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Using neutron diffraction, we have studied the magnetic field effect on charge structures in the charge-ordered multiferroic material LuFe$_2$O$_4$. An external magnetic field is able to change the magnitude and correlation lengths of the…

强关联电子 · 物理学 2009-04-10 Jinsheng Wen , Guangyong Xu , Genda Gu , S. M. Shapiro Brookhaven National Laboratory

X-ray scattering by multiferroic LuFe2O4 is reported. Below 320 K, superstructure reflections indicate an incommensurate charge order with propagation close to (1/3,1/3,3/2). The corresponding charge configuration, also found by electronic…

We investigated the series of temperature and field-driven transitions in LuFe$_2$O$_4$ by optical and M\"{o}ssbauer spectroscopies, magnetization, and x-ray scattering in order to understand the interplay between charge, structure, and…

Hexagonal LuFe2O4 is a promising charge-order (CO) driven multiferroic material with high charge and spin ordering temperatures. The coexisting charge and spin orders on Fe3+/Fe2+ sites result in novel magnetoelectric behaviors, but the…

In this contribution to the special issue on multiferroics we focus on multiferroicity driven by different forms of charge ordering. We will present the generic mechanisms by which charge ordering can induce ferroelectricity in magnetic…

材料科学 · 物理学 2011-07-22 Jeroen van den Brink , Daniel I. Khomskii

Charge and orbital ordering in the low-temperature monoclinic structure of magnetite (Fe_3O_4) is investigated using LSDA+U. While the difference between t_{2g} minority occupancies of Fe^{2+}_B and Fe^{3+}_B cations is large and gives…

强关联电子 · 物理学 2016-11-02 I. Leonov , A. N. Yaresko , V. N. Antonov , M. A. Korotin , V. I. Anisimov

Dielectric and magnetic phenomena in spin and charge frustrated system RFe2O4 (R is a rare-earth metal ion) are studied. An electronic model for charge, spin and orbital degrees in a pair of triangular-lattice planes is derived. We analyze…

强关联电子 · 物理学 2009-11-13 Makoto Naka , Aya Nagano , Sumio Ishihara

Ferroelectric and ferromagnetic materials possess spontaneous electric and magnetic order, respectively, which can be switched by the corresponding applied electric and magnetic fields. Multiferroics combine these properties in a single…

Neutron diffraction measurements on multiferroic LuFe2O4 show changes in the antiferromagnetic (AFM) structure characterized by wavevector q = (1/3 1/3 1/2) as a function of electric field cooling procedures. The increase of intensity from…

强关联电子 · 物理学 2011-11-09 A. M. Mulders , M. Bartkowiak , J. R. Hester , E. Pomjakushina , K. Conder

The possibility of multiferroicity arising from charge ordering in LuFe2O4 and structurally related rare earth ferrites is reviewed. Recent experimental work on macroscopic indications of ferroelectricity and microscopic determination of…

强关联电子 · 物理学 2013-06-13 Manuel Angst

Trirutile-type LiFe$_2$F$_6$ is a charge-ordered material with Fe$^{2+}$/Fe$^{3+}$ configuration. Here its physical properties, including magnetism, electronic structure, phase transition, and charge ordering, are studied theoretically. On…

材料科学 · 物理学 2017-12-11 Ling-Fang Lin , Qiao-Ru Xu , Yang Zhang , Jun-Jie Zhang , Yan-Ping Liang , Shuai Dong

We performed elastic neutron scattering measurements on the charge- and magnetically-ordered multiferroic material LuFe(2)O(4). An external electric field along the [001] direction with strength up to 20 kV/cm applied at low temperature…

材料科学 · 物理学 2010-04-22 Jinsheng Wen , Guangyong Xu , Genda Gu , S. M. Shapiro

We show results of broadband dielectric measurements on the charge ordered, proposed to be mul- tiferroic material LuFe2O4. The temperature and frequency dependence of the complex permittivity as investigated for temperatures above and…

强关联电子 · 物理学 2013-05-30 Daniel Niermann , Florian Waschkowski , Joost de Groot , Manuel Angst , Joachim Hemberger

LuFe2O4 exhibits multiferroicity due to charge order on a frustrated triangular lattice. We find that the magnetization of LuFe2O4 in the multiferroic state can be electrically controlled by applying voltage pulses. Depending on with or…

强关联电子 · 物理学 2015-05-13 Chang-Hui Li , Fen Wang , Yi Liu , Xiang-Qun Zhang , Zhao-Hua Cheng , Young Sun

The structural features of the charge ordering states in LuFe2O4 are characterized by in-situ cooling TEM observations from 300K down to 20K. Two distinctive structural modulations, a major q1= (1/3, 1/3, 2) and a weak q2=q1/10 + (0, 0,…

材料科学 · 物理学 2009-11-13 Y. Zhang , H. X. Yang , C. Ma , H. F. Tian , J. Q. Li *

We present a self-interaction corrected local spin density (SIC-LSD) study of the electronic structure and possible charge order of magnetite, Fe$_{3}$O$_{4}$. The issue of charge order in magnetite is explored in both cubic and…

强关联电子 · 物理学 2009-11-10 Z. Szotek , W. M. Temmerman , A. Svane , L. Petit , G. M. Stocks , H. Winter

The spin ordering and spin-charge coupling in LuFe2O4 were investigated on the basis of density functional calculations and Monte Carlo simulations. The 2:1 ferrimagnetism arises from the strong antiferromagnetic intra-sheet Fe3+-Fe3+ and…

材料科学 · 物理学 2009-12-22 H. J. Xiang , E. J. Kan , Su-Huai Wei , M. -H. Whangbo , Jinlong Yang

In the manganite Nd0.5Ca0.5MnO3, charge ordering occurs at much higher temperature than the antiferromagnetic order (TCO=250K,TN=160K). The magnetic behavior of the phase TN<T<TCO is puzzling: its magnetization and susceptibility are…

强关联电子 · 物理学 2016-08-31 F. millange , S. de Brion , G. Chouteau

We have carried out a detailed investigation of the magnetic field dependence of charge ordering in La2-xBaxCuO4 (x~1/8) utilizing high-resolution x-ray scattering. We find that the charge order correlation length increases as the magnetic…

超导电性 · 物理学 2009-11-13 Jungho Kim , A. Kagedan , G. D. Gu , C. S. Nelson , T. Gog , D. Casa , Young-June Kim

The possibility of charge order is theoretically examined for the Kondo lattice model in two dimensions, which does not include bare repulsive interactions. Using two complementary numerical methods, we find that charge order appears at…

强关联电子 · 物理学 2013-06-19 Takahiro Misawa , Junki Yoshitake , Yukitoshi Motome
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