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相关论文: Spin-phonon coupling in ZnCr2Se4

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We studied the optical properties of antiferromagnetic ZnCr2Se4 by infrared spectroscopy up to 28,000 cm-1 and for temperatures from 5 to 295 K. At the magnetic phase transition at 21 K, one of the four phonon modes reveals a clear…

强关联电子 · 物理学 2009-04-01 T. Rudolf , Ch. Kant , F. Mayr , M. Schmidt , V. Tsurkan , J. Deisenhofer , A. Loidl

The temperature dependence of eigenfrequencies and intensities of the IR active modes has been investigated for the antiferromagnetic chromium spinel compounds CdCr2O4, ZnCr2O4, ZnCr2S4, ZnCr2Se4, and HgCr2S4 by IR spectroscopy for…

强关联电子 · 物理学 2007-07-05 T. Rudolf , Ch. Kant , F. Mayr , J. Hemberger , V. Tsurkan , A. Loidl

Utilizing magnetic susceptibility, specific heat, thermal expansion and IR spectroscopy we provide experimental evidence that the two subsequent antiferromagnetic transitions in ZnCr_2S_4 at T_N1 = 15 K and T_N2= 8 K are accompanied by…

强关联电子 · 物理学 2009-11-11 J. Hemberger , T. Rudolf , H. -A. Krug von Nidda , F. Mayr , A. Pimenov , V. Tsurkan , A. Loidl

We study the effect of spin-phonon coupling in small magnetic clusters, concentrating on a S=1/2 ring of 4 spins coupled antiferromagnetically. If the phonons are treated as classical variables, there is a critical value of the spin-phonon…

强关联电子 · 物理学 2009-11-11 M. Elhajal , F. Mila

Detailed far-infrared spectra of the optical phonons are reported for antiferromagnetic MnO. Eigenfrequencies, phonon damping and effective plasma frequencies are studied as a function of temperature. Special attention is paid to the phonon…

强关联电子 · 物理学 2008-06-26 T. Rudolf , Ch. Kant , F. Mayr , A. Loidl

The spin-lattice coupling plays an important role in strongly frustrated magnets. In ZnCr$_2$O$_4$, an excellent realization of the Heisenberg antiferromagnet on the ``pyrochlore'' network, a lattice distortion relieves the geometrical…

强关联电子 · 物理学 2009-11-10 A. B. Sushkov , H. D. Drew , O. Tchernyshyov , W. Ratcliff , S. W. Cheong

The infrared phonon spectrum of the spinel CdCr2O4 is measured as a function temperature from 6 K to 300K. The triply degenerate Cr phonons soften in the paramagnetic phase as temperature is lowered below 100 K and then split into a singlet…

材料科学 · 物理学 2009-11-13 R. Valdés Aguilar , A. B. Sushkov , Y. J. Choi , S-W. Cheong , H. D. Drew

We study the magnetically-induced phonon splitting in cubic ACr$_2$O$_4$ (A=Mg, Zn, Cd, Hg) spinels from first principles, and demonstrate that the sign of the splitting, which is experimentally observed to be opposite in CdCr$_2$O$_4$…

材料科学 · 物理学 2016-05-04 Aleksander L. Wysocki , Turan Birol

The isospin-phonon coupling in Sr2IrO4 is investigated by temperature dependent phonon Raman scattering. Anomalous behavior in the frequency of all studied optical phonons is observed below the magnetic transition temperature TN ~240 K. The…

强关联电子 · 物理学 2019-04-23 Kousik Samanta , Danilo Rigitano , Pascoal Jose Giglio Pagliuso , Eduardo Granado

We have studied the influence of magnetic order on the optical phonons of the geometrically frustrated spinel ZnCr$_2$O$_4$ from first-principles. By mapping the first-principles phonon calculations onto a Heisenberg-like model, we…

材料科学 · 物理学 2009-11-11 Craig J. Fennie , Karin M. Rabe

Polar phonons of HgCr2S4 and CdCr2S4 are studied by far-infrared spectroscopy as a function of temperature and external magnetic field. Eigenfrequencies, damping constants, effective plasma frequencies and Lyddane-Sachs-Teller relations,…

强关联电子 · 物理学 2008-06-26 T. Rudolf , Ch. Kant , F. Mayr , J. Hemberger , V. Tsurkan , A. Loidl

Spin-phonon coupling originated from spin-lattice correlation depends upon different exchange interactions in transition metal oxides containing 3d magnetic ions. Spin-lattice coupling can influence the coupling mechanism in magnetoelectric…

We utilize near-infrared femtosecond pulses to investigate coherent phonon oscillations of Ca2RuO4. The coherent Ag phonon mode of the lowest frequency changes abruptly not only its amplitude but also the oscillation-phase as the spin order…

强关联电子 · 物理学 2019-04-24 Min-Cheol Lee , Choong H. Kim , Inho Kwak , C. W. Seo , C. H. Sohn , F. Nakamura , C. Sow , Y. Maeno , E. -A. Kim , T. W. Noh , K. W. Kim

We have investigated the dielectric anomalies associated with spin ordering transitions in the tetragonal spinel Mn$_3$O$_4$, using thermodynamic, magnetic, and dielectric measurements. We find that two of the three magnetic ordering…

材料科学 · 物理学 2007-10-16 R. Tackett , G. Lawes , B. C. Melot , M. Grossman , E. S. Toberer , R. Seshadri

We report on infrared, Raman, magnetic susceptibility, and specific heat measurements on CdCr2O4 and ZnCr2O4 single crystals. We estimate the nearest-neighbor and next-nearest neighbor exchange constants from the magnetic susceptibility and…

强关联电子 · 物理学 2010-02-03 Ch. Kant , J. Deisenhofer , T. Rudolf , F. Mayr , F. Schrettle , A. Loidl , V. Gnezdilov , D. Wulferding , P. Lemmens , V. Tsurkan

Spin-phonon interactions in 2D magnetic materials are crucial in advancing next-generation spintronic devices. Therefore, identifying new materials with significant spin-phonon interactions is of great importance. In this context, MnSe,…

材料科学 · 物理学 2025-02-27 Suman Kalyan Pradhan , Arnab Bera , Soham Das , Yongli Yu , Jicheng Wang , Rui Wu

First-principles calculations reveal large zone-center spin-phonon coupling and magnetically-driven phonon anisotropy in cubic perovskites Sr$M$O$_3$ ($M$=V,Cr,Mn,Fe,Co). In particular, the frequency and splitting of the polar Slater mode…

强关联电子 · 物理学 2012-09-10 Jun Hee Lee , Karin M. Rabe

We have investigated the coupling of lattice with spin via strain interactions in the CoFe2O4/PMN-PT composite system. X-ray diffraction and Raman spectroscopic studies illustrate a remarkable modification in CoFe2O4lattice across Curie…

In order to explore the consequences of spin-orbit coupling on spin-phonon interactions in a set of chemically-similar mixed metal oxides, we measured the infrared vibrational properties of Co$_4B_2$O$_9$ ($B$ = Nb, Ta) as a function of…

We demonstrate that the onset of complex spin orders in ACr$_2$O$_4$ spinels with magnetic A$=$Co, Fe and Cu ions lowers the lattice symmetry. This is clearly indicated by the emergence of anisotropic lattice dynamics -- as evidenced by the…

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