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A new method based on quasi-independent parallel simulations approach, replica-averaging, has been developed to study the influence of flow on mechanical force-mediated polymer processes such as denaturation and breaking of bonds. This…

化学物理 · 物理学 2024-06-19 Sagar Kania , Anh H. Nguyen , Alparslan Oztekin , Edmund Webb

Monte Carlo simulations are used to study the conformational properties of a folded semiflexible polymer confined to a long channel. We measure the variation in the conformational free energy with respect to the end-to-end distance of the…

软凝聚态物质 · 物理学 2018-09-05 James M. Polson

The research is important for a molecular theory of liquid and has a wide interest as an example solving the problem when dynamic parameters of systems can be indirectly connected with their equilibrium properties. In frameworks of the…

统计力学 · 物理学 2007-05-23 Andrei N. Yakunin

We present simulation data for the motion of a polymer chain through a regular lattice of impenetrable obstacles (Evans-Edwards model). Chain lengths range from N=20 to N=640, and time up to $10^{7}$ Monte Carlo steps. For $N \geq 160$ we…

软凝聚态物质 · 物理学 2016-08-17 A. Baumgärtner , U. Ebert , L. Schäfer

A brief review of modeling and simulation methods for a study of polymers at interfaces is provided. When studying truly multiscale problems as provided by realistic polymer systems, coarse graining is practically unavoidable. In this…

软凝聚态物质 · 物理学 2009-10-19 Fathollah Varnik , Kurt Binder

We compare Monte Carlo simulations of knotted and unknotted polymers whose ends are connected to two parallel walls. The force $f$ exerted on the polymer is measured as a function of the separation $R$ between the walls. For unknotted…

统计力学 · 物理学 2009-11-07 Oded Farago , Yacov Kantor , Mehran Kardar

By using the blob theory and computer simulations, we investigate the properties of a linear polymer performing a stationary rotational motion around a long impenetrable rod. In particular, in the simulations the rotation is induced by a…

We write exact equations for the thermodynamic properties of a linear polymer molecule confined to walk on a lattice of finite size. The dimension of the space in which the lattice resides can be arbitrary. We also calculate polymer…

综合物理 · 物理学 2011-10-04 Esdmund A. Di Marzio , Charles M. Guttman

We study the thermodynamic properties of a semiflexible polymer confined inside strips of widths L<=9 defined on a square lattice. The polymer is modeled as a self-avoiding walk and a short range interaction between the monomers and the…

统计力学 · 物理学 2007-05-23 Jurgen F. Stilck

Polymer entanglements lead to complicated topological constraints and interactions between neighbouring chains in a dense solution or melt. Entanglements can be treated in a mean field approach, within the famous reptation model, since they…

软凝聚态物质 · 物理学 2007-05-23 S. Kutter , E. M. Terentjev

We study the localisation of lattice polymer models near a permeable interface in two dimensions. Localisation can arise due to an interaction between the polymer and the interface, and can be altered by a preference for the bulk solvent on…

统计力学 · 物理学 2024-07-24 C J Bradly , N R Beaton , A L Owczarek

Molecular dynamics simulation of a generic polymer model is applied to study melts of polymers with different types of intrinsic stiffness. Important static observables of the single chain such as gyration radius or persistence length are…

软凝聚态物质 · 物理学 2017-09-13 Roland Faller , Alexander Kolb , Florian Müller-Plathe

The hydrodynamic lift force that polymers experience near boundaries is known to be a crucial element when considering rheological flows of dilute polymer solutions. Here we develop theory to describe the hydrodynamic lift force on extended…

软凝聚态物质 · 物理学 2015-05-27 Charles E Sing , Alfredo Alexander-Katz

This work addresses the question of whether it is possible to define simple pair-wise interaction terms to approximate free energies of proteins or polymers. Rather than ask how reliable a potential of mean force is, one can ask how…

软凝聚态物质 · 物理学 2009-10-31 Dirk Reith , Thomas Huber , Florian Mueller-Plathe , Andrew E. Torda

We consider a stiff polymer chain in poor solvent and apply a force at one end of the chain. We find that by varying the stiffness parameter, polymer undergoes a transition from the globule state to the folded like state. The conformation…

软凝聚态物质 · 物理学 2015-05-13 Sanjay Kumar , Debaprasad Giri

Motivated by the experiments on DNA under torsion, we consider the problem of pulling a polymer out of a potential well by a force applied to one of its ends. If the force is less than a critical value, then the process is activated and has…

软凝聚态物质 · 物理学 2009-10-31 K. L. Sebastian

We consider polymers attached to the tip of a cone, and the resulting force due to entropy loss on approaching a plate (or another cone). At separations shorter than the polymer radius of gyration R_g, the only relevant length scale is the…

统计力学 · 物理学 2011-12-15 Mohammad F. Maghrebi , Yacov Kantor , Mehran Kardar

The stretching of a polymer chain by a large scale chaotic flow is considered. The steady state which emerges as a balance of the turbulent stretching and anharmonic resistance of the chain is quantitatively described, i.e. the dependency…

chao-dyn · 物理学 2009-10-31 Michael Chertkov

We study the dynamics of a polymer, described as a variant of a Rouse chain, driven by an active terminal monomer (head). The local active force induces a transition from a globule-like to an elongated state, as revealed by the study of the…

统计力学 · 物理学 2020-01-28 Laura Natali , Lorenzo Caprini , Fabio Cecconi

From understanding the sand on the beach to the foam on your beer, soft sphere simulations have been crucial to the study of the amorphous world around us. However, many of the materials we interact with on a daily basis aren't comprised of…

软凝聚态物质 · 物理学 2024-03-18 R. C. Dennis