相关论文: Electric multipole plasmons in deformed sodium clu…

Background: The major challenge for nuclear theory is to describe and predict global properties and collective modes of atomic nuclei. Of particular interest is the response of the nucleus to a time-dependent external field that impacts the…

We report an improved implementation for evaluating the analytical gradients of the random phase approximation (RPA) electron-correlation energy based on atomic orbitals and the localized resolution of identity scheme. The more efficient…

We have studied the multipole polarizability of a graded spherical particle in a nonuniform electric field, in which the conductivity can vary radially inside the particle. The main objective of this work is to access the effects of…

The problems related to the existence of the spurious dipole mode (SDM) in the self-consistent nuclear-structure models are considered. A method is formulated that allows to eliminate coupling of the SDM with the physical modes in the…

The self-consistent separable random-phase approximation (SRPA) model with Skyrme forces is extended to the case of magnetic excitations and applied to the description of spin-flip and orbital M1 giant resonances in the isotopic chain…

The present work demonstrates a robust protocol for probing localized electronic structure in condensed-phase systems, operating in terms of a recently proposed theory for decomposing the results of Kohn-Sham density functional theory in a…

The random phase approximation (RPA) is attracting renewed interest as a universal and accurate method for first-principles total energy calculations. The RPA naturally accounts for long-range dispersive forces without compromising accuracy…

We present a calculation of the properties of vibrational states in deformed, axially--symmetric even--even nuclei, within the framework of a fully self--consistent Quasparticle Random Phase Approximation (QRPA). The same Skyrme energy…

Fully microscopic RPA/LDA calculations of the dipole plasmon for very large neutral and charged sodium clusters, Na_N^Z+, in the size range 950 < N < 12050 are presented for the first time. 60 different sizes are considered altogether,…

Plasmon and polariton modes are derived for an ideal semi-infinite (half-space) plasma and an ideal plasma slab by using a general, unifying procedure, based on equations of motion, Maxwell's equations and suitable boundary conditions.…

The status of different extensions of the Random Phase Approximation (RPA) is reviewed. The general framework is given within the Equation of Motion Method and the equivalent Green's function approach for the so-called Self-Consistent RPA…

We explore different variants of the random phase approximation (RPA) to the correlation energy derived from closed-shell ring-diagram approximations to coupled cluster doubles theory. We implement these variants in range-separated…

Within the Energy Density Functional (EDF) approach, the use of mean-field wave-functions deliberately breaking (some) symmetries of the underlying Hamiltonian is an efficient and largely utilized way to incorporate static correlations.…

The accurate computation of non-linear optical properties (NLOPs) in large polymers requires accounting for electronic correlation effects with a reasonable computational cost. The Random Phase Approximation (RPA) used in the adiabatic…

The relative energies of different phases or polymorphs of molecular solids can be small, less than a kiloJoule/mol. Reliable description of such energy differences requires high quality treatment of electron correlations, typically beyond…

We extend the capabilities of correlation energy functionals based on the adiabatic-connection fluctuation-dissipation theorem by implementing the analytical atomic forces within the random phase approximation (RPA), in the context of plane…

The fully self-consistent Random Phase Approximation (RPA) is constructed within the Unitary Correlation Operator Method (UCOM), which describes the dominant interaction-induced short-range central and tensor correlations by a unitary…

We analyze particular two-photon processes as possible means to explore electronic quadrupole states in free small deformed atomic clusters. The analysis is done in the time-dependent local density approximation (TDLDA). It is shown that…

The effects of ground-state correlations on the damping of isovector giant dipole resonances in $LS$ closed shell nuclei $^{16}$O and $^{40}$Ca are studied using extended random-phase-approximation (RPA) approaches derived from the…

We evaluate the stopping and image forces on a charged particle moving parallel to a doped sheet of graphene by using the dielectric response formalism for graphene's $\pi$-electron bands in the random phase approximation (RPA). The forces…