相关论文: Quantum Tunneling in Ferrimagnetic Nanoparticles C…
This mini-review presents a simple and accessible summary on the fascinating physics of quantum nanomagnets coupled to a nuclear spin bath. These chemically synthesized systems are an ideal test ground for the theories of decoherence in…
A new quantum approach is presented that can account for the description of small ferromagnetic particles magnetization tunneling. An estimate of the saturation value of an external applied magnetic field along the easy axis is obtained. An…
Theoretical foundations of the problem of quantum spin tunneling in magnetic nanostructures are presented. Several model problems are considered in detail, including recent new results on tunneling in antiferromagnetic nanoparticles and…
Interacting spins in quantum magnet can cooperate and exhibit exotic states like the quantum spin liquid. To explore the materialization of such intriguing states, the determination of effective spin Hamiltonian of the quantum magnet is…
Within a wide class of ferromagnetic and antiferromagnetic systems, quantum tunneling of magnetization direction is spin-parity dependent: it vanishes for magnetic particles with half-integer spin, but is allowed for integer spin. A…
We examine the quantum tunneling of magnetization in molecular spin in weak interaction with a bath subject to Redfield master equation. By designing a microscopic model for a multilevel spin system using only a generic Hamiltonian and…
We derive the quantization of magnetic helicity in the solid-state and demonstrate tunable macroscopic quantum tunneling, coherence, and oscillation for a skyrmion spin texture stabilized in frustrated magnets. We also discuss the parameter…
The low-energy physics of systems coupled to their surroundings is understood by truncating to effective Hamiltonians; these tend to reduce to a few canonical forms, involving coupling to "baths" of oscillators or spins. The method for…
Starting from a phenomenological Hamiltonian originally written in terms of angular momentum operators we derive a new quantum angle-based Hamiltonian that allows for a discussion on the quantum spin tunneling. The study of the…
We study theoretically the thermodynamic properties and spin dynamics of a class of magnetic rings closely related to ferric wheels, antiferromagnetic ring systems, in which one of the Fe (III) ions has been replaced by a dopant ion to…
The quantum tunneling of the magnetization vector between excited levels are studied theoretically in single-domain ferromagnetic nanoparticles with biaxial crystal symmetry placed in an external magnetic field at an arbitarily directed…
High energy resolution spectroscopic studies of quantum magnets have proven to be extremely valuable in directly accessing magnetodynamics quantities, such as energy barriers, magnetic interactions, lifetime of excited states and…
This chapter takes a microscopic view of quantum tunneling of magnetization (QTM) in single-molecule magnets (SMMs), focusing on the interplay between exchange and anisotropy. Careful consideration is given to the relationship between…
Process of quantum tunneling of particles in various physical systems can be effectively controlled even by a weak and slow varying in time electromagnetic signal if to adapt specially its shape to a particular system. During an…
Magnetic nano-skyrmions develop quantized helicity excitations, and the quantum tunneling between nano-skyrmions possessing distinct helicities is indicative of the quantum nature of these particles. Experimental methods capable of…
We consider a large spin \bf S in the magnetic field parallel to the uniaxial crystal field, interacting with N >> 1 nuclear spins \bf I_i via Hamiltonian \cal H = -DS_z^2 - H_zS_z+ A{\bf S}\cdot \sum_{i=1}^N {\bf I}_i with A << D, at…
Achieving long-range ferrimagnetic order in purely organic systems remains a major challenge in molecular magnetism. Here we report the synthesis and characterization of heterospin-coupling motifs, formed by covalently linking spin-1/2 and…
We address the characterization of molecular nanomagnets at the quantum level and analyze the performance of local measurements in estimating the physical parameters in their spin Hamiltonians. To this aim, we compute key quantities in…
We review studies on spin-dependent tunneling phenomena in systems containing ferromagnetic nanoparticles. We discuss preparation methods of assembling nanoparticles as well as the mechanisms and results of spin-dependent transport…
Understanding quantum tunneling in many-body systems is crucial for advancing quantum technologies and nanoscale device design. Despite extensive studies of quantum tunneling, the role of interactions in determining directional transport…