相关论文: Wide range dielectric spectroscopy on glass-formin…
Dielectric spectroscopy covering more than 18 decades of frequency has been performed on propylene carbonate in its liquid and supercooled-liquid state. Using quasi-optic submillimeter and far-infrared spectroscopy the dielectric response…
We have performed dielectric spectroscopy on the molecular glass-formers glycerol, propylene carbonate (PC) and the ionic melts CKN and CRN. The frequency range covers almost 20 decades from some micro-Hz to some THz. The meausrement…
We summarize current developments in the investigation of glassy matter using nonlinear dielectric spectroscopy. This work also provides a brief introduction into the phenomenology of the linear dielectric response of glass-forming…
We analyze dielectric-loss spectra of glass forming salol extending up to 400 GHz allowing for the detection of the high-frequency minimum, where the fast critical dynamics predicted by the mode-coupling theory of the glass transition…
A non-contact scanning-probe-microscopy method was used to probe local near-surface dielectric susceptibility and dielectric relaxation in poly-vinyl-acetate (PVAc) near the glass transition. Dielectric spectra were measured from 10-4 Hz to…
Significant progress has been made in recent years in understanding the dynamics of pure hydrogen-bonded systems by analyzing the spectral shape of various susceptibilities. Monohydroxy- and polyalcohols are currently considered to form…
We present a thorough characterization of the glassy dynamics of three propylene glycols (mono-, di- and trimer) by broadband dielectric spectroscopy. By covering a frequency range of more than 15 decades, we have access to the entire…
We present the results of broadband dielectric spectroscopy on two glass formers with strong Johari-Goldstein beta-relaxations. In addition to the alpha- and beta-relaxation dynamics, the extension of the spectra up to 1 THz also allows…
Advances in high-precision dielectric spectroscopy has enabled access to non-linear susceptibilities of polar molecular liquids. The observed non-monotonic behavior has been claimed to provide strong support for theories of dynamic arrest…
A multispeckle technique for efficiently measuring correctly ensemble-averaged intensity autocorrelation functions of scattered light from non-ergodic and/or non-stationary systems is described. The method employs a CCD camera as a…
Dielectric data on glycerol and propylene carbonate covering 18 decades of frequency are presented and compared to each other. Both materials exhibit qualitatively similar behavior except for marked differences in the high-frequency region…
We present nonlinear dielectric measurements of glass-forming glycerol and propylene carbonate applying electrical fields up to 671 kV/cm. The measurements extend to sufficiently high frequencies to allow for the investigation of the…
We suggest a way to disentangle self- from cross-correlation contributions in the dielectric spectra of glycerol. Recently it was demonstrated for monohydroxy alcohols that a detailed comparison of the dynamic susceptibilities of photon…
We investigated the optical properties of 13 different dielectric materials (slide glass, quartz, Al2O3 (c-cut), DyScO3 (110), KTaO3 (001), LaAlO3 (001), (LaAlO3)0.3-(Sr2AlTaO6)0.7 (001) (LSAT), MgF2 (100), MgO (100), SiC, SrTiO3 (001),…
Transmission electron diffraction is a powerful and versatile structural probe for the characterization of a broad range of materials, from nanocrystalline thin films to single crystals. With recent developments in fast electron detectors…
Optical pump-probe spectroscopy is a powerful tool for the study of non-equilibrium electronic dynamics and finds wide applications across a range of fields, from physics and chemistry to material science and biology. However, a shortcoming…
Brillouin scattering has been used to measure the dynamic structure factor of glycerol as a function of temperature from the high temperature liquid to the glassy state. Our investigation aims at understanding the number and the nature of…
We introduce a dynamic light scattering technique capable of resolving motion that changes systematically, and rapidly, with time. It is based on the visibility of a speckle pattern for a given exposure duration. Applying this to a vibrated…
Dielectric spectra of human blood reveal a rich variety of dynamic processes. Achieving a better characterization and understanding of these processes not only is of academic interest but also of high relevance for medical applications as,…
We introduce a nanomechanical platform for fast and sensitive measurements of the spectrally-resolved optical dielectric function of 2D materials. At the heart of our approach is a suspended 2D material integrated into a nanomechanical…