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The random-phase-approximation semiclassical scheme for description of plasmon excitations in large metallic nanospheres, with radius range 10-60 nm, is formulated in an all-analytical version. The spectrum of plasmons is determined…

介观与纳米尺度物理 · 物理学 2015-05-14 J. Jacak , J. Krasnyj , W. Jacak , R. Gonczarek , A. Chepok , L. Jacak

We present a novel electric-field-resolved approach for probing ultrafast dynamics of localized surface plasmons in metallic nanoparticles. The electric field of the broadband carrier-envelope-phase stable few-cycle light pulse employed in…

Metal nanoparticle surfaces comprise of multiple planes with various atomic arrangements that interact with gases differently1,2. Identification of gas adsorption properties on all facets is an essential prerequisite for rational design of…

材料科学 · 物理学 2015-07-28 Pin Ann Lin , Jonathan Winterstein , John Kohoutek , Henri Lezec , Renu Sharma

The random-phase-approximation semiclassical scheme for description of plasmon excitations in large metallic nanospheres (with radius 10--100 nm) is developed for a case of presence of dynamical electric field. The spectrum of plasmons in…

介观与纳米尺度物理 · 物理学 2015-05-18 W. Jacak , J. Krasnyj , J. Jacak , A. Chepok , L. Jacak , W. Donderowicz , D. Z. Hu , D. M. Schaadt

We aim to clarify the role that absorption plays in nonlinear optical processes in a variety of metallic nanostructures and show how it relates to emission and conversion efficiency. We define a figure of merit that establishes the…

The role of surface collective excitations in the electron relaxation in small metal particles is studied. It is shown that the dynamically screened electron-electron interaction in a nanoparticle contains a size-dependent correction…

凝聚态物理 · 物理学 2009-10-31 T. V. Shahbazyan , I. E. Perakis

Steady-state plasmonic lasing is studied theoretically for a system consisting of many dye molecules arranged regularly around a gold nano-sphere. A three-level model with realistic molecular dissipation is employed to analyze the…

光学 · 物理学 2018-01-31 Yuan Zhang , Klaus Mølmer

We study the effect of Coulomb correlations on the ultrafast optical dynamics of small metal particles. We demonstrate that a surface-induced dynamical screening of the electron-electron interactions leads to quasiparticle scattering with…

凝聚态物理 · 物理学 2009-10-31 T. V. Shahbazyan , I. E. Perakis , J. -Y. Bigot

Collective electronic excitations at metal surfaces are well known to play a key role in a wide spectrum of science, ranging from physics and materials science to biology. Here we focus on a theoretical description of the many-body…

材料科学 · 物理学 2009-11-11 J. M. Pitarke , V. M. Silkin , E. V. Chulkov , P. M. Echenique

Ultrafast pump-probe measurements of plasmonic nanostructures probe the non-equilibrium behavior of excited carriers, which involves several competing effects obscured in typical empirical analyses. Here we present pump-probe measurements…

In this letter we propose an experiment to measure the Kondo effect for magnetic atoms adsorbed on the surface of a metallic nanowire. In addition to the traditional sp-d hybridization, by introducing the strong electromagnetic field of the…

介观与纳米尺度物理 · 物理学 2007-05-23 Ren-Shou Huang , Yia-Chung Chang

We show that nonlinear dynamics in diode lasers with optical injection leads to frequency tunable microwave sidebands which are suitable for atomic physics experiments. We demonstrate the applicability of the sidebands in an experiment…

原子物理 · 物理学 2012-07-24 C. I. Laidler , S. Eriksson

Surface and volume plasmons excited in a metal cluster by moving electron and corresponding inelastic scattering spectra are studied based on the hydrodynamic approach. Along with the bulk losses traditionally taken into account, the…

等离子体物理 · 物理学 2016-04-20 V. B. Gildenburg , V. A. Kostin , I. A. Pavlichenko

Anomalous resonances in properly shaped plasmonic nanostructures can in principle lead to infinite absorption/gain efficiencies over broad bandwidths. By developing a closed-form analytical solution for the fields scattered by conjoined…

介观与纳米尺度物理 · 物理学 2015-06-12 Nasim Mohammadi Estakhri , Andrea Alu

The collective excitation spectra are studied for a multisubband quasi-one-dimensional electron gas on the surface of liquid helium. Different intersubband plasmon modes are identified by calculating the spectral weight function of the…

强关联电子 · 物理学 2009-11-10 Marcos R. S. Tavares , G. -Q. Hai , F. M. Petters , N. Studart

We review studies of superintense laser interaction with solid targets where the generation of propagating surface plasmons (or surface waves) plays a key role. These studies include the onset of plasma instabilities at the irradiated…

光学 · 物理学 2018-04-18 A. Macchi

A canonical quantization scheme for localized surface plasmons (LSPs) in a metal nanosphere is presented based on a microscopic model composed of electromagnetic fields, oscillators that describe plasmons, and a reservoir that describes…

介观与纳米尺度物理 · 物理学 2021-04-28 Kuniyuki Miwa , George C. Schatz

The local field approach and kinetic equation method is applied to calculate the surface plasmon radiative damping in a spheroidal metal nanoparticle embedded in any dielectric media. The radiative damping of the surface plasmon resonance…

介观与纳米尺度物理 · 物理学 2015-06-11 Nicolas I. Grigorchuk

The theory for the electric and magnetic fields energy absorption by small metallic particles subjected to the irradiation by ultrashort laser pulses of different duration in the region of surface plasmon excitation is developed. For the…

介观与纳米尺度物理 · 物理学 2011-07-26 Nicolas I. Grigorchuk , Petro M. Tomchuk

Enhanced optical absorption of molecules in the vicinity of metallic nanostructures is key to a number of surface-enhanced spectroscopies and of great general interest to the fields of plasmonics and nano-optics. Yet, experimental access to…

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