, focusing on the transmission probability. Our aim is to understand and control photon-assisted quantum transport in this…

介观与纳米尺度物理 · 物理学 2026-01-09 Rachid El Aitouni , Aotmane En Naciri , Clarence Cortes , David Laroze , Ahmed Jellal

A new perspective on how to manipulate molecules by means of very strong laser pulses is emerging with insights from the so-called light-induced potentials, which are the adiabatic potential energy surfaces of molecules severely distorted…

化学物理 · 物理学 2016-03-03 Bo Y. Chang , Ignacio R. Sola , Seokmin Shin

We report on inelastic electron tunneling spectroscopy measurements carried out on single molecules incorporated into a mechanically controllable break-junction of Au and Pt electrodes at low temperature. Here we establish a correlation…

介观与纳米尺度物理 · 物理学 2010-11-16 Youngsang Kim , Hyunwook Song , Florian Strigl , Hans-Fridtjof Pernau , Takhee Lee , Elke Scheer

Cavity optomechanical systems enable fine manipulation of nanomechanical degrees of freedom with light, adding operational functionality and impacting their appeal in photonic technologies. We show that distinct mechanical modes can be…

光学 · 物理学 2022-10-05 Karl Pelka , Guilhem Madiot , Rémy Braive , André Xuereb