相关论文: Nonlinear Optical Response of C60 Molecules
We report our theoretical results on the emergence of a nonlinear frequency-asymmetric optical response characteristic of chiral crystal systems with neither spatial inversion symmetry nor mirror symmetry. Based on the group theoretical…
Starting from a multipole expansion of intra- molecular Coulomb interactions, we present configuration interaction calculations of the molecular energy terms of the hole configurations hu^m, m=2-5, of C60^{m+} cations, of the electron…
This article reviews recent progress in quasi-phasematched $\chi^{(2)}$ nonlinear nanophotonics, with a particular focus on dispersion-engineered nonlinear interactions. Throughout this article, we establish design rules for the bandwidth…
We show that standard approximations in nonlinear optics are violated for situations involving a small value of the linear refractive index. Consequently, the conventional equation for the intensity-dependent refractive index, $n(I) = n_0 +…
The total photodisintegration cross sections of three-body nuclei are calculated with semirealistic NN potentials below pion threshold. Full final state interaction with Coulomb force is taken into account via the Lorentz integral transform…
Nonlinear optical responses provide a powerful way to understand the microscopic interactions between laser fields and matter. They are critical for plenty of applications, such as in lasers, integrated photonic circuits, biosensing and…
The three-nucleon (NNN) interaction derived within the chiral effective field theory at the next-to-next-to-leading order (N2LO) is regulated with a function depending on the magnitude of the momentum transfer. The regulated NNN interaction…
Using the sum-rules, the sum-over-states expression for the diagonal term of first hyperpolarizability can be expressed as the sum of three-state interaction terms. We study the behavior of a generic three-state term to show that is…
The conductance of C60 on Cu(100) is investigated with a low-temperature scanning tunneling microscope. At the transition from tunneling to the contact regime the conductance of C60 adsorbed with a pentagon-hexagon bond rises rapidly to…
An important ingredient for applications of nuclear physics to e.g. astrophysics or nuclear energy are the cross sections for reactions of neutrons with rare isotopes. Since direct measurements are often not possible, indirect methods like…
Coulomb breakup of a projectile in the Coulomb field of a fully stripped heavy nucleus is at present one of the most popular experimental methods to obtain information on reactions of interest in nuclear astrophysics. Its theoretical…
We investigate the nuclear and the Coulomb contributions to the breakup cross sections of $^6$Li in collisions with targets in different mass ranges. Comparing cross sections for different targets at collision energies corresponding to the…
We propose an advanced Chebyshev expansion method for the numerical calculation of linear response functions at finite temperature. Its high stability and the small required resources allow for a comprehensive study of the optical…
Coherent nonlinear optical micro-spectroscopy is a frequently used tool in modern material science, as it is sensitive to many different local observables, which comprise, among others, crystal symmetry and vibrational properties. The…
The orientation of individual C60 molecules adsorbed on Cu(100) is reversibly switched when the tip of a scanning tunneling microscope is approached to contact the molecule. The probability of switching rises sharply upon displacing the tip…
The development of nanomaterials with a large nonlinear susceptibility is essential for nonlinear nanophotonics. We show that transition-metal-dichalcogenide (TMD) nanotriangles have a large effective second-order susceptibility…
We propose an approach to sensitively probe the chirality of molecules by measuring their coherent optical absorption spectra. It is shown that quantum dynamics of the cyclic three-level chiral molecules driven by appropriately-designed…
The main objective of the present work is the development of an analytically tractable model of screened electron-electron and electron-exciton interactions in layered systems composed of two parallel semiconductor quantum wells separated…
The Coulomb-nuclear interference (CNI) has recently been used by the TOTEM Collaboration to analyse proton-proton elastic-scattering data from the LHC and to draw physics conclusions. This paper will present an eikonal calculation of the…
The current paper opens a series of papers that are aimed at the determination of barriers that govern the covalent coupling between partners of C60-based composites consisting of two or more fullerenes C60 (C60 dimer and oligomers) (Part…