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Local-susceptibility measurements via the NMR shifts of $^{31}$P and $^{51}$V nuclei in the high-pressure phase of (VO)$_{2}$P$_{2}$O$_{7}$ confirmed the existence of a unique alternating antiferromagnetic chain with a zero-field spin gap…

强关联电子 · 物理学 2007-05-23 J. Kikuchi , K. Motoya , T. Saito , M. Azuma , M. Takano

Magnetic excitations in an array of (VO)_2P_2O_7 single crystals have been measured using inelastic neutron scattering. Until now, (VO)_2P_2O_7 has been thought of as a two-leg antiferromagnetic Heisenberg spin ladder with chains running in…

凝聚态物理 · 物理学 2016-08-31 A. W. Garrett , S. E. Nagler , D. A. Tennant , B. C. Sales , T. Barnes

Magnetic excitations in an array of (VO)2P2O7 single crystals have been measured using inelastic neutron scattering. Until now, (VO)2P2O7 has been thought of as a two-leg antiferromagnetic Heisenberg spin ladder with chains running in the…

统计力学 · 物理学 2008-02-03 Alan Tennant , Stephen Nagler , Ted Barnes , Andrew Garrett , Jose Riera , Brian Sales

$^{75}$As NMR measurements were performed on a polycrystalline sample of spin-1/2 alternating-spin-chain Heisenberg antiferromagnet AgVOAsO$_4$. Temperature-dependent NMR shift $K(T)$, which is a direct measure of the intrinsic spin…

材料科学 · 物理学 2017-12-27 N. Ahmed , P. Khuntia , H. Rosner , M. Baenitz , A. A. Tsirlin , R. Nath

Detailed experiments on single-crystal (VO)_2P_2O_7 continue to reveal new and unexpected features. We show that a model composed of two, independent planes of spin chains with frustrated magnetic coupling is consistent with nuclear…

强关联电子 · 物理学 2009-10-31 G. S. Uhrig , B. Normand

Low-frequency spin dynamics in the S=1/2 antiferromagnetic spin-chain compound \alpha-VO(PO_3)_2 has been studied by means of 31P NMR. The nuclear spin-lattice relaxation rate 1/T_1 at the P site exhibits H^{-1/2} dependence on the applied…

强关联电子 · 物理学 2009-11-07 Jun Kikuchi , Naohiko Kurata , Kiyoichiro Motoya , Touru Yamauchi , Yutaka Ueda

The magnetic susceptibilities chi versus temperature T of powders and single crystals of the ambient-pressure (AP) and high-pressure (HP) phases of (VO)_{2}P_{2}O_{7} are analyzed using an accurate theoretical prediction of chi(T, J1, J2)…

强关联电子 · 物理学 2010-11-12 D. C. Johnston , T. Saito , M. Azuma , M. Takano , T. Yamauchi , Y. Ueda

1H nuclear magnetic resonance (NMR) measurements in [YPc2]0, an organic compound formed by radicals stacking along chains, are presented. The temperature dependence of the macroscopic susceptibility, of the NMR shift and of the spin-lattice…

强关联电子 · 物理学 2015-05-20 F. Branzoli , P. Carretta , M. Filibian , S. Klyatskaya , M. Ruben

We report on our 51V-NMR study of static and dynamical magnetic properties in the quasi-one-dimensional antiferromagnet BaCo2V2O8. Although the NMR spectrum shows well-defined antiferromagnetic (AF) order in the N\'eel ground state, the AF…

$^{51}$V NMR studies on CaV2O4 single crystals and $^{17}$O NMR studies on $^{17}$O-enriched powder samples are reported. The temperature dependences of the $^{17}$O NMR line width and nuclear spin-lattice relaxation rate give strong…

强关联电子 · 物理学 2010-11-17 X. Zong , B. J. Suh , A. Niazi , J. Q. Yan , D. L. Schlagel , T. A. Lograsso , D. C. Johnston

Static and dynamic properties of the quasi-two-dimensional antiferromagnet K$_2$V$_3$O$_8$ have been investigated by $^{51}$V-NMR experiments on nonmagnetic V$^{5+}$ sites. Above the structural transition temperature $T_{\rm{S}}$ = 115 K,…

强关联电子 · 物理学 2019-10-01 H. Takeda , H. Yasuoka , M. Yoshida , M. Takigawa , N. J. Ghimire , D. Mandrus , B. C. Sales

We present the synthesis and a detailed investigation of structural and magnetic properties of polycrystalline NaVOAsO$_4$ by means of x-ray diffraction, magnetization, electron spin resonance (ESR), and $^{75}$As nuclear magnetic resonance…

强关联电子 · 物理学 2019-01-30 U. Arjun , K. M. Ranjith , B. Koo , J. Sichelschmidt , Y. Skourski , M. Baenitz , A. A. Tsirlin , R. Nath

Thermodynamic properties, $^{31}$P nuclear magnetic resonance (NMR) measurements, and density-functional band-structure calculations for $\varepsilon$-LiVOPO$_4$ are reported. This quantum magnet features a singlet ground state and…

强关联电子 · 物理学 2020-06-03 Prashanta K. Mukharjee , K. M. Ranjith , M. Baenitz , Y. Skourski , A. A. Tsirlin , R. Nath

The magnetic behavior of the low-dimensional phosphates (Sr,Ba)_2 Cu(PO_4)_2 and BaCuP_2O_7 was investigated by means of magnetic susceptibility and ^{31}P nuclear magnetic resonance (NMR) measurements. We present here the NMR shift K(T),…

强关联电子 · 物理学 2009-11-10 R. Nath , A. V. Mahajan , N. Buttgen , C. Kegler , A. Loidl

The static and dynamic properties of V^{4+} spins (S = 1/2) in the frustrated square lattice compound Pb2(VO)(PO4)2 were investigated by means of magnetic susceptibility chi and 31P nuclear magnetic resonance (NMR) shift (K) and 31P nuclear…

强关联电子 · 物理学 2010-11-12 R. Nath , Y. Furukawa , F. Borsa , E. E. Kaul , M. Baenitz , C. Geibel , D. C. Johnston

The magnetic properties of Na2CuP2O7 were investigated by means of 31P nuclear magnetic resonance (NMR), magnetic susceptibility, and heat capacity measurements. We report the 31P NMR shift, the spin-lattice 1/T1, and spin-spin 1/T2…

强关联电子 · 物理学 2016-08-31 R. Nath , A. V. Mahajan , N. Buettgen , C. Kegler , J. Hemberger , A. Loidl

Inelastic neutron scattering is used to identify single-particle and continuum spin excitations in the quasi-one-dimensional $S=1/2$ antiferromagnet \ba. In the data analysis, close attention is given to resolution effects. A gap in the…

强关联电子 · 物理学 2007-05-23 A. Zheludev , M. Kenzelmann , S. Raymond , T. Masuda , K. Uchinokura , S. -H. Lee

Neutron-scattering experiments on (VO)_2P_2O_7 reveal both a gapped magnon dispersion and an unexpected, low-lying second mode. The proximity and intensity of these modes suggest a frustrated coupling between the alternating spin chains. We…

强关联电子 · 物理学 2009-10-31 G. S. Uhrig , B. Normand

Single crystals of the spin-gap system $\rm (VO)_2P_2O_7$ have been investigated by means of Raman scattering. At temperatures below T=75 K~$\approx 2\Delta_{01}({\bf k}=0)$, with $\Delta_{01}$ the singlet-triplet gap, a shoulder appears at…

超导电性 · 物理学 2009-10-31 M. Grove , P. Lemmens , G. Güntherodt , B. C. Sales , F. Büllesfeld , W. Assmus

We report the local (NMR) and bulk (magnetization and heat capacity) properties of the vanadium-based S=1/2 uniform spin chain compound Bi6V3O16(Bi4V2O10.66). In the low-temperature {\alpha} phase, the magnetic ions (V4+) are arranged in…

强关联电子 · 物理学 2019-09-19 T. Chakrabarty , I. Heinmaa , V. Yu. Verchenko , P. L. Paulose , R. Stern
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