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We introduce an energy functional for ground-state electronic structure calculations. Its variables are the natural spin-orbitals of singlet many-body wave functions and their joint occupation probabilities deriving from controlled…

化学物理 · 物理学 2016-12-04 Ralph Gebauer , Morrel H. Cohen , Roberto Car

This work presents exchange potentials for specific orbitals calculated by inverting Hartree-Fock wavefunctions. This was achieved by using a Depurated Inversion Method. The basic idea of the method relies upon the substitution of…

原子与分子团簇 · 物理学 2016-10-21 A. M. P. Mendez , D. M. Mitnik , J. E. Miraglia

We benchmark three standard approximations for the many-body problem -- the Hartree-Fock, projected Hartree-Fock, and random phase approximations -- against full numerical configuration-interaction calculations of the electronic structure…

原子物理 · 物理学 2012-08-31 Micah D. Schuster , Calvin W. Johnson , Joshua T. Staker

In the first order of the fine structer constant, the polarization operator of a photon is investigated in a constant and homogeneous magnetic field at arbitrary photon energies. For weak and strong fields H, compared with the Schwinger…

高能物理 - 理论 · 物理学 2016-10-12 V. M. Katkov

It is known that the variational methods are the most powerful tool for studying the Coulomb three-body bound state problem. However, they often suffer from loss of stability when the number of basis functions increases. This problem can be…

原子物理 · 物理学 2016-09-08 V. I. Korobov

In this paper we study the problem of uniqueness of solutions to the Hartree and Hartree-Fock equations of atoms. We show, for example, that the Hartree-Fock ground state of a closed shell atom is unique provided the atomic number $Z$ is…

数学物理 · 物理学 2015-05-20 M. Griesemer , F. Hantsch

A numerical method to solve time-dependent Hartree-Fock-Bogoliubov equation is proposed to treat the case with Gogny effective interaction. To check the feasibility of the method, it is applied to oxygen isotope O20 and small amplitude…

核理论 · 物理学 2007-07-23 Y. Hashimoto , K. Nodeki

The diagonalization of the metrical and canonical Hamilton operators of a scalar field with an arbitrary coupling, with a curvature in N-dimensional homogeneous isotropic space is considered in this paper. The energy spectrum of the…

广义相对论与量子宇宙学 · 物理学 2011-04-20 Yu. V. Pavlov

The current work presents a new single-reference method for capturing at the same time the static and dynamic electron correlation. The starting-point is a determinant wavefunction formed with natural orbitals obtained from a new…

化学物理 · 物理学 2017-08-16 Mario Piris

We first strictly expressed the basic notions and research methods of abstract operators, which systematically expounded the main results of abstract operator theory. By combining abstract operators with the Laplace transform, we can easily…

偏微分方程分析 · 数学 2016-07-05 Guang-Qing Bi , Yue-Kai Bi

We generalize Schroedinger's factorization method for Hydrogen from the conventional separation into angular and radial coordinates to a Cartesian-based factorization. Unique to this approach, is the fact that the Hamiltonian is represented…

量子物理 · 物理学 2022-01-28 Xinliang Lyu , Christina Daniel , James K. Freericks

We present an efficient \textit{ab initio} method for calculating the electronic structure and total energy of strongly correlated electron systems. The method extends the traditional Gutzwiller approximation for one-particle operators to…

强关联电子 · 物理学 2014-07-01 Y. X. Yao , J. Liu , C. Liu , W. C. Lu , C. Z. Wang , K. M. Ho

Ground state energies and decay widths of particle unstable nuclei are calculated within the Hartree-Fock approximation by performing a complex scaling of the many-body Hamiltonian. Through this transformation, the wave functions of the…

核理论 · 物理学 2009-01-23 A. T. Kruppa , P. -H. Heenen , H. Flocard , R. J. Liotta

High harmonic generation in polarizable multi-electron systems is investigated in the framework of multi-configuration time-dependent Hartree-Fock. The harmonic spectra exhibit two cut offs. The first cut off is in agreement with the well…

量子物理 · 物理学 2009-11-11 J. Zanghellini , Ch. Jungreuthmayer , T. Brabec

he properties of excitons formed in spherical quantum dots are studied using the $\mathbf{k}\cdot\mathbf{p}$ method within the Hartree approximation. The spherical quantum dots considered have a central core and several concentric layers of…

介观与纳米尺度物理 · 物理学 2019-10-11 Mariano Garagiola , Omar Osenda

Using effective field theory for a proton and antiproton bound in a Coulomb potential, the shift of the ground state energy level is calculated to arbitrary order in the scattering length. Including the next order contact interaction, the…

核理论 · 物理学 2007-05-23 Xinwei Kong , Finn Ravndal

The atomic third-order open-shell many-body perturbation theory is developed. Special attention is paid to the generation and algebraic analysis of terms of the wave operator and the effective Hamiltonian as well. Making use of…

原子物理 · 物理学 2015-05-19 R. Jursenas , G. Merkelis

It is important to obtain effective operators by integrating out high energy degrees of freedom in physics. We suggest a general method of calculating accurate irrelevant operators in a scattering process without use of equation of motions.…

高能物理 - 唯象学 · 物理学 2011-07-04 N. Haba , K. Kaneta , S. Matsumoto , T. Nabeshima

The polarization operator of a photon in a constant and uniform magnetic field is studied taking into account the radiation width and shift of the Landau levels in both weak and strong fields compared with the critical field…

高能物理 - 唯象学 · 物理学 2019-11-27 V. M. Katkov

Four-component Dirac Hartree--Fock is an accurate mean-field method for treating molecular systems where relativistic effects are important. However, the computational cost and complexity of the two-electron interaction makes this method…

化学物理 · 物理学 2021-06-08 Shichao Sun , Torin Stetina , Tianyuan Zhang , Hang Hu , Edward F. Valeev , Qiming Sun , Xiaosong Li